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NEW DIRECTIONS OF X-RAY SPECTROSCOPY APPLIED TO HOT, LOW DENSITY PLASMAS

E. Källne

To cite this version:

E. Källne. NEW DIRECTIONS OF X-RAY SPECTROSCOPY APPLIED TO HOT, LOW DENSITY PLASMAS. Journal de Physique Colloques, 1987, 48 (C9), pp.C9-335-C9-342.

�10.1051/jphyscol:1987959�. �jpa-00227377�

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JOURNAL DE PHYSIQUE

Colloque C9, s u p p l 6 m e n t au n 0 1 2 , Tome 4 8 , dbcembre 1 9 8 7

NEW DIRECTIONS 0F.X-RAY SPECTROSCOPY APPLIED TO HOT, LOW DENSITY PLASMAS

E . K ~ L L N E

JET Joint Undertaking, GB-Abingdon OX14 3 E A . Great-Britain

ABSTRACT

X-ray spectroscopy has frequently been used a s a major t o o l f o r diagnosing t h e center hot p a r t of fusion plasmas. High resolution X-ray l i n e s p e c t r a and broad band X-ray emission s p e c t r a a r e used t o deduce ion temperatures and impurity concentrations i n t h e plasma. X-ray l i n e s mostly studied a r e t h e n=2 t o 1

t r a n s i t i o n s produced by electron impact excitation. However, time resolved s p e c t r a observed during t h e f u l l plasma discharge have shown t h e importance of other e x c i t a t i o n mechanisms. These new r e s u l t s a r e discussed and implications towards next generation of X-ray instrumentation i n plasma diagnostics is outlined.

1

.

INTRODUCTION

The plasma parameters f o r t h e plasmas produced by t h e presently operating l a r g e tokamaks have entered new regimes compared t o those of t h e plasmas produced by smaller tokamaks previously. Thus, f o r example, i ) t h e ion and electron

temperatures a r e now higher (up t o 30 and 10 keV, respectively, compared t o 8 and 2 keV, previously), i i ) t h e plasma cross s e c t i o n is much l a r g e r (by about a f a c t o r of 5001, i i i ) t h e variations and f l u c t u a t i o n s of parameters a r e l a r g e r both on longer and s h o r t e r time s c a l e s and i v ) the pulselengths a r e longer, up t o 30s (canpared t o

<

500ms before). A l l these changes introduce new requirements on t h e diagnostic

techniques applied t o measure t h e plasma parameters. I n this paper t h e present applications of X-ray spectroscopy t o l a r g e tokamaks w i l l be discussed together with sane prospects f o r f u t u r e developments. Several papers have recently ap ared reviewing application of X-ray spectroscopy i n fusion research i n general and

psi

describing i n d e t a i l t h e b a s i s of sane of t h e s p e c i a l applications of X-ray

spectroscopy2. This paper w i l l highlight sane new d i r e c t i o n s of X-ray spectroscopy i n i t i a t e d by r e s u l t s frcm t h e l a r g e tokamaks.

2. THE PLASMA SOURCE

There a r e presently t h r e e l a r g e tokamaks i n operation i n t h e world, J o i n t European Torus (JET) i n UK, Tokamak Fusion Test Reactor (TFTR) i n USA and JT-60 i n Japan.

The goal f o r these projects is t o produce a burning plasma through t h e reaction

Article published online by EDP Sciences and available at http://dx.doi.org/10.1051/jphyscol:1987959

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C9-336 JOURNAL DE PHYSIQUE

The r a t e parameters f o r t h e r e a c t i o n ( s e e Fig.1) has a maximum around a n i o n temperature of 20

-

30 keV. Presently, t h e plasmas a r e produced using hydrogen, helium and deuterium as f i l l gas, while t r i t i u n is planned t o be used i n t h e l a s t operation period of JET. Ion temperatures achieved up till now a r e i n t h e range of 10

-

30 keV which i s s u f f i c i e n t f o r reaching t h e maximum of t h e c r o s s s e c t i o n of t h e d-t reaction. Electron temperatures a r e around 5

-

1 0 keV, e l e c t r o n d e n s i t i e s lo1'

-

10'' cm'', pulse lengths 5

-

209. Table I s m a r i z e s these parameters and g i v e s t h e t o t a l input power used f o r Ohmic and f o r a d d i t i o n a l h e a t i n g such a s n e u t r a l beams and radiof requency waves.

