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Submitted on 1 Jan 1984

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NEW METHOD FOR THE SEARCH FOR THE NEUTRON ELECTRIC DIPOLE MOMENT

SUITABLE FOR SMALL REACTORS

R. Golub

To cite this version:

R. Golub. NEW METHOD FOR THE SEARCH FOR THE NEUTRON ELECTRIC DIPOLE MO-

MENT SUITABLE FOR SMALL REACTORS. Journal de Physique Colloques, 1984, 45 (C3), pp.C3-

265-C3-267. �10.1051/jphyscol:1984344�. �jpa-00224061�

(2)

JOURNAL DE PHYSIQUE

Colloque C3, supplbment au n03, Tome

4 5 ,

mars 1984 page

C 3 - 2 6 5

NEW METHOD FOR THE SEARCH FOR THE NEUTRON ELECTRIC DIPOLE MOMENT SUITABLE FOR SMALL REACTORS

R.

Golub

Physik Department E

21,

Technische U n i v e r s i t a t Miinchen,

8046

G a r c h i n g , F.R .G.

RQsumB

-

Une s o u r c e "superthermique" de n e u t r o n s u l t r a f r o i d s contenant une s o l u t i o n d i l u e e de fIe3 p o l a r i s d dans ~e~ p e u t s e r v i r en mdme temps c o m e une s o u r c e , un p o l a r i s e u r , une c h m b r e de resonance magnetique e t un ana- l y s e u r de p o l a r i s a t i o n . On p e u t l ' u t i l i s e r pour r e c h e r c h e r l e moment Blec- t r i q u e d i p o l a i r e du n e u t r o n (edm)

.

A b s t r a c t

-

A superthermal source of Ultra-Cold Neutrons (UCN) c o n t a i n i n g a d i l u t e s o l u t i o n of p o l a r i z e d Re3 i n a e 4 can s e r v e a s a UCN s o u r c e , p o l a r i z e r , magnetic resonance chamber and p o l a r i z a t i o n a n a l y z e r . We d i s c u s s t h e proper- t i e s of such an arrangement when used t o s e a r c h f o r t h e neutron e l e c t r i c d i p o l e moment (edm).

With t h e r e c e n t demonstration

(1)

t h a t t h e s t o r a g e time of UCN i n l i q u i d Helium i s i n reasonable agreement w i t h p r e d i c t i o n s and t h a t t h e "superthermal" UCN source

i s

f e a s i b l e ,

it

now seems a p p r o p r i a t e t o c o n s i d e r new methods of applying t h e extremely high UCN d e n s i t i e s

( 2 )

made p o s s i b l e by t h i s source.

I n t h e "superthermal" UCN source n e u t r o n s w i t h wavelength around

A

-10 a r e s c a t - t e r e d by l i q u i d Eie4 i n t o t h e UCN energy r e g i o n with t h e emission of a phonon. I f t h e l i q u i d Helium

i s

c o n t a i n e d i n s i d e a v e s s e l s u i t a b l e f o r s t o r i n g UCN t h e neutron den- s i t y

w i l l

buil/d up t o a v a l u e (pU N) determined by t h e p r o d u c t i o n r a t e Q =

+

(C

i s

t h e macroscopic c r o s s s e c t i o n For UCN p r o d u c t i o n and $I

i s

t h e i n c i d e n t f l u g ) an8 t h e s t o r a g e time, T , of UCN i n t h e v e s s e l r e s u l t i n g from t h e e f f e c t s of w a l l l o s s e s ,

6

decay, ~ e " ~ s c a t t e r i n g and a b s o r p t i o n by He3.

The UCN s o c o l l e c t e d , can be t r a n s p o r t e d t o a n o t h e r v e s s e l f o r use i n experiments.

For t h e s e a r c h f o r t h e neutron edm by t h e "conventional" method t h e n e u t r o n s must p a s s through a p o l a r i z e r b e f o r e e n t e r i n g t h e experimental chamber where t h e y a r e s u b j e c t e d t o e l e c t r i c and magnetic f i e l d s a r r a n g e d s o a s t o a l l o w t h e d e t e c t i o n o f t h e edm ( 3 ) .

