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Submitted on 1 Jan 1977
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16O-12C scattering : description of the gross structure
features using an optical model
A.J. Cole, N. Longequeue, J.F. Cavaignac
To cite this version:
16O-12C
SCATTERING : DESCRIPTION OF
THE
GROSS STRUCTURE
FEATURES USING AN OPTICAL MODEL
A. J.
COLE,
N.LONGEQUEUE
and J. F. CAVAIGNAC Institut des SciencesNucléaires,
B.P.257,
38044 GrenobleCedex,
France(Reçu
le 17 mars1977,
accepté
le 16 mai1977)
Résumé. 2014 La mesure de la diffusion de 16O sur 12C
a été faite dans une
région angulaire
limitée dans les directions avant et arrière à des énergies laboratoires de 16O de 80, 85, 91, 93, 95, 101 et122 MeV. La fonction d’excitation du maximum de la distribution
angulaire
situé près de 156° (c.m.)a aussi été mesurée par pas de ~ 0,5 MeV entre 80 et 101 MeV (lab.). Les résultats ont été ajoutés à d’autres résultats existants et la gross structure de l’évolution de la diffusion avec
l’énergie
a étéanalysée en utilisant un modèle
optique
dont le rayon imaginaire croit avecl’énergie.
Abstract. - Measurements of the
scattering
of 16O on 12C have been made over a limitedangular
range in the forward and backward
hemispheres
atlaboratory
(16O)
energies
of 80,85,91,93,95,101,122 MeV. The excitation function of the maximum near 156° (c.m.) has also been measured in steps
of ~ 0.5 MeV between 80
and
101 MeV (lab.). The data were combined with otherexisting
measure-ments and the gross structure features analyzed
using
anoptical
model whose imaginary radiusincreases with energy.
Classification
z
Physics Abstracts 24.50
1. Introduction. - The
12C_Ilo
system
has,
inrecent years, been the
subject
of intenseexperimental
and theoreticalinvestigations mainly
due to the existence ofanomalously high
backwardangle
cross-sections
exhibiting
strong
oscillationsapproximately
describedby
[PLB(cos
0)]2
whereLg
is theangular
momentum
corresponding
to animpact
parameter
characteristic of the surface of the interaction
[1, 2, 3].
In addition forenergies
EB
Ec.m.
30 MeV(EB
is the Coulomb barrier ~ 12MeV)
the backwardangle
cross-section fluctuatesstrongly
with energygiving
rise to thesupposition
of the existence ofmolecular resonances,
especially
atEr
= 19.7 MeV[2]
andEc...
= 22.5 MeV[1]
where the influence ofresonance like effects in reaction channels have been
established
[3, 1].
At low energyEB
Ec.m.
17 MeVmeasurements of the total reaction cross-section
[4]
were
explained using
anoptical
model whichhowever,
possessed
theunphysical
characteristic ofrelatively
small ( ~0.7)
transmission coefficients for lowpartial
waves.
One may
question
the wisdom oftrying
to fitfluctuations
which,
in this system, have a width of~ 0.5 MeV with a gross structure model
(optical
model).
Neverthelessby using dependent optical
models some success has been obtained infitting
angular
distributions at backwardangles [5],
(1).
Thephysical origin
of thedependence
is howevernot clear and a number of
explanations
related eitherto the non formation of the
compound
nucleus[6]
or to theangular
momentum mismatch in direct reaction channels[7]
have beenproposed.
Yet anotherpossible origin
wasproposed by
the authors ofrefe-rence
[5]
whosupposed
that thedependent imaginary
potential
used in theiranalyses
of’6p_12C
scattering
at 65 and 80 MeV
(160 lab.)
simulates coherent inter-ference between the elasticscattering
and the atransfer reaction.
However,
it remains to be established that such interference canreproduce
therapid
fluctua-tions observed in excitation function measurements
while
preserving
theregular
oscillatory
structuree) Charles, P., Private communication.
1044
observed at backward
angles.
Certainly,
asingle
direct mechanism may be ruled out since such
ampli-’
tudes vary too
slowly
with energy. This fact wasemphasized
by
Devries[8]
who limited hisanalysis
of160_12C
scattering
in terms of the a transfermechanism to the data at 80 MeV where
rapid
fluc-tuations with energy weresupposed
to be lessimpor-tant.
Above 80 MeV
published
dataincluding angular
distribution measurements is limited to forwardangle
distributions measured at 111 MeV[9]
and 168 MeV[10].