TABLE I

Plasma and operating parameters

FIG.l Reaction r a t e <ov> as a

function of i o n t m p e r a t u r e f o r d+d and d + t reactions.

The i n t e r i o r of t h e vacuum chamber where t h e plasma is contained i s covered with t i l e s f r a n a low Z element ( f o r JET carbon is used). Therefore, t h e main contaminant of t h e plasma emanates from low Z elements ( i e . , carbon, oxygen) but t h e r e a r e a l s o minor t r a c e s of metal contaminants which have been r e l e a s e d frcm t h e walls of t h e vacuum chamber ( i e . , n i c k e l , chromiun).

3. PLASMA PARAMETERS

The s p a t i a l d i s t r i b u t i o n s of t h e plasma parameters a r e important t o diagnose and t h e v a r i a t i o n s (due t o t r a n s p o r t , e t c ) i n t h e s e s p a t i a l parameters a r e t h e c r u c i a l i s s u e s i n fusion research presently. The i m p u r i t i e s e n t e r i n g t h e plasma w i l l be successively ionized, low Z elements w i l l quickly be completely s t r i p p e d while t h e metals w i l l l o o s e most but not all of t h e i r electrons. The p a r t i a l l y s t r i p p e d ions r a d i a t e and it i s t h i s c h a r a c t e r i s t i c r a d i a t i o n t h a t give s i g n a t o r i e s of t h e plasma parameters i n t h e region where t h e i o n s were de-excited. The t r a n s p o r t of ions, both towards t h e c e n t e r and o u t of t h e c e n t e r ( s e e Fig.2) has up till now only been measured i n d i r e c t l y through measurements of r a d i a l d i s t r i b u t i o n s of o t h e r plasma parameters such as Te(R) and ne(R).

Schematic of JET vacuum vessel.

The dimensions a r e b= 4.2m, R=1.5m with a major r a d i u s of 2.96m.

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.I

- - - FIG.3 Twporal evoiution of a plasma

discharge with a n FP pulse f ran 10 t o 12. Displayed are f r a n l w e r t o upper t r a c e s : i o n t a n p e r a t u r e (Ti keV)

,

e l e c t r o n tanperature (Te keV), RF power

(MW), average e l e c t r o n d e n s i t y - - - * - - -

(ne 1018 ans) and plasma c u r r e n t T

,I

($ MA). (w 2

-

/

I n a d d i t i o n t o t h e s p a t i a l d i s t r i b u t i o n s of plasma parameters t h e r e i s a t a p o r a l evolution during t h e plasma discharge ( s e e Fig.3). The plasma pulse can f o r example be characterized by a s t a r t - u p phase, a quiescent phase, an a d d i t i o n a l heating phase and an ending phase. The various plasma parameters as well as t h e impurity

behaviour must be measured during the various phases with a time r e s o l u t i o n s u f f i c i e n t t o d i s t i n g u i s h behaviour during t h e f a s t o s c i l l a t i o n s as well a s record t h e f u l l plasma discharge.

4. X-RAY SPECTROSCOPY

Around t h e tokamak t h e r e is a manifold of d i f f e r e n t diagnostic equipment; h e r e we s h a l l concentrate on t h e X-ray s p e c t r a n e t e r s presently i n use and t h e a n a l y s i s of d a t a f r a n such i n s t r m e n t s .

