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THE INFLUENCE OF COLLISIONAL DAMPING ON SURFACE PLASMON-POLARITON DISPERSION
A. Boardman, P. Egan
To cite this version:
A. Boardman, P. Egan. THE INFLUENCE OF COLLISIONAL DAMPING ON SURFACE PLASMON-POLARITON DISPERSION. Journal de Physique Colloques, 1984, 45 (C5), pp.C5-179- C5-190. �10.1051/jphyscol:1984526�. �jpa-00224144�
JOURNAL DE PHYSIQUE
Colloque C5, supplément a u n04, Tome 45, avril 1984 page C5-179
T H E INFLUENCE OF COLLISIONAL DAMPING ON SURFACE PLASMON-POLARITON DISPERSION
A . D . Boardman and P . Egan
Department of Pure and AppZied physics, U n i v e r s i t y of SaZford, SaZford M5 4YT, U . K .
Résumé - Nous p r é s e n t o n s une a n a l y s e d é t a i l l é e , a n a l y t i q u e e t numérique, de l ' i n f l u e n c e c o n j o i n t e d e l ' a m o r t i s s e m e n t dû aux c o l l i s i o n s e t de l a d i s p e r s i o n s p a t i a l e s u r l e s p l a s m o n s - p o l a r i t o n s d e s u r f a c e . On t r o u v e que l e s courbes de d i s p e r s i o n p r é s e n t e n t p l u s i e u r s branches, d o n t l ' u n e e s t l e mode couramment admis comme é t a n t à i n v e r s i o n de c o u r b u r e e t q u i c o r r e s p o d à une fréquence r é e l l e e t un nombre d ' o n d e complexe. On montre qu'une i n t e r a c t i o n i m p o r t a n t e e n t r e l ' a m o r - t i s s e m e n t dû aux c o l l i s i o n s e t l a d i s p e r s i o n s p a t i a l e p e u t supprimer c e t t e i n v e r s i o n de c o u r b u r e .
A b s t r a c t - A d e t a i l e d a n a l y t i c a l and n u m e r i c a l a n a l y s i s i s g i v e n o f t h e j o i n t i n f l u e n c e o f c o l l i s i o n a l damping and s p a t i a l d i s p e r s i o n on s u r f a c e p l a s m o n - p o l a r i t o n s . I t i s shown t h a t t h e d i s p e r s i o n has s e v e r a l branches, one o f w h i c h i s t h e c u r r e n t l y a c c e p t e d bend-back mode t h a t a r i s e s u n d e r r e a l f r e q u e n c y and complex wave number assumptions. I t i s p r o v e d t h a t an i m p o r t a n t i n t e r a c t i o n between c o l l i s i o n a l damping and s p a t i a l d i s p e r s i o n o c c u r s t h a t can cause t h i s bend-back t o be suppressed.
1 - INTRODUCTION
The i n c l u s i o n o f c o l l i s i o n a l dampin? i n t o a d e s c r i p t i o n o f s u r f a c e /1,2,3,4/
p l a s m o n - p o l a r i t o n s has been d i s c u s s e d s e v e r a l t i m e s i n t h e l i t e r a t u r e /1,2/.
I t i s n o t a s t r a i g h t f o r w a r d r n a t t e r , e s p e c i a l l y i f t h e model i s r e l a t e d t o a t t e n u a t e d t o t a l r e f l e c t i o n (ATR) experiments /2,5/.