The p r e s e n t super-thermal source

i s

mounted on t h e end of a c o l d neutron quide ex- t e r n a l t o t h e ILL r e a c t o r . However p r e v i o u s work ( 2 ) h a s i n d i c a t e d t h a t

it

should be p o s s i b l e t o o p e r a t e such

a

source i n s i d e a neutron moderator where t h e e f f e c t i v e f l u x averaged over t h e Helium v e s s e l

i s

s e v e r a l t i m e s g r e a t e r t h a n 10'' cm-' s e c - l . This can produce UCN d e n s i t i e s on t h e o r d e r of

10'

U C N / C ~ ~ . A "conventional" way of u s i n g t h e s e UCN would be t o t r a n s p o r t them t o an a p p a r a t u s s i m i l a r t o t h e p r e s e n t one ( 3 ) l o c a t e d o u t s i d e t h e b i o l o g i c a l s h i e l d i n g , through a p o l a r i z e r . However,

it

h a s been suggested

( 4 )

t h a t t h e e n t i r e edm experiment can be performed " i n - s i t u " i n t h e Helium v e s s e l l o c a t e d i n s i d e t h e moderator.

P o l a r i z e d ~ e " s e l e c t i v e l y absorbs neutrons of o n l y one s p i n ( d i r e c t e d o p p o s i t e t o t h e He3 s p i n ) and h a s long been c o n s i d e r e d a s a p o s s i b l e neutron p o l a r i z e r

( 5 ) .

A

Article published online by EDP Sciences and available at http://dx.doi.org/10.1051/jphyscol:1984344

(3)

C3-266 JOURNAL DE PHYSIQUE

superthermal UCN source c o n t a i n i n g p o l a r i z e d He3

w i l l

have d i f f e r e n t s t o r a g e times

r + , r -

( T + / T - = y-/y = Ic>l) f o r t h e two neutron p o l a r i z a t i o n s and hence t h e two p o l a r - i s a t i o n s

w i l l

b u i l d

zp

t o d i f f e r e n t d e n s i t i e s according t o equ.

1.

I f d u r i n g t h e UCN b u i l d up t i m e , a d-c magnetic f i e l d , B o , p a r a l l e l t o t h e ~e~ p o l a r i z a t i o n

i s

a p p l i e d t o g e t h e r with a p e r p e n d i c u l a r r o t a t i n g magnetic f i e l d , B , ( f r e q u e n c y

w )

t h e t o t a l number of UCN i n t h e chamber

w i l l

s e r v e a s an i n d i c a t o r l o f t h e neutron magnetic r e s - onance and one can s e a r c h f o r t h e edm by l o o k i n g f o r t h e e f f e c t of an e l e c t r i c f i e l d on t h e magnetic resonance p r o b a b i l i t y .

hXile t h e a b s o r p t i o n r a t e of UCN by t h e p o l a r i z e d He3

i s

a d i r e c t measure of t h e p o p u l a t i o n o f UCN w i t h a n t i - p a r a l l e l s p i n s ( - s t a t e ) and can b e observed by t h e s c i n - t i l l a t i o n s i n t h e l i q u i d Helium following a neutron a b s o r p t i o n ,

it

seems more prac- t i c a l t o p e r i o d i c a l l y measure t h e t o t a l number of UCN p r e s e n t by i n s e r t i n g a d e t e c - t o r i n t o t h e Helium f i l l e d chamber while s h u t t i n g o f f t h e i n c i d e n t neutron f l u x . The t o t a l number of UCN p r e s e n t can be c a l c u l a t e d from t h e Schroedinger e q u a t i o n and i s shown v s . U =

(w-w

) /y+ I n f i g . 1 f o r K = 4.24 and 52 = 2.12

( 5 i s

t h e s t r e n g t h of t h e r o t a t i n g fieldOmeasured i n u n i t s of y )

