HAL Id: jpa-00227635
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Submitted on 1 Jan 1988
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LOW-POWER OPTICAL BISTABILITY AND PHASE CONJUGATION IN POLYDIACETYLENE
W. Blau
To cite this version:
W. Blau. LOW-POWER OPTICAL BISTABILITY AND PHASE CONJUGATION IN POLYDIACETYLENE. Journal de Physique Colloques, 1988, 49 (C2), pp.C2-85-C2-86.
�10.1051/jphyscol:1988218�. �jpa-00227635�
JOURNAL DE
PHYSIQUEColloque
C2,
Suppl6ment a u n 0 6 , T o m e 49, j u i n 1 9 8 8LOW-POWER OPTICAL BISTABILITY AND PHASE CONJUGATION I N POLYDIACETYLENE
W. BLAU
Department o f Pure and A p p l i e d P h y s i c s , T r i n i t y C o l l e g e , D u b l i n
2 ,I r e l a n d
Thelarally induaed optical bietability i s reparted at 514 nm using a Fnbry-&rot cavity filled with polydiacetylene. 8imultancoua degenerate f-uave mixing shavs corresponding bistable behaviour of the phase
conjugate
a m .The
study of t,hixd-order optieal nonlinearitiee in Polydiacetylenes(m)
ham rccvivcd conoidcmblc intcrcet.
This
i a mainly due to the large n o n ~ c e o ~ n t nonlinearitiee caueed by thedelocalised
n-electron eyatanaof
the canjusated polymer baakbone. Such nodinearities shov great premise for ultrahigh sped devioee for optical s i d pmassingand
o o m p u t b .h e n m l l y induced mfraotive I d e x
changes have
recently receivedsacoh
attentioni n
optical bistability. On k r t h i a basis l o w parer bistable e l m - have been dawnatxnted using ZnSe i n t e r f n fil-m.A
d a ydidvantape of using eaaioaduatarn for this purpose is the rccpimaent
to
oparrte o l w o to the &rdeap.A t
this
point PDAabe#raa uaehrl.
They ha^ st- abeorptionlines,
morethan
100rrm
wide. lhrtbenno~n, dcpendins on the end-t a dtbt
pol-r oideohainn PDAe
exist
in either ayellow, red
o rblue
f o m w i t habaowti~
m a x h at 4 7 0r n ,
630 rnaKt
6 X ) rm~ reqcctively.Additionally,
doping w i t h9bC15
or I p am intpddubc furthcc absorptionin the
nsar i n f d meionmhg
out beyond1
m.In
the
p e o m t study, a ealuble R I Aurn used. Either
ayellau solution in
tol- or a s o l i d m d f i b aasisthg of aHIA/P61yvinylahLoAde mixture ue q l o y s d . In
either a-etha
o p t i d absoFption araenmily adjuotahle
by c h m s h g therrlativc
R Mammntratian.
A Rky-Zlaot asvity wsl, rasdt
bt
o o a t b acmi-tnmmpnmt ( h Or f i )Article published online by EDP Sciences and available at http://dx.doi.org/10.1051/jphyscol:1988218
C2-86
JOURNAL DE PHYSIQUE
I n the o c p e x - h m t n M alrcmolod Archer operattng on the X=514 run l i n e wu employsd. Fig. l a ~howa a t y p i e d b l a t o b l e loop o b t a i n e d i n the W t a l u e m e e o l u t i o n . A d t o h - u p frcm a low t x u n a u i t t i a ta a
high
t r a n s m i t t i n # a t a t ecen
be ssvl a t an a c c i d e n t m r of 3.9 mW.The s t a t e of n biztablr: element mu>- he probed s i m u l t a n e o ~ ~ ~ l ~ v i a o p t i c s 1
~>h.asr= C-onjugation by d n g c n e r n t . ~ four-wave mixing. The m d i n g wave i n t.hs Fabry-Perot. c ~ v i t y provides t h e farward and backwards g o i n g pump tmven, khercns t.he probe beam ha8 t o be s e n t i n separately a t a m 1 1 angle. The
-e m n j u g n t e signal r e t r a e e s t h e probe beam and is nnhnnncld due t o t h e i n t e r f e r e n c e e f f e c t s i n s i d e the cavity. I n the experimnnt, p a r t of the l a s e r berm UILS u p l i t o f f by a gloss s d g e ( R S . 0 5 ) and e e n t i n t o t h e ample v i a r e f l e c t i o n o f f a second g l a s s p l a t e ( R S . 5 ) st an angle of 1.2 d e g m a . The phase c o n j u g a t e signal w u l d then be detected behind t h i s glms p l a t e with o t h i r d photcxficdc. Fig. l b d e p i c t s the +s c o n j u g a t e x w f l e c t i v i t y R V e n u s t h e incident. p m r p intensity i n t h e s a m e aample an s h m i n Fin.
la. A c o r r e s ~ n d i n g b i s t s b l e l o o p is observad.
The e x p e r i m e n t a l o b e e r v a t i o n s are i n r e s s o n a b l e agreement with mods1 calculations b e d on thenrmlly induced index change..
0 1 2 3 4 5 8
INPUT POWER ( m W ) INPUT P O W E R (mW1
Fi8. 1. ( a ) Experimental curvcr qhow~ng nulpuc power vcnur tncidtnr laser v w e r