A t t h e b a s i c l e v e l , i f c o l l i s i o n s a r e accounted f o r i n a model o f t h e e l e c t r o n gas t h e n t h e r e s u l t i n g s u r f a c e p o l a r i t o n d i s p e r s i o n e q u a t i o n becomes complex. The wave number k and a n g u l a r f r e q u e n c y UJ a r e then, i n p r i n c i p l e , b o t h complex. The s o l u t i o n o f t h e d i s p e r s i o n e q u a t i o n w i t h complex k and r e a l UJ o r complex UJ and r e a l k a r e n o t t r i v i a l l y d i s t i n c t p o s s i b i l i t i e s . Indeed, i f s p a t i a l d i s p e r s i o n i s i g n o r e d t h e n t h e c u r r e n t p o s i t i o n ernbraces t h e f o l l o w i n g s i t u a t i o n s . I f UJ i s r e a l and k i s complex, and equal t o kr+iki, a p l o t o f UJ a g a i n s t kr f o l l o w s t h e u s u a l c o l l i s i o n l e s s s u r f a c e p o l a r i t o n d i s p e r s i o n c u r v e u p t o t h e r e g i o n UJ UJ / J 2 , where UJ i s
P P
t h e plasma f r e q u e n c y . I t t h e n bends back towards t h e l i g h t l i n e . T h i s has been c o n f i r m e d e x p e r i m e n t a l l y f o r s i l v e r / 6 / . If UJ i s complex, and e q u a l Article published online by EDP Sciences and available at http://dx.doi.org/10.1051/jphyscol:1984526
C5-180 J O U R N A L DE PHYSIQUE
t o wr+iwi and k i s r e a l t h e n a p l o t o f lur a g a i n s t k does n o t show t h i s bend-back and f o l l o w s t h e c o l l i s i o n l e s s s u r f a c e p o l a r i t o n c u r v e . The f i r s t p o s s i b i l i t y corresponds t o an ATR measurement i n w h i c h t h e e x c i t a t i o n f r e q u e n c y i s f i x e d and t h e a n g l e o f i n c i d e n c e i s scanned w h i l e t h e second c o r r e s p o n d s t o a f i x e d a n g l e o f i n c i d e n c e w i t h an e x c i t a r i o n f r e q u e n c y scan.
I t i s t h e bend-back t h a t i s o f t h e g r e a t e s t t h e o r e t i c a l i n t e r e s t and i t i s i m p o r t a n t t o d i s c o v e r what happens when s p a t i a l d i s p e r s i o n i s i n c l u d e d . P a r t of t h e answer suggests i t s e l f i m m e d i a t e l y . A t h i g h enough wave numbers i n t h e e l e c t r o s t a t i c r e g i o n t h e (w,kr) d i s p e r s i o n d i a g r a m must have a s p a t i a l d i s p e r s i o n branch even if a t l o w e r wave numbers i t
i s suspected t h a t bend-back can s t i l l o c c u r . The d e t a i l e d answer i s a c o m p l i c a t e d one. I t i s shown i n t h i s paper t h a t bend-back can s t i l l o c c u r b u t , even though t h e wave numbers i n t h e r e g i o n o v e r w h i c h i t o c c u r s a r e s m a l l , i t can be s t r o n g l y i n f l u e n c e d b y s p a t i a l d i s p e r s i o n . I n d e e d if t h i s i n f l u e n c e i s s t r o n g enough i t can i s o l a t e and suppress t h e phenomenon.