,

t h e parameter v a l u e s which g i v e t h e maximum s l o p e of s i g n a l s t r e n g t h v s . a p p l l e d frequency i . e . t h e maximum s e n s i t i v i t y t f o r t h e edm s e a r c h ( 4 ) . Also shown

i s

t h e comparable curve f o r t h e "conventional"

method where t h e r o t a t i n g f i e l d

i s

a p p l i e d f o r s h o r t p e r i o d s a t t h e beginning and end of the measurement time. The c u r v e s a r e f o r s o u r c e s l o c a t e d a t t h e same p o s i t i o n allowing a f a c t o r of 3 f o r volume d i l u t i o n i n t h e c o n v e n t i o n a l method and assuming

100% ~e~ p o l a r i z a t i o n , and t h e same UCN s t o r a g e time i n both v e s s e l s which a r e t a k e n t o be e q u a l i n volume. It i s seen t h a t t h e maximum s l o p e ( p o s i t i o n shown by arrows)

i s

s l i g h t l y l a r g e r f o r t h e c o n v e n t i o n a l method b u t t h i s comparison does n o t allow f o r t r a n s m i s s i o n l o s s e s through t h e n e c e s s a r y UCM g u i d e , p o l a r i z e r s and windows which

w i l l

be n e c e s s a r y i n t h e c o n v e n t i o n a l system. The number of UCN remaining i n t h e v e s s e l

i s

r e l a t e d t o p ( a ) ~ / 2 y

+'

CONVENTIONAL

2 4 6 8 1 0 a

m

Fig. 1- S i g n a l s t r e n q t h vs. a p p l i e d frequency f o r t h e optimized " i n - s i t u " and

"conventional" methods. Arrows i n d i c a t e p o s i t i o n s of maximum s l o p e .

(4)

He3 p o l a r i z a t i o n s on t h e o r d e r of 70-80% have a l r e a d y been o b t a i n e d by l a s e r - o p t i c a l pumping and i n s o l i d ~e~ and

it

seems t h a t

s t i l l

h i g h e r p o l a r i z a t i o n s can be o b t a i n e d by cryogenic t e c h n i q u e s (6). A ~e~ p o l a r i z a t i o n of 90%

w i l l

r e s u l t i n an i n c r e a s e o f

Y+

by 25% over t h a t due t o t h e w a l l l o s s e s a l o n e f o r K = 4.24.

A s shown p r e v i o u s l y

( 2 )

t h e a p p a r a t u s

w i l l

have t o be c a r e f u l l y s h i e l d e d by -30 cm o f cooled Bismuth t o reduce t h e h e a t i n p u t t o a c c e p t a b l e l e v e l s

i n

t h e c a s e o f a h i g h - f l u x source. Under t h e s e c o n d i t i o n s i f we assume t h e s t r u c t u r e surroundinq t h e l i q u i d Helium c o n s i s t s of 4 mm o f Beryllium ( o r Beryllium Oxide) t h e

6

decay r a t e a f t e r 1 y e a r of exposure t o t h e neutron f l u x

w i l l

be about

lo-'

of t h e UCN counting r a t e f o r a 20 l i t r e c y l i n d r i c a l Helium v e s s e l and 10 second counting time. I n addi- t i o n i f t h e d e t e c t o r

i s

i n s e r t e d near t h e c e n t e r of t h e Helium v e s s e l t h e s e

6

r a y s

(which have a range o f a few m i l l i m e t e r s i n l i q u i d Helium) w i l l n o t even r e a c h t h e d e t e c t o r . A much h i g h e r decay r a t e would

be

caused by a c t i v a t i o n of t h e d e t e c t o r

it-

s e l f . T h i s can be d e a l t w i t h by keeping t h e d e t e c t o r i n a s h i e l d e d a r e a while t h e neutron f l u x

i s

a p p l i e d .

