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Exposure to high concentration of formaldehyde: a case study

Marchant, R.; Yoshida, K.; Figley, D. A.

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Exposure to High Concentration

of Formaldehyde.

A

Case Study

by R. Marchant, K. Yoshida and D.A. Figley

ANALYZED

Reprinted from

Transactions, Indoor Air Quality in Cold Climates:

Hazards and Abatement Measures

APCA Specialty Conference

Ottawa, Ontario, April 1985

p. 148-154

(IRC Paper No. 1384)

Price $3.00

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ABSTRACT

A series of health problems suffered by an elderly couple soon

after they occupied a new

2 4 0 3 3

mobile home and initial

measurement of an indoor formaldehyde concentration of

0.7

ppm

prompted an investigation of the formaldehyde sources.

Peu de temps apres avoir emmgnagg dans une maison mobile neuve

de

240

m3, un couple

3g6 a CprouvC toute une sCrie de problGmes

de sant6; apres avoir relev6 dans l'habitation une

concentration de formaldChyde de

0,7

ppm, on a proc6d6

3

une

6tude visant

3 dgterminer la provenance de cette substance.

(4)

EXPOSURE

TO

HIGH CONCENTRATION OF FORMALDEHYDE.

A CASE STUDY

R. Marchant,

Occupational and Environmental Health Physician, Saskatoon

K. Yoshida, Department of Social and Preventive Medicine, University of

Saskatchewan, Saskatoon,

and D.A. Figley, Division of Building Research, National Research Council of

Canada, Saskatoon

Indoor air quality has become a serious concern for home dwellers since the

introduction of energy-efficient building technology. Combined with

increased use of synthetic building materials, low ventilation rates can

result in build-up of formaldehyde gases.

A series of health problems suffered by an elderly couple soon after they

moved into a new 240-m3 mobile home and initial measurement of an indoor

formaldehyde concentration of 0.7 ppm prompted an investigation to determine

the source of contamination. The formaldehyde concentrations were

persistent, day and night, and remained in the same order of magnitude in

all rooms, indicating a widespread source of emission.

The occupants' medical history and physical examination indicated no

problems that could account for the current symptoms except formaldehyde

exposure. Protection was by evacuation of the premises rather than

substitution of the hazardous (building) materials or improvement of the

ventilation system. Symptoms characteristic of formaldehyde sensitivity

subsided when the subjects moved to an ordinary home.

Reprinted with permission from the transactions Indoor Air Quality

in

Cold

Climates: Hazards and Abatement Measures, published in 1986 by the Air

- - -

(5)

EXPOSURE TO HIGH CONCENTRATION OF FORMALDEHYDE.

A CASE STUDY

1.0 INTRODUCTION

Indoor a i r q u a l i t y i s of i n c r e a s i n g c o n c e r n a s t h e number of

e n e r g y - e f f i c i e n t a i r - t i g h t b u i l d i n g s grows. S t u d i e s show t h a t t h e a i r

q u a l i t y of mobile homes i s of even g r e a t e r concern t h a n t h a t of c o n v e n t i o n a l

_

r e s i d e n t i a l b u i l d i n g s because of some of t h e b u i l d i n g m a t e r i a l s used. Many

may g i v e o f f formaldehyde g a s ( 1 ) . This s t u d y d e a l s w i t h a m u l t i -

d i s c i p l i n a r y approach t o t h e problems a s s o c i a t e d w i t h formaldehyde

o f f - g a s s i n g i n a mobile home, i n c l u d i n g i n d u s t r i a l h y g i e n e , e m i s s i o n s o u r c e i d e n t i f i c a t i o n , and h e a l t h assessment.

I n d u s t r i a l h y g i e n e s t u d i e s d e m o n s t r a t e t h a t t h e measured formaldehyde

c o n c e n t r a t i o n s i n mobile homes v a r y e x t e n s i v e l y : from 0.1 t o 0.5 ppm (mean

0.36 ppm) f o r two mobile homes i n P i t t s b u r g h , PA, up t o 1.77 ppm (mean of 0.44 ppm) f o r 200 mobile homes r e g i s t e r i n g c o m p l a i n t s i n Washington S t a t e , t o 3.0 ppm (mean 0.4 ppm) f o r 431 mobile homes r e g i s t e r i n g c o m p l a i n t s i n Minnesota, and from 0.023 t o 4.2 ppm (mean of 0.88 ppm) f o r mobile homes

r e g i s t e r i n g c o m p l a i n t s i n Wisconsin ( 2 ) .