The p r e s e n t a t i o n h e r e c o n c e n t r a t e s on t h r e e (w/w ) l r e g i o n s namely O < ~ ' < 0 . 4 , R=w/w 0 . ? < ~ ~ < 0 . 6 a n d 0 . 6 < 2 ~ < 0 . 9 . T n t h e f i r s t a n d P l a s t r e g i o n a n a l y t i c a l r e s u l t s a r e o b t a i n e d . P' These t h e n p r o v i d e a n i n t e r p r e t a t i o n f o r t h e c e n t r e r e g i o n t h a t fias t o be i n v e s t i g a t e d c o r n p u t a t i o n a l l y . The o u t s f d e r e g i o n s , t h e r e f o r e , c o n t i n u e i n
terms o f l a b e l l i n g i n t o t h e c e n t r e r e g i o n . The p r o b l e m i s c o n v e n i e n t l y a n a l y s e d i n terms o f I4'=c2k2/u2, where c i s t h e v e l o c i t y o f 1 i g h t i n vacuo. The c o n c l u s i o n s drawn a r e t h e n f i n a l l y t r a n s l a t e d i n t o
w,kr p l o t s i n which t h e f e a t u r e s d i s c u s s e d above a r e c l e a r l y d i s p l a y e d . II - THE DISPERSION EQUATION
I f b o t h s p a t i a l d i s p e r s i o n and damping a r e accounted f o r i n a hydrodynamic d e s c r i p t i o n o f t h e e l e c t r o n gas t h e n t h e b u l k t r a n s v e r s e wave number kT and t h e b u l k l o n g i t u d i n a l wave number k L a r e , r e s p e c t i v e l y , g i v e n by /1 ,4/
and
where t h e t i m e dependence i s assumed t o be e-iwt,w i s t h e a n g u l a r f r e q u e n c y , 3 2
v i s a c o n s t a n t e l e c t r o n c o l 1 i s i o n f r e q u e n c y and^^= V F where VF i s t h e Fermi v e l o c i t y . The s u r f a c e mode d i s p e r s i o n e q u a t i o n f o r a vacuum-bounded s e m i - i n f i n i t e plasma, d e r i v e d e a r l i ~ r i n a d i f f e r e n t way by Clemmow and E l g i n /1/ f o r a gaseous e l e c t r o n plasma, i s
{ w 2 - w P / ( i t i v / w ) } ( c 2 k 2 - w 2 ) ~ t u ' ( c ' k 2 - ~ P ' / ( i + i v / w ) ) 1
This d i s p e r s i o n equation involves r a d i c a l s and i s beyond ordinary a n a l y t i c a l methods of determining t h e r o o t s . As i s shown below t h e
' s q u a r i n g up' of t h e equation, very f o r t u n a t e l y , l e a d s t o a cubic e q u a t i o n . The r o o t s of t h i s equation can, of c o u r s e , be w r i t t e n down but may o r may not be piiysically admissible. I t i s necessary then t o develop a r o o t lacceptance' c r i t e r i o n . P a r t of t h e algorithm can be p h y s i c a l ; t h e main approach however, i s t o check whether t h e r o o t s a t i s f i e s t h e o r i g i n a l d i s p e r s i o n e q u a t i o n .
K2
~ f N = K=ck/w and .Q=w/w , then
P P
where
a , 4 c 2 ~ 3 ( Q + i q ) , b=c2n2+2Q2-1+2iQq, d = l - ~ ~ - i Q q ( 2 e 5 ) and q=v/w ,c =B/c. I f N = X ~ % b i s introduced t o equation ( 2 . 4 ) i t reduces even f u r t h e r t o P
x3+qx+r=0 (2.6)
where
q=
-&
( b 3 t b a d ) , r = - ( 2 b 6 + 1 8 a b 3 d t 2 7 a 2 d 2 ) / 2 7 a 3 ( 2 . 7 ) Equation ( 2 . 6 ) has s o l u t i o n sThe cube r o o t s must now be chosen t o make y z = -
2
i . e . yz i s r a t i o n a l Hence t h e t h r e e r o o t s required a r e y t z , h y t ~ ~ z and h2y+hz where X and h 2 a r e1 1
t h e two complex r o o t s of 1 i . e . - ( 1 - i J 3 ) and - - Z ( l t i J 3 j . The general s o l u t i o n i s t h e r e f o r e
3v'2a~=2bb2+(2b3(b3t9ad)+27a2d2+ ~ 2 7 a ~ d ~ ( 4 1 i ~ + 2 7 a d ) l ' ~ + { 2 b 3 ( b 3 t 9 a d ) t 2 7 a 2 d 2 - ~ 7 a 3 d " ( 4 b 3 t 2 7 a d ) } y 3 ( 2 . 9 ) This equation does not involve any approximation and can t h e r e f o r e be used t o study t h e damped and undamped s u r f a c e modes.