It was therefore considered useful toextend the range of the data
by
measuring
smallportions
of the forward and backwardangle
distribu-tions between 80 and 120 MeV(lab. 160) .
The energy resolution available(dE/E N
10-3)
precluded
a searchfor details of fluctuations in the excitation function
although large
effects,
such as those observed at lowerenergies
[2],
ifpresent,
could be observed.Further,
a verification of the presence of a backward
angle
risein the
angular
distributions and a test of thesimple
[PLs(cos
0)]2
behavior observed at lowerenergies
wasconsidered useful.
Using
the160(5+)
beam of the Grenoble ISNcyclotron
we therefore measured smallportions
of the forward and backwardangle
distri-butionsfor 160_12C
scattering
atlaboratory energies
of
80, 85, 91, 93, 95,
101 and 122 MeV. Inaddition,
the excitation function of the maximum situated near1560 c.m. was measured between 80 and 101 MeV. 2.
Experimental procedures.
- Theexperiment
wascarried out at the ISN isochronous
cyclotron
of Grenoble. Theexperimental
arrangement
for the 80 to 101 MeV data is shown infigure
1. A collimatedFIG. 1. -
Experimental arrangement. Dimensions are given in
’
millimetres. z
beam
of 160(5+)
of up to 15 nA(particle)
was directedonto self
supporting 12C
foils of thickness 100 ± 5ug/cm2 .
Two AE - E detector
telescopes
T1
andT2
mountedon a
single
movable arm, andseparated by
20°detected
particles
on the left andright
sides of the beam. Theangular
aperture
of the detectors were 0.5°and 0.7°. The
160
particles
emitted in the forward direction and therecoiling
12C
particles
(correspond-ing
to backwardangle
160
in the c.m.system)
wereidentified on line
by
a PDP9 datahandling
sys-tem
[7].
The
collimating
system DD’ defined the beam direction to within 2° which was notsufficiently
precise
for theperformance
of theexperiment.
Thus before eachangular
distribution run theangle
between the beam direction and the chamber axis was measuredusing
a 100J.lg/cm2
gold
target.
Thisasymmetry
angle
was obtained when the ratio of the elastic counts in the left andright
detectors wasequal
to the ratio of their solidangles.
The constancy of the beam direc-tion was then monitoredcontinuously using
alarge
gold
targetevaporated
ina 12C
backing
in asecondary
chamber,
the ratio between the count rates in twodetectors
(Ml
andM2)
at ± 25° withrespect
to this chamber axisindicating
if anychange
tookplace
in the beam direction. Data wereaccepted
provided
thatthe asymmetry
angle
remained constant to within 0.2°. As a further check theangular
distributions were measured on both sides of the beam and theangular
shift necessary for theirsuperposition
wascompared
to the initial asymmetry measuredusing
thegold
target.
Theagreement
wasalways
better than0.2° which was therefore
assigned
as theangular
errorto each data
point.
Thequality
of the identificationspectrum did not
permit
us to rule out the presence of small contributions of otherisotopes
of,C
and 0. However because ofnegative
reactionQ
values,
contamination of the elasticpeaks
was dueonly
tothe presence of
the 13C
targetimpurity
(1%)
and wastherefore
neglected.
Atypical
energyspectrum
is shown infigure
2. The measured solidangle
ratio between the two detectionsystems
was checkedby
moving
the armcompletely
to the left or to theright
side of the beam and crosscalibrating using
thegold
target.
FIG. 2. -12C energy spectrum 81ab = 10.8°.
The beam energy was measured in a separate
magne-tic
analyzing
system to within 0.5 MeV. For energychanges
of up to 5 MeV aluminium foils mounted on amovable arm were used as
degraders.
Theexperimental
energy resolution varied between 500 keV and 1 MeV
depending
on thedegrader.
With nodegrader
theeffects. The forward
angle
elasticscattering
measure-ment at 122 MeV was
performed
in alarger
chamberinstalled on the same beam line. For this
experiment,
the two detectors were mounted on
separately
movablearms. Otherwise the
experimental
arrangements
wereidentical.
At forward
angles
thehigh
count rate from the16O
elastic could causepile
upproblems
in the12C
channel.
Anti-pile
up devices were therefore includedin the electronic set up and scalers were used to
measure the raw AE count rates and the
pile
up rates.In addition a
generator
simulated12C
peak
was fedthrough
each system and was used to make dead time corrections.Any gain changes
in the electronics could thus also be detected.3. Results and data
analysis.