The c o n c e n t r a t i o n of formaldehyde i n s i d e homes f l u c t u a t e s d i u r n a l l y and

s e a s o n a l l y a s w e l l a s w i t h t e m p e r a t u r e and humidity. Assessments of

e m i s s i o n s o u r c e s f o r t h e o f f - g a s s i n g of formaldehyde have shown t h a t p r e s s e d

wood p r o d u c t s c a n be a major s o u r c e ( 3 ) . Modern mobile home c o n s t r u c t i o n

p r a c t i c e s have t e n d e d t o make u s e of m a t e r i a l s ( 4 ) t h a t may be bonded w i t h urea-formaldehyde r e s i n .

H e a l t h e f f e c t s t h a t have been documented seem t o c o r r e l a t e w i t h t h e

e n v i r o n m e n t a l measurements. Symptoms may i n c l u d e i r r i t a t i o n of t h e e y e s and

t h r o a t , d i s t u r b e d s l e e p , u n u s u a l t h i r s t on awakening ( 5 ) , coughing and wheezing, d i s o r i e n t a t i o n , d i a r r h o e a , nausea and vomiting ( 6 ) , d i z z i n e s s and

l e t h a r g y , headache, l o s s of a p p e t i t e , b u r n i n g s e n s a t i o n of t h e s k i n

(7),

asthma and s e n s i t i z a t i o n ( 6 ) . Few of t h e s e symptoms have accompanying

p h y s i c a l s i g n s , b u t many have been documented i n o c c u p a n t s of mobile homes ( 8 , 9 ) .

2.0 INVESTIGATION

2.1 General

The mobile home under i n v e s t i g a t i o n (CSA approved and b u i l t i n Canada i n 1983) was occupied from March t o May 1984 by a n e l d e r l y c o u p l e , t h e o n l y

o c c u p a n t s s i n c e i t s manufacture. It was l o c a t e d i n a mobile home p a r k i n a

suburban d i s t r i c t of Saskatoon, Saskatchewan. The home was 4 m wide m d

24 rn l o n g (240 m3 of volume) w i t h a l i v i n g room, a t t a c h e d k i t c h e n , bathroom,

and t h r e e bedrooms.

A l l of t h e i n t e r i o r w a l l s were covered w i t h p a r t i c l e board p a n e l l i n g

w i t h a l a m i n a t e d wood g r a i n o r " l i n e n look" f i n i s h ; t h e back was u n f i n i s h e d .

The c e i l i n g was covered w i t h g l o s s y p l a s t i c t i l e s . P a r t i c l e board was u s e d

f o r cupboards, s h e l v i n g and c o u n t e r t o p s , t h e u n d e r s i d e s u n f i n i s h e d . The

s u b f l o o r was made of 19-mm p a r t i c l e board and w a s covered by u n d e r l a y and

w a l l - t o - w a l l c a r p e t i n g of medium s h a g i n t h e l i v i n g room, s h o r t s h a g i n t h e

bedrooms, and l i n o l e u m i n t h e k i t c h e n and bathroom. The e x t e r i o r , f l o o r ,

and c e i l i n g - - r e i n s u l a t e d w i t h g l a s s f i b r e i n s u l a t i o n . The c r a w l s p a c e

(6)

N a t u r a l ( w i t h o u t f o r c e d a i r f l o w ) v e n t i l a t i o n w a s p r o v i d e d by lOO-mm

d i a m e t e r d u c t i n t a k e s i n t h e n o r t h e a s t c o r n e r o f t h e l i v i n g room and i n t h e southwest c o r n e r of t h e m a s t e r bedroom c l o s e t 1.8 m above t h e f l o o r . A r a n g e hood i n t h e k i t c h e n p r o v i d e d f o r c e d a i r f l o w . The bathroom was n o t equipped w i t h a n e x h a u s t fan. The n a t u r a l gas f o r c e d - a i r f u r n a c e was p r o v i d e d w i t h a 1251nm d i a m e t e r f r e s h a i r i n t a k e .