The X-ray geometry is chosen with consideration t o source s i z e , source s t r e n g t h , accessible aperture. The source s t r e n g t h , i e . , eg, t h e i n t e n s i t y of a character- i s t i c X-ray l i n e can be calculated. For example, we assume a nickel concentration of lo-"

-

lo-' ne, ne being 1013 and an e l e c t r o n temperature of 3.5 keV. With t h e s e parameters t h e source region ( a s h e l l of 100 cm width) emits a l i n e i n t e n s i t y of l o x 2 photons/an2.s.sr f o r Is-2p t r a n s i t i o n s of ~1"'. This i n t e n s i t y is

concentrated i n one l i n e and emitted during s h o r t t i m e s s o t h e s p e c t r a n e t e r must have a high throughput and a high count r a t e c a p a b i l i t y . The l a t t e r is e s p e c i a l l y important considering t h e background f l u x e s of neutrons and Y : s which a r e detected by t h e X-ray d e t e c t o r with an e f f i c i e n c y of 5

-

1 0%.

FIG.4 Schematics of t h r e e X-ray c r y s t a l spect r a n e t er g e m e t ri es :

a ) Rowland c i r c l e , b) van Hamos c ) double c r y s t a l .

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C9-338 JOURNAX DE PHYSIQUE

Three d i f f e r e n t geanetries have been used f o r X-ray spectraneters a t tokamaks (see Fig.4) m e tht-oughput of these systems a r e canparable (eg., f o r p a r t i c u l a r systems i n use and considered f o r JET: a ) 9.10-' sr.cm2, b) 3.10-' sr.cm2 and c ) 2.10'' sr.cm2 ) while t h e main difference is the accessible bandwidth (0.5%, 7% and oontinuous scanning, respectively) and t h e v e r s a t i l i t y .

The most canmon system i n use a t all t h e t h r e e l a r g e tokamaks is t h e Rowland c i r c l e geometry, and here we w i l l highlight sane of t h e r e s u l t s obtained with such systens with examples f r a n t h r e e l a r g e tokamaks JET, TFIB and JT-60.

4.1 Line p r o f i l e measurements

The Doppler broadened l i n e width o f , f o r example N i 2

'+,

can e a s i l y be measured. The instrumental contribution t o t h e l i n e width is t y p i c a l l y a t e n t h of t h e t o t a l broaderling (Fig.5). The simplicity of t h e method, a l i n e p r o f i l e of a well-resolved l i n e has made t h i s measurenent i n t o one of t h e most important diagnostic measurements f o r ion tenperatures f r a n t h e center of the plasma. However, these measurenents have a l s o revealed t h a t a s i n g l e line-of-sight observation, a s i s usually performed, is not s u f f i c i e n t t o disentangle t h e pure thermal broadening mechanism f r a n e f f e c t s o f , f o r example, r o t a t i o n and turbulence. A t conditions presently prevailing i n t h e l a r g e tokamak plasmas, t h e s h i f t of .the l i n e is comparable t o t h e l i n e broadening during neutral beam i n j e c t i o n (see Fig.5).

Effects of r a d i a l d i s t r i b u t i o n s of eg., t o r o i d a l velocity (Fig.61, ion temperature and electron temperature, a l l influence t h e Doppler broadened 1 i n e p r o f i l e and more detailed analysis is necessary. For example, the absolute l i n e position during the quiescent phase of t h e discharge i s not e a r n , s o it i s not hown whether t h e plasma is r o t a t i n g o r not i n t h i s phase. I n order t o answer t h i s question it would be necessary t o perform absolute wavelength measur ents t o an accuracy of ppn l e v e l , i e . , as is required f o r Lamb s h i f t measurments? Lacking such measurenents (these a r e r e a l l y not f e a s i b l e a t t h e l a r g e tokamaks) data is interpreted as being r e l a t i v e measurements with the assmption of a non-rotating plasma i n t h e quiescent, ohmic phase (Fig.7).

/

FIG.6 Schematic f o r l i n e of s i g h t observations indicating t h e plasma t o r u s with plasma current I

,

neutral beam i n j e c t i o n (NBI)

&d angle of line-of-sight $.

FIG.5 A typical X-ray l i n e p r o f i l e fran N i 2 6 + f o r JET before and during (lower) NBI i n j e c t i o n . A Voigt p r o f i l e f i t t e d t o t h e experimental data is shown.

