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HISTORICAL REVIEW OF STUDIES ON AIR QUALITY AND CARBON SCIENCE IN SUB-SAHARIAN AFRICA

CATHY LIOUSSE, LABORATOIRE D’AEROLOGIE

The DACCIWA Air pollution and Health team

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ONCE UPON A TIME :

¡ 1990 : FOS-DECAFE on biomass burning in Cote d’Ivoire : emissions, atmospheric composition.

¡ 1992 : SAFARI on biomass burning in South Africa : emissions, atmospheric composition, climate, ecology (at the same time TRACE-A experiment on transport, chemical composition of the atmosphere over the tropical South Atlantic Ocean)

¡ 1996 : EXPRESSO on biomass burning in Central Africa : emissions, atmospheric composition

¡ From 1994 : IDAF (now INDAAF) long-term network of observations on atmospheric composition and deposition (8 rural sites in West and Central Africa (Niger, Mali, Senegal, Benin, Côte d’Ivoire, Cameroon and Congo); still active : see https://indaaf.obs-mip.fr/network/ with link to DEBITS in South Africa (4 sites);

in 2020, the INSA project on Integrated Nitrogen Studies.

¡ 2006 : AMMA project in West Africa on Monsoon, Climate, Weather predictions : this includes important works on biomass burning and dust emissions, aerosol measurements in rural areas, regional modeling on aerosol radiative impact.

¡ From 2012 : WASCAL project on climate change studies and climate services (https://wascal.org/projects/)

Laurent et al. 2008, Liousse et al., 2010, Tummon et al., 2010, Malavelle et al., 2011, Ndatchoh et al. 2015, Ouafo et al. 2018 etc..

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BIOMASS BURNING EMISSIONS

Liousse et al., 2010, Granier et al., 2011, Stroppiana et al. 2011, N’Datchoh et al., in prep.

AMMABB GFED-GFAS AMMABB - GFED

After having tested the role of emission factor and burnt area data, lack of knowledge on vegetation parametrization seems to be responsible for such differences

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BIOMASS BURNING AND DUST SOURCES ARE NOT THE ONLY CAUSES OF POLLUTION IN AFRICA

A cocktail of pollutants Large increase of urban population

1950 2050 Few regulations

Intense photochemistry

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ONCE UPON A TIME : STUDIES ON AIR QUALITY

¡ 2005: first experiments on air pollution in Cotonou (Benin) during the AMMA project

¡ 2008: POLCA on Air pollution and Health in Bamako (Mali), Dakar (Senegal) and Yaoundé (Cameroon)

¡ 2014: Anthropogenic emission inventories in Africa for 2005 and 2030

¡ 2016: DICE anthropogenic emission inventory in Africa by Marais and Wiedinmeyer

¡ 2014-2018 : DACCIWA on Air pollution and Health in Abidjan (Cote d’Ivoire) and Cotonou (Benin), emission inventory studies and health impact

¡ 2015-2018 : CHAIREPOL on Air Pollution and Health in Abidjan, Ouagadougou, Cotonou and Dakar (indoor and outdoor pollution)

¡ 2018-2022 : PASMU on Air pollution and Health in Abidjan and Korhogo

¡ From 2015 : GDRI-ARSAIO on Air pollution and Health in South Africa

¡ A few other studies conducted in Dakar, Cotonou, Accra by local universities with international collaborations

Yaoundé Accra

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PARTICULATE MATTER CONCENTRATIONS ARE ALWAYS HIGHER THAN THE WHO NORMS

From Djossou et al., 2018 (DACCIWA results) Confirmed by recent papers

(e.g. Adon et al., 2020, Gnamien et al. 2020)

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ORGANIC CARBON AND DUST PARTICLES ARE THE MOST IMPORTANT AEROSOL COMPONENTS WITH STRONG SEASONAL VARIATIONS

Cotonou-wet season Dakar

BC OC Dust Water soluble

Ouagadougou Bamako

Abidjan-traffic Cotonou - traffic Abidjan- wood burning site

POLCA and AMMA campaigns Val et al., 2013 (Doumbia phD) Cachier, pers. com.

DACCIWA dry season Adon et al., 2020

South Africa : Vaal triangle Josipovic et al., 2018

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0 2 4 6 8 0

5 10

15 BK1

BK2DK Fines

POM (µg/cm2)

GM-CSF/Temoin

THE AEROSOL PRO-INFLAMMATORY RESPONSE HIGHLY

CORRELATED WITH CARBONACEOUS AEROSOL (BC, OC, WSOC)

POLCA campaign : Val et al., 2013 DACCIWA campaign : Tran et al., in prep.

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HIGH SPATIAL VARIABILITY OF POLLUTANT CONCENTRATIONS AT A CITY SCALE (E.G. ABIDJAN)

NO2 PM2.5

DACCIWA program : Bahino et al., 2018 PASMU program : Gnamien et al., 2020

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NEARLY ONE MILLION OF PEOPLE PER YEAR DIED FROM AIR POLLUTION IN AFRICA

0 10000 20000 30000 40000 50000 60000 70000 80000 90000 100000

Angola Burundi Benin Burkina Faso Central African Rep, te d'Ivoire Cameroon Dem, Rep, Congo Congo Cape Verde Djibouti Algeria Egypt Eritrea Ethiopia Gabon Ghana Guinea Gambia Guinea-Bissau Eq, Guinea Kenya Liberia Libya Lesotho Morocco Madagascar Mali Mozambique Mauritania Mauritius Malawi Namibia Niger Nigeria Rwanda W, Sahara Sudan S, Sudan Senegal Sierra Leone Somalia o Tomé and Principe Swaziland Seychelles Chad Togo Tunisia Tanzania Uganda South Africa Zambia Zimbabwe Premature deaths (all causes)

285000

DACCIWA results : N’Datchoh et al., in prep., from RegCM anthropogenic PM2.5 modeling.

In agreement with data given by Lelieveld et al., 2020 and by WHO.

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EXPLOSIVE EMISSIONS AND IMPACTS IF NO MITIGATIONS ARE PLANIFIED

African anthropogenic emissions of organic particles could lead the world (25% in 2005 => 60% in 2030) Emissions x 4 => OC x 4 in urban areas and x 2.5 in rural areas (RegCM modeling)

Liousse et al., 2014

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EMISSION FACTOR MEASUREMENTS : A TOOL TO TEST MITIGATION EFFORT

TRAFFIC EF

0 1 2 3 4 5

Vieilles

essences Essences

récentes Vieilles

diesel Diesel

récent Vieilles

MobylettesMobylettes

récentes Motos Gbaka

124 26

5

Black: BC Green : OC

/5 /50

Keita et al., 2018

/5

DECAFE 1991

DACCIWA 2016 POLCA 2009 AMMA 2005 POLCA 2009

DACCIWA 2016

DACCIWA 2016

Needs to focus on residential, waste burning, and traffic sectors

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TAKE-HOME MESSAGES

¡ Long-term measurements of air pollution in african megacities are urgently needed

¡ Emissions : need local observations and international intercomparisons

¡ New proxys for health such as aerosol oxydant capacity are really important to study air pollution and health effects

¡ Reconciling epidemiological studies with biological studies : need more cohort studies with personal exposure measurements (exposology) : a way to act on source mitigation.

¡ Need to integrate sociological factors to take into account the people vulnerability to air pollution

¡ Do not separe urban studies on health and climate (we need win-win results).

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Thanks for your attention

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