2.2 H e a l t h E f f e c t s

The owners became ill upon moving i n t o t h e i r new mobile home, a l t h o u g h t h e y had been w e l l u n t i l t h e n e x c e p t f o r c h r o n i c i l l n e s s e s ( d e c r e a s e d

h e a r i n g , Rheumatoid a r t h r i t i s , a n g i n a , a t r i a l f i b r i l l a t i o n , o b e s i t y , h y p e r t e n s i o n and d i v e r t i c u l i t i s ) . The w i f e was i n t h e home a l l t h e time.

Her

e a r l y symptoms ( f i r s t n i g h t ) were n a u s e a , v o m i t i n g , and d i z z i n e s s . A s time went on t h e symptoms i n c r e a s e d t o i n c l u d e headache, nausea, vomiting, s l e e p d i s t u r b a n c e , d i z z i n e s s , s h o r t n e s s of b r e a t h , b u r n i n g e y e s , runny n o s e , and c h r o n i c f a t i q u e . Headaches were r e l i e v e d by 292's and i c e packs;

d i z z i n e s s was r e s o l v e d by b r e a t h i n g f r e s h a i r .

The husband developed r u n n i n g e y e s and nose. On waking h e e x p e r i e n c e d headache, b l u r r e d v i s i o n , d i z z i n e s s , and f a t i g u e . H i s s l e e p w a s f r e q u e n t l y i n t e r r u p t e d . He s p e n t h i s days d r i v i n g a t a x i c a b and b e f o r e g o i n g t o work h e would have t o walk o u t s i d e f o r h a l f a n hour t o " c l e a r h i s head."

Both were non-smokers and n o n d r i n k e r s ; t h e y had n o t e x p e r i e n c e d any i n f e c t i o n s o r e x a c e r a b a t i o n s of c h r o n i c i l l n e s s t h a t c o u l d account f o r t h e i r c u r r e n t problems. The p h y s i c a l e x a m i n a t i o n w a s normal e x c e p t f o r t h o s e s i g n s r e l a t e d t o c h r o n i c a i l m e n t s .

2.3 Formaldehyde Sampling Procedure

Air sampling ( s t a t i o n a r y a r e a , NIOSH s t a n d a r d No. P & CAM 125 proposed by P h y s i c a l and Chemical A n a l y s i s Branch of t h e N a t i o n a l I n s t i t u t e f o r

O c c u p a t i o n a l H e a l t h and S a f e t y ) c o n s i s t e d of a t r a i n of two midget impingers f i l l e d w i t h 20 mL of a b s o r b i n g s o l u t i o n ( d i s t i l l e d d e i o n i z e d w a t e r ) and a s p i r a t e d a t 1 L/min f o r 60 min (10). The c o l l e c t i o n e f f i c i e n c y of t h i s method i s e x p e c t e d t o be 95%. The sampler i n l e t was k e p t 0.3 m above t h e f l o o r s o as t o c o l l e c t a r e p r e s e n t a t i v e zone of ambient a i r c o n t a i n i n g formaldehyde.

The a n a l y t i c a l method ( 1 0 ) used t h e c h r o m o t r o p i c a c i d - s u l f u r i c a c i d method. Formaldehyde c o l l e c t e d i n t h e a b s o r b i n g s o l u t i o n r e a c t s w i t h t h e chromotropic a c i d - s u l f u r i c a c i d t o form a p u r p l e mono-cationic chromogen. Absorbtance of t h e c o l o u r e d s o l u t i o n is r e a d i n a s p e c t r o p h o t o m e t e r a t 580-~lm wavelength. The measuring r a n g e of t h i s method i s 0.1 t o 2.0 ppm, w i t h a p r e c i s i o n of 25%.

2.4 Formaldehyde Emission Sources

High, uniform HCOH c o n c e n t r a t i o n s i n d i c a t e d a n e v e n l y d i s t r i b u t e d s o u r c e r a t h e r t h a n a p o i n t s o u r c e . P r e l i m i n a r y o b s e r v a t i o n s of f u r n i s h i n g s and o c c u p a n t - r e l a t e d a c t i v i t i e s d i d n o t i n d i c a t e p o t e n t i a l formaldehyde s o u r c e s , and an i n v e s t i g a t i o n of t h e t r a i l e r c o n s t r u c t i o n m a t e r i a l s w a s

i n i t i a t e d . S i n c e i n t e r i o r - g r a d e p a r t i c l e b o a r d s ( u s u a l l y bonded w i t h

urea-formaldehyde r e s i n ) have been shown t o be p o t e n t i a l l y h i g h formaldehyde s o u r c e s ( l l ) , t e s t s were conducted t o d e t e r m i n e t h e r e l a t i v e e m i s s i v e

s t r e n g t h s of t h e b u i l d i n g m a t e r i a l s used i n t h e home. Measurement of formaldehyde o f f - g a s s i n g from b u i l d i n g m a t e r i a l s i n v o l v e s p l a c i n g material

samples i n an e n v i r o n m e n t a l chamber w i t h c o n t r o l l e d c o n d i t i o n s of