(6)

There a r e l a r g e p e r i o d i c f l u c t u a t i ons i n plasma p a r m e t e r s , e s p e c i a l l y i n e l e c t r o n t m p e r a t u r e (sawteeth o s c i l l a t i o n s ) , which can be observed a l s o i n t h e i o n

tenperature ( s e e Fig.7). Hmever,. it i s d i f f i c u l t t o s e p a r a t e effects of

f l u c t u a t i o n s i n l i n e widths and l i n e positions and thereby i n t e r p r e t t h e r e S U l t s as being due t o v a r i a t i o n s i n thermal broadening (ie., i o n tenperature) o r plasma r o t a t i o n . A f u r t h e r i n d i c a t i o n t h a t t h e r e a r e phenanena not y e t understood a r e t h e d i f f e r e n t r e s u l t s on thermal broadening obtained by X-ray s p e c t r a and by v i s i b l e s p e c t r f excited by charge exchange with t h e e n e r g e t i c n e u t r a l beams e n t e r i n g t h e plasma

.

Thus, w e have come t o a point i n X-ray spectroscopy when t h e r e q u i r m e n t s f o r l i n e p r o f i l e a n a l y s i s ( i n o r d e r t o g e t s u f f i c i e n t diagnostic r e s u l t s ) are both t o be a b l e t o absolutely c a l i b r a t e t h e l i n e positions t o ppn accuracy and t o be a b l e t o record l i n e p r o f i l e s with higher s e n s i t i v i t y than presently can be achieved.

RF Pulse

5

4

3

FIG.7 Time evolution of i o n

P

i-- 2

tenperature (upper) and t o r o i d a l v e l o c i t y (lower) f o r a JET

plasma discharge ( # 9687) w i t h 1

both n e u t r a l beam i n j e c t i o n (NBI) and r a d i o frequency heating (RF)

.

15

5' E 10

s

3 05 0

5 10 15

WBI

Through a more d e t a i l e d l i n e p r o f i l e a n a l y s i s including t h e f a r wings of t h e l i n e it might be possible t o o b t a i n information on t h e e l e c t r o n and i o n v e l o c i t y

d i s t r i b u t i o n s ; departures frcm Maxwellian d i s t r i b u t i o n s could discern themselves i n t h e t a i l s of l i n e p r o f i l e s , f o r example.

4.2 Line I n t e n s i t i e s

Spectra of H- and H e - l i k e i o n s p e c i e s have been recorded up t o N i presently1 **

(Fig.8). I n t e r p r e t a t i o n of t h e s p e c t r a and t h e associated s a t e l l i t e s t r u c t u r e has advanced t h e atomic theory s o t h a t c a l c u l a t i o n s now e x i s t which can well predict t h e experimental spectra. To simulate f o r example t h e s p e c t r a of Nil6* (Fig.8) it i s n e c g s a r y t o include not only e l e c t r o n impact e x c i t a t i o n f r a n t h e ground s t a t e of N i 2

'+

but a l s o inner-shell e x c i t a t i o n of Li-, Be-, B-like i o n s , d i e l e c t r o n i c recanbination of H-, He-, i-, Be-, and B-like, r a d i a t i v e recanbination and cascade e f f e c t s f r a n high n l e v e l s

'5 .

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JOURNAL DE PHYSIQUE

X-ray s p e c t r a from N i 2 ' + (b) and Ni2'+ ( a ) f r a n JET with a t h e o r e t i c a l f i t t o t h e expande

t

d a t a included as a s o l i d l i n e s

.