I I I - ZERO DAMPING
Although t h i s c a s e has been discussed i n a general form before, i t i s t r u e t o Say t h a t t h e d i s c u s s i o n was very l i m i t e d and t h a t a f u l l and unambiguous development has n ~ t been previously given. Here t h e meaning o f various branches of t h e d i s p e r s i o n diagrarn i s derived and a c l e a r i n d i c a t i o n of which of t h e curves can be l a b e l l e d a s s u r f a c e waves i s given. The
C5-182 JOURNAL DE PHYSIQUE
r e p r e s e n t a t i o n adopted here i s a u s e f u l and r e v e a l i n g one t h a t a l l o w s t h e r o l e o f c o l l i s i o n s and s p a t i a l d i s p e r s i o n t o be u n d e r s t o o d q u i t e c l e a r l y . L e t us f i r s t c o n s i d e r t h e s o l u t i o n s i n t h e r e g i o n 1 i . e . O<n2<0.4.
T h i s r e g i o n i s chosen t o make a b s o l u t e l y c e r t a i n t h a t t h e a n a l y t i c a l work i s v a l i d b u t i n p r a c t i c e t h e upper l i m i t c o u l d be r a i s e d . I n t h i s r e g i o n we s k i r t t o t h e l e f t of t h e p r o b l e m a t i c p o i n t ~ k 0 . 5 t h a t would be s i n g u l a r i f E+O and q 4 . I n t h i s r e g i o n l b 3 1>8x10-~, a d 4 4 ~ 1 0 - ~ and ( a b d ) 3 / 2 Hence i f
q'= 127a3d3(4b3+27ad)l ( 3 . 2 )
t h e n p>>q' and we have f o r t h e r o o t s i n s i d e { 1
so t h a t t h e t h r e e r o o t s NI, N2 and N3 a r e g i v e n b y
3(2)%aN1=2%b2tp%, 3(2)%a% =2zb2-p't/- 1 - ~ ~ ~ / ( 3 ~ ' ) ( 3 . 6 ) where 2/3 r e f e r s t o +/-. Hence
Here N g i v e s t h e l a r g e K a p p r o x i m a t i o n and NZl3 a r e s m a l l p e r t u r b a t i o n s 1
o f O(() f r o m t h e c o l d plasma case and a r e , i n f a c t , t h e f i r s t two terms o f an expansion, g i v e n i n a d i f f e r e n t form, by Clemmow and E l g i n /1/.
The a t t e n u a t i o n c o e f f i c i e n t s o f a vacuum bounded s e m i - i n f i n i t e plasma a r e a, y and 6 where / 4 /
Vacuum: 62 = ~ 2 - ~ 2
Plasma: a 2 = 1+K2-fi2
y 2 = ( [ 2 ~ 2 + l - ~ 2 ) / c 2 I f N1 i s used t h e n
where t h e s i g n s a r e a r b i t r a r y and independent. F o r a s u r f a c e wave a d i s p e r s i o n e q u a t i o n i s a r r i v e d by r e q u i r i n g t h a t al>O,cl>O s o t h e n e g a t i v e s i g n s must be chosen i n e q u a t i o n ( 3 . 1 1 ) .
The d i s p e r s i o n e q u a t i o n i n t h e c o l l i s i o n l e s s case r e d u c e s t o
n 2 a - ( 1 - n 2 ) 6 = ~ ' / y (3.12) Hence on s u b s t i t u t i o n o f al and 61 t h e l e f t - h a n d s i d e o f ( 3 . 1 2 ) g i v e s
and t h e r i g h t hand s i d e g i v e s
B u t we o n l y o b t a i n Rl< O when yl< O. T h i s means t h a t NI c a n n o t r e p r e s e n t a s u r f a c e wave s o l u t i o n .