- In contrast to theresults at lower
energies
our data exhibit anearly
monotonic decrease in the
magnitude
of the backwardangle
cross-section as the energy increases. Fluctua-tions of width less than 500 keV if present, wereobscured
by
theexperimental
energy resolution. Further and rathersurprisingly,
although
the back .angle
differential cross-sections exhibitdeep
oscilla-tions the maxima and minima do not moveprogres-sively
towards 1800 c.m. as would beexpected
froma
[PLg(cos 0)]2
description.
The forwardangle
datapresent
no suchanomaly.
Since norapid
variations with energy wereobserved,
it wasthought
reasonableto
try
and fit thepositions
of the backangle
maxima with apotential
model.Initially,
a shallow1-depen-dent
potential
usedby Badawy et
al.[11]
in anattempt
to fit the 1660 excitation function between 15 and 30 MeV
(c.m.),
was tried but failed to fit theanoma-lous back
angle
behaviour.By
adjusting
the1-depen-dence parameters at each energy
good
fits could be obtainedbut
nosimple
energydependence
of the model wasapparenta
Recently,
von Oertzen[12],
has remarked on thesuccess of
deep
potentials
given
for
example by
the doublefolding
model[13]
inaccounting
for thesystematics a of
heavy
ion transfer reactions., It wastherefore decided to
try
adeep
7potential
of the(conventional)
form :The Coulomb
potential Vc(r, Rc)
was that due to acharged sphere
of radius 2.86 fm. The value of the radius parameter has beenjustified
in reference[14].
Thedepth
of the real part was chosenfollowing
Satchler
[15]
asroughly
half thatgiven
by
the doublefolding
model. The geometry parameters weredeter-mined
by fitting
the variation with energy of thepositions
of the backwardangle
maxima. An excellent fit was obtained with the valuesgiven
in table ITABLE I
Optical
model parameters(*) The potential radii are obtained by multiplying by
A f/3
where A 1 = 12.
FIG. 3 _l6å-l2C scattering. Variations of the positions of the back
angle maxima with energy. The solid lines extending up to N 100 MeV
correspond
to calculations made with the potentialparameters of table I. Above this energy the simple oscillatory
structure of the backward angle distributions is lost and the
evo-lution of a particular maximum is thus impossible to follow.
and is
displayed
infigure
3.Remarkably
thesepara-meters
imply
a mean squareradius of
the realpoten-tial
r2>v
= 14.8fm2
which
is
almostexactly
thatgiven
by
the doublefolding
modelprescription
were (
r2 ) pl
and
r2 ) p2
are the mean square radiiof the densities of the
interacting particles and (
r2 >d,
that
of
aphenomenological
nucleon-nucleon force.Taking
the
meansquare
radii
of the densities fromelectron
scattering
measurements[16]
and that of thetwo
body
force from reference[17]
gives
a value of1046
The
predictions
offigure
3 were shown to be sensi-tive to the values of a andRo
independently.
Thissensitivity
was notpreserved
when fits to thepositions
of the forwardangle
minima were made. Theseposi-tions
which,
as can be seen infigure
4,
were wellfitted
by
theparameter
setgiven
in table I wereshown to be determined
uniquely by
the value ofr2
)v.
The broken lines infigure
4give
some idea ofthe
sensitivity
to this parameter. It was verified thatvariations in the
imaginary potential
parameters
have little effect on these conclusions. At any oneenergy variations in either the
depth
or thegeometry
parameters
were shown to affectchiefly
thedepths
of forwardangle
minima and themagnitude
of the backwardangle
differential cross-section.FIG. 4. - l60_l2C scattering. Variations of the positions of forward
angle minima with energy. The solid lines correspond to calculations made with the potential parameters of table I.
The determination of the
imaginary potential
(tableI)
was carried out as follows. Below 33 MeV c.m. a linear increase of the radiusparameter
was foundby
comparing
the excitation function data ofBadawy
et al.
[11]
with theoptical
modelpredictions.
However,
since this data exhibits
rapid
fluctuations with energy it was deemed necessary to define anexperimental
energy
averaged
cross-section at each energyEo
through
the relationwith AE = 1.0 MeV. The linear
part
of the functionrule)
given
in table I was thus obtainedby demanding
a
good
overall fit to themagnitude
of this energyaveraged
cross-section. As can be seen infigure
5 the energyaveraged
data reveal gross structure resonanceswhich are
reproduced
by
the calculation. This struc-ture was shown to beindependent
of AE forL wncr i
c.m.