(7)

method cannot be used f o r i n - s i t u t e s t i n g of m a t e r i a l s . Matthews

( 3 )

h a s proposed a p o r t a b l e s u r f a c e e m i s s i o n m o n i t o r f o r measuring formaldehyde

r e l e a s e from b u i l d i n g m a t e r i a l s , b u t t h i s s y s t e m i s n o t commercially

a v a i l a b l e .

T e s t i n g f o r t h e r e l a t i v e HCOH e m i s s i o n s t r e n t h s of t h e v a r i o u s p a r t i c l e

board s u r f a c e s i n t h e t r a i l e r i n v o l v e d c o v e r i n g a s u r f a c e w i t h a 2 L

r e c t a n g u l a r p o l y e t h y l e n e box and a l l o w i n g 24 h t o e l a p s e u n t i l t h e HCOH

r e a c h e d a n e q u i l i b r i u m c o n c e n t r a t i o n . The c o n c e n t r a t i o n was t h e n measured.

Although t h i s i s n o t a s t a n d a r d i z e d t e s t , i t i s u s e f u l f o r r a n k i n g t h e

r e l a t i v e s t r e n g t h s of s u r f a c e e m i s s i o n s o u r c e s ; c o n c e n t r a t i o n v a l u e s t h u s

o b t a i n e d a r e n o t d i r e c t l y r e l a t e d t o i n d o o r a i r p o l l u t a n t l e v e l s . This t e s t

was c a r r i e d o u t on c a r p e t s , t h e f r o n t and back of w a l l p a n e l l i n g , and

k i t c h e n c a b i n e t s . Measurements of t h e HCOH c o n c e n t r a t i o n were a l s o t a k e n i n

w a l l c a v i t i e s , c l o s e t s , and k i t c h e n cupboards. The r e s u l t s a r e g i v e n i n

Table 1.

2.5 Formaldehyde L e v e l s

The t e s t v a l u e s ( e m i s s i o n s o u r c e s ) l i s t e d i n Table 1 were u s e d a s

i n d i c a t i o n of p o t e n t i a l s o u r c e s of HCOH. The l a r g e s u r f a c e a r e a and h i g h

e q u i l i b r i u m c o n c e n t r a t i o n of p a r t i c l e board w a l l p a n e l l i n g s u g g e s t t h a t i t i s t h e major HCOH s o u r c e i n t h e mobile home. By c o n t r a s t , t h e p a r t i c l e board s u b f l o o r / c a r p e t s y s t e m had e q u i l i b r i u m v a l u e s lower t h a n t h e i n d o o r

a i r l e v e l s . The HCOH l e v e l s i n t h e k i t c h e n cupboards and c l o s e t s were n o t

s i g n i f i c a n t l y above t h e i n d o o r l e v e l s , and were c o n s i d e r e d t o b e secondary

s o u r c e s . The h i g h e r HCOH c o n c e n t r a t i o n i n t h e cupboard o v e r t h e

r e f r i g e r a t o r r e s u l t e d from e l e v a t e d t e m p e r a t u r e caused by h e a t l i b e r a t e d from t h e condenser c o i l s of t h e r e f r i g e r a t o r .

I n i t i a l p o i n t sampling by t h e p u b l i c h e a l t h i n s p e c t o r s (Saskatoon

Community H e a l t h U n i t ) i n d i c a t e d a formaldehyde l e v e l of 0.8 ppm. I n t h e

i n d u s t r i a l hygiene s u r v e y , t h e c o n c e n t r a t i o n was d e t e r m i n e d i n two iropingers

s e p a r a t e l y t o o b t a i n t h e s l i p p a g e . The mass of formaldehyde c o l l e c t e d i n

t h e two impingers w a s c o r r e c t e d by t h e sampling e f f i c i e n c y of 0.95 t o o b t a i n

a t r u e mean c o n c e n t r a t i o n of formaldehyde d u r i n g t h e sampling p e r i o d ( 1 h

e a c h i n l a t e a f t e r n o o n b e f o r e cooking and i n t h e e v e n i n g ) . The s l i p p a g e

v a l u e s of t h e impingers were: 13.5% f o r t h e l i v i n g room sample, and 18.6%

f o r t h e bedroom sample.