Canparisons of experimental and t h e o r e t i c a l X-ray s p e c t r a f o r He-like systems have usually been made using s p e c t r a f r a n the quiescent phase of t h e plasma discharge

"'

observing through a c e n t r e midplane. Single line-of-sight observations of X-ray s p e c t r a a r e influenced by r a d i a l p r o f i l e e f f e c t s f r a n e l e c t r o n tanperatufje, e l e c t r o n density and ion density. Only very few r a d i a l measurements e x i s t s o f a r and we must r e s o r t t o modelling our results with several uniaown parameters9. I n t h e near f u t u r e , however, we w i l l be a b l e t o observe r a d i a l p r o f i l e s of X-ray spectra. This w i l l be a considerable s t e p forward i n t h e information content f r a n X-ray

diagnostic. Fig.9 shows schematic of a double c r y s t a l monochranater t o come i n t o operation a t JET.

FIG.9 Schematics of X-ray double c r y s t a l monochranator on t o p of JET t o observe r a d i a l p r o f i l e s of impurity r a d i a t i o n i n t h e region (1-24) A''.

(8)

Time resolved observations of X-ray s p e c t r a a r e presently made during t h e complete plasma discharge which i n d i c a t e s t h a t during t h e various phases of t h e plasma discharge d i f f e r e n t e x c i t a t i o n m e c h a n i s s a r e i n e f f e c t . So, f o r example, it has been observed (Fig.10) t h a t t h e i n t e n s i t y of t h e resonance l i n e of t h e He-like t i t a n i u n occurs e a r l y i n t h e discharge, much t o o e a r l y t o be explained by t h e ionisation-recanbination balance p i c t u r e which is norm

at t

y w e d t o i n t e r p r e t t h e X-ray s p e c t r a form t h e quiescent phase of t h e discharge

.

I n s t e a d , it i presently proposed t h a t t h e s e e a r l y s p e c t r a a r e excited by e n e r g e t i c e l e c t r o n beans 72

.

Detailed a n a l y s i s of t h e f u l l s p e c t r a with t h e s a t e l l i t e l i n e s is needed f o r i n t e r p r e t a t i o n as well as recording of spectra during t h e s t a r t - u p phase w i n g d i f f e r e n t controlled s t a r t - u p scenarios.

INTENSITY \ - I S M A 8, -45T

I 1

4lvM

FIG.10 Resonance l i n e i n t e n s i t y of r.

Ti2'+ during a plasma discharge ( f r a n ref.11).

-

2 4 6 8

TIME (a) wm

During a d d i t n a l heating t h e r e l a t i v e i n t e n s i t i e s i n t h e X-ray s p e c t r a a l s o change dramatically@ i n d i c a t i n g t h a t ion-ion c o l l i s i o f i beccine i m p r t a n t . Such changes i n t h e X-ray s p e c t r a have been observed previously without a d e t a i l e d explanation f o r t h e observed r e l a t i v e l i n e i n t e n s i t i e s i n t h e He-like spectra. X-ray s p e c t r a f r a n t h e l a r g e tokamaks under t h e d i f f e r e n t operating scenarios, however, show dramatic i n t e n s i t y f l u c t u a t i o n s . It is c l e a r t h a t d e t a i l e d a n a l y s i s of t h e t i m e - r e s q l v e d s p e c t r a is needed i n o r d e r t o understand t h e various atomic processes caning i n t o operation during t h e d i f f e r e n t phases of t h e plasma discharge.

5. FUTURE X-RAY DIAGNQSTIC REQUIREMENTS

I n a d d i t i o n t o n e u t r a l beam i n j e c t t o n frozen p e l l e t s a r e i n j e c t e d i n t o t h e plasma t o increase t h e c e n t r a l e l e c t r o n density. During t h e s h o r t periods of the p e l l e t i n j e c t i o n , t h e s e n s i t i v i t y of t h e presently a v a i l a b l e X-ray s p e c t r a n e t e r s is not s u f f i c i e n t ; thus we need new approaches i n X-ray diagnostics. Given t h e f a c t t h a t t h e X-~gy s p e c t r a can give a multiparameter information f r a n t h e c e n t r a l core of t h e plasma it is a challenge t o think about how t o improve t h e s e n s i t i v i t y by maybe two orders of magnitude, i f possible keeping s u f f i c i e n t r e s o l u t i o n (E/AE = 2

-

5000) i n t h e wavelength region of i n t e r e s t and a l s o being a b l e t o observe t h e s p a t i a l d i s t r i b u t i o n of X-ray s p e c t r a . I t is q u i t e c l e a r t h a t t h e t r a d i t i o n a l approaches presently i n use w i l l not be a b l e t o achieve t h e s e goals and we must use imagination t o s e e t h e next generation of X-ray diagnostic applied t o h o t , low density plasmas.