FIG. 5. - l60_12C scattering. Energy averaged excitation function
(solid line) for the maximum situated near 160° (c.m.) calculated from the data of Badawy et al. [11] as described in the text. The
optical model prediction (dotted line) was made using the
para-meters given in table I. Since the experimental data exist only on the
range 15 to 34 MeV c.m., the averaged cross-section is incorrect in N 2 MeV wide regions at the beginning and end of this range.
FIG. 6. - l60.12C scattering. Variation of total reaction cross-section with energy [4] (full line) compared with the optical model
prediction made using the parameters of table I.
As a further check we
compared
theprediction
madeusing
these parameters with the total reactioncross-section data of Kuenher and
Almquist
[4].
Figure
6 shows that excellent agreement was obtained.Above 30 MeV c.m. it was found necessary to add
a non linear term to the function
rule)
in order toreproduce
the absolute value of the backangle
diffe-rential cross-section at 52.3 MeV c.m.(Fig.
11).
When this was done a
good
fit to our excitationfunc-tion measured between 34 and 41 MeV c.m. was
obtained
(Fig.
7). Further,
the maximum value ofrI(E)
(2.15 fm at 70 MeVc.m.)
gives
an excellent fitto the forward
angle scattering
data of Hiebert andGarvey
[10]
(Fig.
8).
At lowenergies
the influence of the non linear term isnegligible.
Since a smooth monotonic increase of the
imaginary
potential
radiusparameter
gives
agood description
of all data considered it would be
tempting
to try tointerpret
thiscomportment
in terms of somephysical
model. However a number of
problems preclude
suchspeculation.
The mostimportant
is the existence ofFIG. 7. - l60_12C scattering. Prediction of excitation function for the maximum situated near 1560 c.m. The data points are those
measured in the present work.
FIG. 8. - l60_l2C
scattering. 168 MeV (lab.) data of ref. [10]. The prediction (full line) was made with the maximum value of
r1(E) as explained in the text. Other predictions (dotted lines) are
shown to give an idea of the sensitivity to rl(E). Other parameters
are as given in table I.
parameter
with energy may bereplaced by
anexpo-nential increase in the
potential depth.
Also a firstorder
Taylor expansion
indicates that the addition of a derivative Saxon Woods term, whosedepth
increases
linearly
with energy, to an energyindepen-dent volume Saxon Woods form is
equivalent,
overshort energy ranges, to a
single
volume term with alinearly increasing
radiusparameter.
Calculations made with these forms over small energy rangesverified these
equivalences
and thus underlined thephenomenological ambiguity.
Even if no suchambi-guity
existed adifficulty
would arise since one expectsthe
optical
model to underestimate the average ofa
rapidly fluctuating
cross-sectionby
the averageof the cross-section due to the
fluctuating
part
of thescattering
wave function. Since theorigin
of theobserved fluctuations
is,
atpresent,
unknown it isimpossible
to decide how much of the energyaveraged
cross-section should be allocated topotential
scatter-ing.
Finally
we remark on the fact that our parameterssuffer from the same drawback as those of Kuenher
and
Almquist
[4]
in as much as at lowenergies
they
imply
non zero valuesof
1 1], for
lowpartial
waves.In order to
investigate
thispoint
astrongly absorbing
core was added to our
optical
potential
theparameters
of which are
given
infigure
9. The small diffuseness was chosen to minimise the effect of the core in thesurface
region
whileavoiding
the introduction ofsharp
discontinuities in thepotential.
As can be seenin
figure
9(inset),
increasing
thedepth
of this termFIG. 9. -16O-12C scattering. Sensitivity of the calculated 17.2 MeV
(c.m.) angular distribution to the addition of a strongly absorbing core to the imaginary potential of table I
with RCORE = 0.5.4 1/3 fm. (A, = 12),
ACORE = 0.3 fm. The effect
of the core on the transmission coefficients T, is shown as an inset.
has a
large
effect on the transmission coefficients forlow
partial
waves whileproducing
nosignificant
change
in thepartial
waves scattered from thepoten-tial surface.
Further,
it is clear from thefigure,
that thelarge changes
in the transmission coefficients for lowpartial
waves do notstrongly
affect the backangle
differential cross-sections. We thus conclude that the nonphysical
character ofthe 111, values
for low
partial
waves is associated with the use ofthe
Saxon Woods
imaginary potential
form factor and that this form isprobably
notappropriate
for use inanalysis
oflight heavy
ionscattering.