The daytime c o n c e n t r a t i o n of formaldehyde i n t h e l i v i n g room was

0.67 ppm; t h e n i g h t time v a l u e i n t h e bedroom was 0.68 ppm. Both v a l u e s f a r

exceed t h e f e d e r a l r e g u l a t o r y l i m i t of 0.1 ppm. A p r e v i o u s s t u d y (12)

showed t h a t among 16 c a s e s w i t h

UFFI

i n s u l a t i o n and h e a l t h c o m p l a i n t s o n l y

one c a s e r e a c h e d a maximum of 0.85 ppm, o r a mean of 0.455 ppm. The v a l u e s

o b t a i n e d i n s i d e t h e mobile home, t h e r e f o r e , a r e comparable t o t h o s e f o r

homes w i t h UFFI i n s u l a t i o n . The formaldehyde c o n c e n t r a t i o n w a s a s h i g h

d u r i n g t h e day a s a t n i g h t , and w a s uniform t h r o u g h o u t t h e rooms t e s t e d .

A second daytime measurement was performed w i t h t h e house

p r e - c o n d i t i o n e d by o p e r a t i n g t h e f u r n a c e f a n c o n t i n u o u s l y f o r t h e p r e v i o u s

24 h. The l i v i n g room HCOH c o n c e n t r a t i o n was 0.41 pprn a t a v e n t i l a t i o n r a t e

of 0.35 a i r changes p e r hour (ACH). The v e n t i l a t i o n r a t e was determined by

N20 t r a c e r g a s decay t e s t .

During t h e h e a l t h a s s e s s m e n t , t h e c o u p l e b o t h d i s p l a y e d symptoms

s i m i l a r t o t h o s e of o t h e r formaldehyde-exposed i n d i v i d u a l s . There was no

o t h e r e v i d e n c e , from h i s t o r y and p h y s i c a l e x a m i n a t i o n , t o e x p l a i n t h e i r symptom complexes f o r any a i l m e n t o t h e r t h a n t h e determined e n v i r o n m e n t a l exposure.

(8)

3.0 DISCUSSION

The o c c u p a n t s ' e x p o s u r e t o a i r b o r n e formaldehyde c a n be c o n t r o l l e d , i n p r i n c i p l e , by s u b s t i t u t i o n of m a t e r i a l s , i s o l a t i o n , and v e n t i l a t i o n . A s t h e b u i l d i n g m a t e r i a l s were i d e n t i f i e d as t h e major s o u r c e of formaldehyde

e m i s s i o n , t h e y might be removed and m a t e r i a l s s u b s t i t u t e d t h a t e m i t

s i g n i f i c a n t l y l e s s o r no formaldehyde. The major HCOH s o u r c e i s t h e w a l l p a n e l l i n g , however, and s u b s t i t u t i o n would i n v o l v e r e b u i l d i n g t h e e n t i r e i n t e r i o r of t h e t r a i l e r .

The second o p t i o n i s i m p r a c t i c a l a l s o . The o c c u p a n t s might b e

p r o t e c t e d from i n h a l i n g t h e formaldehyde by s e a l i n g t h e e m i s s i o n s o u r c e s , b u t a t t h e p r e s e n t t i m e t h e r e i s no r e l i a b l e t e c h n i q u e f o r d o i n g t h i s .