One approach is t o optimize t h e geanetry t o s u i t t h e source function better16.

Hwever, t h e requirenent of both a l a r g e increase i n t m p r a l r e s o l u t i o n and a p o s s i b i l i t y of s p a t i a l mapping of l a r g e extended sources mjlfht call f o r X-ray instrumentation of s a n e new type, e g , an X-ray calorimeter

,

which can give s u f f i c i e n t energy r e s o l u t i o n and work i n a s p a t i a l a r r a y mode s i m i l a r t o what is presently used f o r X-ray tanopaphy.

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C9-342 JOURNAL DE PHYSIQUE

REFERENCES

1. E KUlne and J KUlne, Physica S c r i p t a Tl7, 152, 1987

2. R Bartirano, i n Varema Workshop on Plasma Diagnostics, Varenna 1986 3. E KXlne and J KUlne, i n Atomic Physics 1 0 , eds. H Narumi and I Shimmura,

1987. ~ 3 9 5

4. M von ~ e l l e r m a n n e t dl., Varema Workshop on Plasma Diagnostics, Varema 1986 5. F Banbarda, e t dl., t o appear Phys. Rev. A (1987)

6. M B i t t e r , et al., Phys. Rev. A 32, 3011(1985)

7. S Sakasai

,

et dl., US-Japan Workshop on Assessment of Atanic Data f o r Fusion, Nagoya, 1987

8. J E Rice, E S Mamar, E K a l n e and 3 K a l n e , Phys. Rev. A 35, 3033(1987) 9. K H Behringer, e t dl., Nucl. Fusion

26,

751 (1986)

10. J Fink, H W Morsi

,

H R5hr and U Schunacher, Max Planck I n s t i t u t f fir Plasmaphysk, Garching, IPP 1 /240, Feb 1987

11. T Kubo, e t dl., i n Proc. Atanic C o l l i s i o m f o r Fusion, Oxford 1987

12. T Kato and K M a s a i , i n W and X-ray Spectroscopy of Astrophysical and Laboratory Plasmas, IAU Coll. No. 102, Beaulieu s u r Mer, France 1987

and T Kato, S Morita, K Masai and S Hayakawa, Phys. Rev. A36,1987

13. H Hsuan, e t al., Phys. Rev. A35, 4280(1987) and i n Proc. Atanic C o l l i s i o n s f o r Fusion, Oxford 1987

14. E KQlne, et dl., Phys. Rev. Lett.

52,

2245(1984)

15. E KXLlne, J K x l n e , E S Matmar and J E Rice, Physica S c r i p t a

2,

551 (1985) 16. H W Schnopper and'B P Byrnak, Danish Space Research I n s t i t u t e , Lyngby, Dennark,

2-87

17.

s

~ ' ~ o l t , Astroph. Lett. Canm. 26, 61 (1987)

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En ouvrant cette page avec Netscape composer, vous verrez que le cadre prévu pour accueillir le panoramique a une taille déterminée, choisie par les concepteurs des hyperpaysages

Chaque séance durera deux heures, mais dans la seconde, seule la première heure sera consacrée à l'expérimentation décrite ici ; durant la seconde, les élèves travailleront sur

A time-varying respiratory elastance model is developed with a negative elastic component (E demand ), to describe the driving pressure generated during a patient initiated

The aim of this study was to assess, in three experimental fields representative of the various topoclimatological zones of Luxembourg, the impact of timing of fungicide

Attention to a relation ontology [...] refocuses security discourses to better reflect and appreciate three forms of interconnection that are not sufficiently attended to