F o r N we o b t a i n 2 / 3
2 %
2 1-2n2)f p + / - ( ( l - n 2 ) ~ / ( l - 2 n 1 ( 3 . 1 5 )
='fi (
Now u s i n g p o s i t i v e s i g n s f o r a and 6 a s u b s t i t u t i o n i n t o t h e
2/3 2/3
d i s p e r s i o n e q u a t i o n r e s u l t s i n
T h i s i s < O f o r N2 and > O f o r N3, so o n l y N3 r e p r e s e n t s a s u r f a c e wave i n t h i s r e g i o n . N o t e t h a t N3 l i e s below t h e c o l d plasma s o l u t i o n . We t u r n now t o t h e a n a l y t i c a l l y secure r e g i o n I I I i . e . 0.6 < N2< 0.9 where, once a g a i n , t h e l o w e r l i m i t i s approximate and can be l o w e r e d .
I n t h i s r e g i o n
F o r NI, al, 6 , > O w i t h t h e p o s i t i v e s i g n i n e q u a t i o n ( 3 . 1 1 ) . T h i s makes L1'o w h i c h matches R1 f o r yl'O. Hence NI r e p r e s e n t s a s u r f a c e wave s o l u t i o n . F o r r e g i o n III we a l s o o b t a ~ n
F o r N3,@(o)> O,@(&) > O p r o v i d e d t h a t t h e p o s i t i v e r o o t i s t a k e n so t h a t
JOURNAL DE PHYSIQUE
T h i s c h o i c e l e a d s t o
and
(3.25)
5 0 t h a t N3 c a n n o t r e p r e s e n t a s u r f a c e wave. I n t h e same way t a k i n g n e g a t i v e s i g n s f o r t h e r o o t s i n q u e s t i o n (3.19) and (3.22) t o keep
@ ( a )
,a
(6) > 0 o n l y changes t h e i m a g i n a r y p a r t s o f a and 6 w h i c h t h e n c a n c e l o u t . Hence N2 i s a l s o n o t a s u r f a c e wave. T h i s means t h a t i n t h e c o l l i s i o n l e s s s p a t i a l l y d i s p e r s i v e plasma o n l y N3 shown i n F i g . 1 r e p r e s e n t s a s u r f a c e wave i n t h e r e g i o n 1 below R k 0 . 5 w h i l e NI r e p r e s e n t s a s u r f a c e wave i n r e g i o n I I I above ~fi0.5. The above t e c h n i q u e w i l l now be used t o a n a l y s e t h e much more d i f f i c u l t case when c o l l i s i o n a l damping i s i n c l u d e d .I V - EFFECT OF COLLISIONAL DAMPING
The e f f e c t s o f damping may be i n t r o d u c e d t h r o u g h t h e t r a n s f o r m a t i o n s
F i g . 1 - The r e a l p a r t o f t h e r o o t s o f e q u a t i o n s (2.4) f o r t h e c o l l i s i o n l e s s case w i t h s p a t i a l d i s p e r s i o n .
The c o e f f i c i e n t s o f t h e c u b i c e q u a t i o n become a = 4 F , 2 ~ 3 ( ~ + i q ) , ~ = C ~ R ~ + 2 ~ ~ - i + ? i n ~ , c - l - ~ ~ i ~ ~ . The development i s now r e s t r i c t e d t o f i r s t o r d e r i n 5 and w h i c h i s a v a l i d a p p r o x i m t i o n p r o v i d e d t h a t fi2 does n o t approach t o o c l o s e l y t o 1 i n r e g i o n I I I . I n b o t h r e g i o n s 1 and III
100
50
lc
0 f12 -50- 1 00
0.42 0.44 0.46 0.48p0.50 0.52 0.54 0.56
F i g . 2 - E f f e c t o f modest c o l l i s i o n a l damping on t h e r e a l p a r t o f t h e r o o t s o f e q u a t i o n ( 2 . 4 ) . Note t h e ' k i n k ' i n t h e V I branch.