The t h i r d o p t i o n i s t o i n c r e a s e t h e v e n t i l a t i o n r a t e t o r e d u c e t h e a i r b o r n e c o n c e n t r a t i o n of formaldehyde. For a c o n s t a n t p o l l u t a n t s u p p l y r a t e t o a s p a c e (assuming t h e removal r a t e i s due t o d i l u t i o n a l o n e and t h e r e i s no t r a n s i e n t s t o r a g e l r e l e a s e e f f e c t ) , t h e i n d o o r c o n c e n t r a t i o n c a n be modelled (13) by: where C = i n d o o r a i r HCOH c o n c e n t r a t i o n = o u t d o o r a i r HCOH c o n c e n t r a t i o n (assumed t o be n e g l i g i b l e ) N = p o l l u t a n t s u p p l y r a t e i n the, s p a c e

v

= v e n t i l a t i o n r a t e . I f t h i s model i s a p p l i e d t o t h e i n i t i a l c o n d i t i o n s of 0.41 ppm a t 0.35 a c h , t h e n a v e n t i l a t i o n r a t e of -1.5 a c h (360 m3/h) would be r e q u i r e d t o r e d u c e t h e HCOH c o n c e n t r a t i o n t o 0.1 ppm (14). This s o l u t i o n would impose a l a r g e h e a t i n g / c o o l i n g energy p e n a l t y on t h e o c c u p a n t s and would r e q u i r e s u b s t a n t i a l m o d i f i c a t i o n s t o t h e h e a t i n g and v e n t i l a t i n g system.

L i t e r a t u r e a d d r e s s i n g t h e problem ( 1 5 ) s u g g e s t s t h a t formaldehyde

r e l e a s e from b u i l d i n g m a t e r i a l s h a s a h a l f l i f e of between 30 and 60 months; f o r a c o n s t a n t v e n t i l a t i o n r a t e , i t would t h e r e f o r e t a k e a minimum of

30 months f o r t h e i n d o o r HCOH l e v e l t o d r o p t o one h a l f t h e p r e s e n t l e v e l . I n c r e a s i n g t h e t e m p e r a t u r e a n d / o r h u m i d i t y c o u l d r e d u c e t h e h a l f l i f e , b u t t i m e s i n t h e o r d e r of y e a r s could s t i l l be r e q u i r e d t o d e p l e t e t h e HCOH s o u r c e s . I n t h i s s i t u a t i o n , simply w a i t i n g f o r t h e problem t o d i s a p p e a r does n o t seem t o be a d v i s a b l e .

4.0 CONCLUSION

1. The formaldehyde l e v e l s i n t h e mobile home were c o n s i s t e n t l y h i g h (>0.6 ppm) and u n i f o r m l y d i s t r i b u t e d .

2. The major i d e n t i f i e d e m i s s i o n s o u r c e was t h e p a r t i c l e board p a n e l l i n g u s e d t h r o u g h o u t t h e t r a i l e r .

3. The o c c u p a n t s e x p e r i e n c e d symptoms t h a t c o u l d be a t t r i b u t e d t o formaldehyde exposure.

4. C o n v e n t i o n a l methods of c o n t r o l l i n g t h e p o l l u t a n t i n t h e t r a i l e r would i n v o l v e e x t e n s i v e m o d i f i c a t i o n s and a r e t h e r e f o r e u n s a t i s f a c t o r y .

The s u b j e c t s have s i n c e moved i n t o a n o r d i n a r y home w i t h low i n d o o r formaldehyde l e v e l s and t h e 'symptoms c h a r a c t e r i s t i c of formaldehyde s e n s i t i v i t y h a v e s u b s i d e d .

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REFERENCES

1. S u n t a , B.E., P o p u l a t i o n Exposure t o Atmospheric Formaldehyde I n s i d e

L

Residences. SRI I n t e r n a t i o n a l , Menlo Park, CA, January, 1980.

2. Gupta, K.C. e t a l , Formaldehyde i n Indoor Air: s o u r c e s and T o x i c i t y .

Env. I n t . 8:349, 1982.

3. Matthews, Thomas G., Hawthorne, A.R., Daffron, C.R., Reed, T.J. and

Corey, M.D., Formaldehyde R e l e a s e from Pressed-Wood P r o d u c t s .

Proceedings: 1 7 t h I n t e r n a t i o n a l Washington S t a t e U n i v e r s i t y

P a r t i c l e b o a r d / C o m p o s i t e M a t e r i a l s Symposium, 1983-

4. The Canadian Formaldehyde Report. The Canadian Chemical P r o d u c e r s

A s s o c i a t i o n , October 1983.

5. Morrill, E.E., Air Cond. Heat. Vent., 53:94, 1961.

6. Hileman, B., Formaldehyde, Environ. S c i . Technol.

,

16(10) : 5 4 3 ~ , 1982.