Predictions for the back
angle
differentialcross-sections are shown with the data in
figure
10and,
for the more
complete
data at 122 MeV infigure
11. No detailedfitting
wasattempted
because of thelimited
angular
range of the data.4. Discussion. -
Contrary
to the statement made in the introduction of reference[5]
it ispossible
to fit both forward and backwardangle 16O-12C
scattering
1048
FIG. 10 - 16O-12C scattering. Back angle data between 80 and
100 MeV (lab.) together with optical model predictions made using the parameters given in table I.
FIG. 11. - l60_12C scattering. Data at 122 MeV with the optical model prediction made using the parameters given in table I.
or not the
deep
potential
found in the presentanalysis
hasphysical significance.
The lack ofsensitivity
of thepredictions
to the presence of astrongly absorbing
core
(Fig.
9)
indicates that the interior part of thepotential
at radii 1.5 fm is not well determinedby
the data considered. However at distances greater than this value adeep potential
would seem to be indicated.Further,
ouranalysis
shows that thegeometry parameters of such a
potential
are welldetermined
provided
that data at forward and back-wardangles
over alarge
energy range are considered. Theoretical calculations[18, 19]
of the ion-ionpotential
usually predict
a shallowpotential
such asthat used in the
analysis
of the12C_12C
databy
the Yale group[20]. However,
a recent calculation of the16O-16O
potential
[21]
using
agenerator
coordinatemethod
produced
apotential
rather like that used inthe
present
analysis.
Detailedcomparison
is difficultsince the calculation of the interior and exterior
parts
of thepotential
were made in different limits of theapproximations employed.
We note however that the authorspredict
apotential
of - 430 MeV centraldepth
falling
to half of this value for radii between 2 and 4 fm.They
also conclude that the surface of thepotential
is wellapproximated by
the doublefolding
model.From a
phenomenological point
of view our resultsagree with the
findings
of Kozab et al.[22] who,
inanalyzing
the variation ofcomplete
fusioncross-sections with energy for
2’Al
+160,
2’Al
+2°Ne
and
2’Al
+325,
were led to the conclusion that the realpart
of theoptical potential
wasstrongly
attrac-tive at radii
considerably
smaller than the sum of theradii of the
interacting particles. Analysis
of syste-matics of transfer reactionsby
von Oertzen[13]
also indicated thenecessity
of adeep
realpotential.
On the other hand there exist many
phenomenolo-gical analyses
of ion-ionscattering
using
shallow realpotentials
[24].
It is ouropinion
that suchanalyses
arestrongly
influencedby
the choice of radiuspara-meter which is almost
always
taken to be the sum ofthe radii of the
interacting
nuclei. Apriori
of coursethere is no reason for this choice
which,
at least forlight
targets,
disagrees
with thesupposition
that thepotential
surface is wellrepresented by
the doublefolding
model. Forexample
in the16O-12C
casethe sum of the radii is
Even for zero diffuseness we obtain
which may be
compared
with the value of 14.8fm2
given by
the doublefolding
model (section3).
A somewhat
surprising
result of ouranalysis
is the smallness of theimaginary potential.
Its mainjustifi-cation comes from the
agreement
between thecal-culated and
experimental
reaction cross-sections aswell as the overall agreement with the
magnitudes
ofthe backward
angle
differential cross-sections. Because of theambiguities
detailed in theprevious
section wemay conclude
only
that theimaginary potential
increases with energy. This conclusion may of coursebe understood
partly
in terms of theincreasing density
of states in the 28Sicompound
nucleus andpartly
in terms of theavailability
of anincreasing
numberof
direct
and semi-direct reaction channels withincreasing
energy.Finally,
we should remark onpossible
contribu-tions from the cx transfer mechanism. Our
analysis
hasshown that all the gross structure features of the data
are well described
by
asingle
direct process (elasticscattering).
The a transferreaction,
which may be anpart of the
cross-section,
would beexpected
to be characterizedby
a[PLs(cos 0)]’
behaviour whichdisagrees
with observation above 34 MeV(c.m.).
Below this energy it is not clear whether theinterfe-rence of these mechanisms is
capable
ofproducing
the observed fluctuations but thispossibility
shouldnot be ruled out. Detailed
calculations,
clearly
necessary to test thispoint,
are in progress.Acknowledgments.
- Theexperiments
described in this paper were carried out in collaboration with members of a group ofphysicists
of C.E.N.Saclay.
We wish to thank them for their assistance. Our thanks areespecially
due to Dr’s P. Charles and B. Fernandez for many fruitful discussions and toProfessor J. P.
Longequeue (ISN)
forexperimental
assistance and for carefulreading
of themanuscript.
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