al = + { ( 2 ~ ~ - 1 ) / 2 n ~ + i ~ / c ) , ~ = i { ( 2 ~ ~ - 1 ) / 2 ~ ~ + i n / 5 ) , ~ ~ = 11/2% ( 4 . 3 ) Here, f o r canvenience, we i n t r o d u c e t h e a r t i f i c i a l t r a n s f o r m a t i o n s a c *
6+@ 6 ,
y+pl
t h a t c o n v e r t t h e r e a l and irnaginary p a r t s o f t h e d i s p e r s i o n e q u a t i o n , a f t e r w r i t i n g a=a' t i a " , 6 = 6 ' + i 6" ,y = y ' + i Y u and K=K'+iKU , i n t o
S i n c e we a r e \.)orking t o 0 ( n ) t h i s means t h a t t h e t r u e decay f u n c t i o n s c a n
J O U R N A L DE PHYSIQUE
F i g . 3 - Development o f t h e r e a l p a r t s o f t h e r o o t s o f e q u a t i o n (2.4) as t h e c o l l i s i o n a l damping g e t s s t r o n g e r .
F i g . 4 - D i s p e r s i o n diagram showing k a s a f u n c t i o n o f Kr t h e r e a l p a r t o f K.
H e r e q i s c l o s e t o &65 so t h e r e i s s t r o n g i n t e r a c t i o n between t h e c o l l i s i o n a l and t h e s p a t i a l d i s p e r s i o n branch.
F i g . 5 - A complete p r o g r e s s i o n o f d i s p e r s i o n diagramr from 5 =O,
79
Oshowing t h e u l t i m a t e s u p p r e s s i o n of t h e bend-back.
be r e c o v e r e d a f t e r m u l t i p l y i n g t h r o u g h w i t h a f a c t o r ( 1 - 2 i n / R ) . The p r e s e n c e o f t h i s f a c t o r does n o t , i n any way, a l t e r t h e p r o c e s s o f s o r t i n g o u t w h i c h branch r e p r e s e n t s a s u r f a c e wave.
F o r t h e r o o t N1 we have f r o m t h e l e f t (LI ) and r r i g h t (RI) hand s i d e o f e q u a t i o n s ( 4 . 4 )
These e q u a t i o n s show t h a t f o r (a1)> 0, ( 6 1 ) > O t h e d i s p e r s i o n e q u a t i o n i s s a t i s f i e d o n l y when 2n2>1. T h e r e f o r e , as i n t h e c o l l i s i o n l e s s case
C5-188 J O U R N A L DE PHYSIQUE
N1 r e p r e s e n t s a s u r f a c e wave o n l y i n r e g i o n III.
I n r e g i o n 1 (0<Q2<0.4)
The s u b s t i t u t i o n o f t h e r e a l and i m a g i n a r y p a r t s o f these e q u a t i o n s i n t o t h e r e a l p a r t o f t h e d i s p e r s i o n e q u a t i o n shows t h a t o n l y N3 r e p r e s e n t s a s u r f a c e wave.