7. Hoey, J . R . , T u r c o t t e , F., Couet, E., L'Abbe, L A . , H e a l t h R i s k s i n

Homes I n s u l a t e d w i t h Urea-Formaldehyde Foam. Can. Med. ASSOCO J m ,

130: 115, 1984.

8. Garry, V.,E., Oatman, L., P l e u s s , R. and Gray, D., ~ o r m a l d e h y d e i n t h e

Home. Some Environmental D i s e a s e P e r s p e c t i v e s . Minn. Med. 63: 107,

1980.

9. Breysse, P., Formaldehyde Exposure i n Mobile Homes. Environ. H e a l t h

S a f e t y News, U n i v e r s i t y of Washington, Pullman, p. 26, 1978.

10. NIOSH: NIOSH Manual of A n a l y t i c a l Methods. 2nd Ed. 1974, Formaldehyde

i n Air P & CAM 125.

11. Meyer

,

B.

,

Formaldehyde Release From B u i l d i n g Products. INDOOR AIR 84,

Stockholm, 1984.

12. Wooley, H., Urea-Formaldehyde I n s u l a t i o n i n Saskatchewan Residences.

Occup. H. & S. B r . Report No. 81-01-01, 1981.

13. J a n s s e n , J.E., V e n t i l a t i o n f o r C o n t r o l of Formaldehyde i n Mobile Homes.

ASHRAE T r a n s a c t i o n s , Vol. 89, Pt.lB, 1983.

14. V e n t i l a t i o n f o r Acceptable Indoor Air Q u a l i t y . The American S o c i e t y of

H e a t i n g , R e f r i g e r a t i n g , and Air C o n d i t i o n i n g E n g i n e e r s , ASHRAE 62-1981,

A t l a n t a , 1981.

I 15. Indoor P o l l u t a n t s . Committee on Indoor P o l l u t a n t s , N a t i o n a l Research

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TABLE 1. M a t e r i a l ~ e s t R e s u l t s

( I n s i d e a i r temperature 23OC, r e l a t i v e humidity 35%)

HCOH Conc

b c a t i o n ( P W )

Box A , t o p of l i v i n g room c a r p e t 0.45

Box B,

U/S

of k i t c h e n cupboard s h e l f ( u n f i n i s h e d ) 0.75

Box C , back of w a l l p a n e l above f u r n a c e 0.85

Box D, i n s i d e s u r f a c e of w a l l panel w i t h 300 mm x 5 mm c r a c k 2.0 Box E, i n s i d e s u r f a c e of w a l l p a n e l 1.7 Box F, t o p of bedroom c a r p e t 0.35 I n s i d e of k i t c h e n cupboards over r e f r i g e r a t o r 1.15 I n s i d e of water h e a t e r c l o s e t 0.65 I n s i d e of i n t e r i o r w a l l c a v i t y (bedroom) 3.25 I n s i d e of e x t e r i o r w a l l c a v i t y 0.5

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T h i s paper i s being d i s t r i b u t e d i n r e p r i n t form by t h e I n s t i t u t e f o r Research i n C o n s t r u c t i o n . A l i s t of b u i l d i n g p r a c t i c e and r e s e a r c h p u b l i c a t i o n s a v a i l a b l e from t h e I n s t i t u t e may be o b t a i n e d by w r i t i n g t o t h e P u b l i c a t i o n s S e c t i o n , I n s t i t u t e f o r R e s e a r c h i n C o n s t r u c t i o n , N a t i o n a l Research C o u n c i l of C a n a d a , O t ' t a w a , O n t a r i o , K l A 0R6. Ce document e s t d i s t r i b u 6 s o u s forme de t i r 6 - 8 - p a r t p a r 1 ' I n s t i t u t de r e c h e r c h e en c o n s t r u c t i o n . On p e u t o b t e n i r une l i s t e d e s p u b l i c a t i o n s de 1' I n s t i t u t p o r t a n t s u r les t e c h n i q u e s ou

les

r e c h e r c h e s e n

matisre

d e b a t i m e n t e n C c r i v a n t

3

l a S e c t i o n d e s p u b l i c a t i o n s , I n s t i t u t de r e c h e r c h e en c o n s t r u c t i o n , C o n s e i l n a t i o n a l d e r e c h e r c h e s du Canada, Ottawa ( O n t a r i o ) ,

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