A t t h e low temperatures under c o n s i d e r a t i o n h e r e

it

seems u n l i k e l y t h a t

a

convention- a l UCN d e t e c t o r can be used. However bolometers based on b o t h superconducting g r a i n s

( 7 )

and S i l i c o n r e s i s t o r s (8) a r e s e n s i t i v e enough t o d e t e c t n e u t r o n s when covered

w i t h

a Boron o r Uranium containirxg l a y e r . I n t h e c a s e of a B" l a y e r on a S i r e s i s t o r 3x4x.3mm3 a s i n g l e n e u t r o n would produce a p u l s e of about 10 F v o l t s which

i s

about t e n times h i g h e r t h a n t h e thermal n o i s e . I n t h e c a s e of t h e r a t h e r high c o u n t i n g r a t e s t o be expected i n a 20 l i t r e v e s s e l c o n t a i n i n g around

lo3

UCN/cmbith a 10 s e c emptying time

-

2 x 1 0 ~ counts/sec

-

t h e n o i s e

w i l l

be determined by t h e s t a t i s t i c a l f l u c t u a t i o n s i n t h e neutron c o u n t s r a t h e r t h a n by t h e t h e r m a l n o i s e Ln t h e r e s i s t o r even i n t h e c a s e of analogue measurements.

I n

this

p r e l i m i n a r y f e a s i b i l i t y s t u d y we have d e s c r i b e d a method f o r s e a r c h i n g f o r t h e neutron edm which r e p r e s e n t s t h e most s e n s i t i v e technique t h a t one can p r e s e n t l y imagine while o f f e r i n g t h e p o s s i b i l i t y of c a r r y i n g o u t su& experiments a t r e l a - t i v e l y weak neutron sources. I n a d d i t i o n t o t h e problems d i s c u s s e d h e r e t h e r e a r e o t h e r s t h a t

w i l l

have t o be addressed (e.g. t h e e f f e c t s of t h e r a d i a t i o n on t h e i n s u l a t i n g a b i l i t y o f t h e l i q u i d Helium) and s e v e r a l t e c h n i c a l developments

w i l l

be n e c e s s a r y b e f o r e t h e " i n - s i t u " t e c h n i q u e f o r s e a r c h i n g f o r t h e neutron edm can be p u t i n t o p r a c t i c e .

REFERENCES

GOLUB R . , JEWELL C., AGERON P., MAMF'E

W.,

HECKEL B . , KILVINTON I.

Z . ~ h y s .

B

(1983) 187

GOLUB R., B~NING K . , WEBER H. " R e a l i s i e r u n g s s t u d i e zur S p a l l a t i o n s Neutronenquelle, T e i l 111, Ann. C , ed. G.S. Bauer e t

a1 K !

( J i i l i c h ) , KFZ (Karlsruhe) June 1981 PENDLEBURY J . M . , SMITH K.F., GOLUB R., BYRNE J . , MCCOMB T.J.L., S U m R T . , BURNETT S . M . , TAYLOR A.R., HECKEL B., RAMSEY N.F., GREEN K . , MORSE J . , KILVINGTON A . I . , BAKER C.A., CLARKE S.A., MAMPE W . , AGERON P. ( t h i s conference)

GOLUB R., J . d e Physique-Lettres

2

(1983) L-321

JENKIN J.T., "The F u t u r e o f p o l a r i z i n g f i l t e r s a t t h e I.L.L., (unpublished) and P r i v a t e Communication

FROSSATI G . , J . Physique CollOq.

41

(1980) (27-95 See a d d i t i o n a l r e f e r e n c e s i n r e f e r e n c e 4 ) .

DRUKIER A.K., IGALSON J., SNIADAUER L. Nuc. I n s t . Meth.

15$

(1978)91

FROSSATI G .

,

IMBERT D.

,

PECCOUD L.

,

THOULOUZE D.

,

WAKSMAN B. PrOC

.

1 4I n t ~

.

~Conf.

on Low Temp. Physics Otaenimi, Finland (North Iiolland) Aug. 1975 p. 80

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