I n r e g i o n III f o r 0 . 6 ~ ~ ~ $ 0 . 9 , N ~ , as d i s c u s s e d e a r l i e r , r e p r e s e n t s a s u r f a c e wave b u t i t is now necessary t o see i f N2 and/or N3 a l s o r e p r e s e n t s u r f a c e waves. The e x p r e s s i o n s r e q u i r e d a r e
Note here t h a t t h e decay f u n c t i o n i n t h e vacuum i s , i n f a c t ,
~ ( K ' - Q ' ) $ and n o t $ [ ( ~ ' - ~ ' ) [fi$]'that has been used f o r convenience u p t o now. T h i s decay f u n c t i o n , f o r N2,3, becomes
The use o f e q u a t i o n ( 4 . 1 3 ) l e a d s t o t h e s t r o n g e s t r e q u i r e n e n t , however, w i t h t h e a u t o m a t i c f u l f i l l m e n t o f ( 4 . 1 5 ) . T h i s r e q u i r e m e n t i s f o r t h e r e a l p a r t o f e q u a t i o n ( 4 . 1 3 ) w i t h t h e p o s i t i v e s i g n , and t h e use o f Ne, t o be g r e a t e r t h a n z e r o . I t i s n o t d i f f i c u l t now t o show t h a t t h e N3 r o o t does n o t r e p r e s e n t a s u r f a c e wave b u t Np does. T h e r e f o r e i n r e g i o n III i n a d d i t i o n t o N1 t h e r e i s a branch c o r r e s p o n d i n g t o N2.
T h i s branch o n l y e x i s t s p r o v i d e d t h a t
This r e s t r i c t i o n on n and 5 c o n t r o l s t h e appearance on t h e d i s p e r s i o n diagram o f t h e f a m i l i a r bend-back loop, i n c o m p e t i t i o n w i t h s p a t i a l d i s p e r s i o n . T y p i c a l l y i n the bend-back regionmû.71+0.72 so t h a t t h e c r i t e r i o n (4.16) reduces t o t h e simple r u l e rl26:65. This, assuming t h a t i t i s q u a l i t a t i v e l y useful even c l o s e t o t h e $20.5, g i v e s a u s e f u l guide as t o whether t h e bend-back l o o p can e x i s t o r n o t . (4.16) i s of course always s a t i s f i e d when c= O and i s never s a t i s f i e d when q = 0.
V - NUMERICAL ANALYSIS
Region II i n t h e v i c i n i t y o f ~ ~ 2 0 . 5 does n o t y i e l d t o a n a l y t i c a l a n a l y s i s so i t has t o be i n v e s t i g a t e d c d m p u t a t i o n a l l y . I n Fig.1,2 and 3 are shown computer-generated graphs o f t h e r e a l p a r t s o f NI, N2 and N3. These correspond t o c o n t i n u a t i o n s i n t o r e g i o n II o f t h e previous a n a l y t i c a l a n a l y s i s . A p a r t i c u l a r f e a t u r e i n F i g . 2 i s t h e ' k i n k ' developed i n NI as rl increases. T h i s shows c l e a r l y the i n t e r a c t i o n between the s p a t i a l d i s p e r s i o n branch, which always e x i s t s , and the c o l l i s i o n - i n d u c e d bend-back curve.
Fig.3 shows what happens when the c o l l i s i o n s p l a y a more dominant r o l e.
The t r a n s l a t i o n of t h e a n a l y t i c a l and computational a n a l y s i s i n t o (R,Kr) diagrams i s shown i n F i g s . 4 and 5 f o r t y p i c a l values. Here on d i s p l a y i s t h e f a c t t h a t , when t h e c r i t e r i o n r i 2 6 5 breaks down, t h e bend-back l o o p i s i s o l a t e d , weakened and e v e n t u a l l y suppressed l e a v i n g o n l y t h e N1 s p a t i a l d i s p e r s i o n branch i n e x i s t e n c e .
V I - CONCLUSION
We have presented a v e r y d e t a i l e d a n a l y s i s o f t h e e f f e c t o f c o l l i s i o n s on t h e s p a t i a l l y d i s p e r s i v e plasmon-polariton mode. Through a
combination o f a n a l y t i ' c a l and computational a n a l y s i s i t i s shown t h a t although the c o m o n l y accepted bend-back can occur i t can a l s o be suppressed by t h e s p a t i a l d i s p e r s i o n . It i s hoped t h a t t h i s paper w i l l form t h e b a s i s f o r a wider d i s c u s s i o n o f t h i s ~ r o b i e m .
VI1 - REFERENCES
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CS-190 JOURNAL DE P H Y S I Q U E
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