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HAL Id: hal-02572712

https://hal.univ-angers.fr/hal-02572712

Preprint submitted on 13 May 2020

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Solitons à quelques cycles dans la dynamique de génération de supercontinuum

Philippe Grelu, Dumitru Mihalache, Houria Triki, Hervé Leblond, D Grelu, H Mihalache

To cite this version:

Philippe Grelu, Dumitru Mihalache, Houria Triki, Hervé Leblond, D Grelu, et al.. Solitons à quelques cycles dans la dynamique de génération de supercontinuum. 2020. �hal-02572712�

(2)

Non-SVEA models for supercontinuum generation

Herv´ e Leblond

1

, Philippe Grelu

2

, Dumitru Mihalache

3

, Houria Triki

4

1Laboratoire de Photonique d’Angers LϕA EA 4464, Universit´e d’Angers, France

2Laboratoire Interdisciplinaire Carnot de Bourgogne, UMR 6303 CNRS, Dijon, France

3Horia Hulubei National Institute for Physics and Nuclear Engineering, and Academy of Romanian Scientists, Bucharest, Romania

4Radiation Physics Laboratory, Badji Mokhtar University, Annaba, Algeria

(3)

1 Models for few-cycle solitons

The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3

Supercontinuum generation Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(4)

1 Models for few-cycle solitons

The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3

Supercontinuum generation Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(5)

Introduction

The shortest laser pulses: a duration of a few optical cycles.

Autocorrelation trace, R. Ell et al., Optics Letters 26 (6), 373 (2001).

Pulse duration down to a few fs. Ex. above: 5

fs

=

5×10−15s.

How to model the propagation of such pulses?

(6)

Solitary wave vs envelope solitons

Envelope soliton: the usual optical soliton in the ps range

Pulse durationLλwavelength Typical model: NonLinear Schr¨odinger equation (NLS)

Solitary wave soliton: the hydrodynamical soliton

A single oscillation

Typical model: Korteweg-de Vries equation (KdV)

Few-cycle optical solitons:

L∼λ

The slowly varying envelope approximation is not valid Generalized NLS equation

(7)

Solitary wave vs envelope solitons

Envelope soliton: the usual optical soliton in the ps range

Pulse durationLλwavelength Typical model: NonLinear Schr¨odinger equation (NLS)

Solitary wave soliton: the hydrodynamical soliton

A single oscillation

Typical model: Korteweg-de Vries equation (KdV)

Few-cycle optical solitons:

L∼λ

The slowly varying envelope approximation is not valid Generalized NLS equation

We seek a different approach based on KdV-type models

(8)

Solitary wave vs envelope solitons

Envelope soliton: the usual optical soliton in the ps range

Pulse durationLλwavelength Typical model: NonLinear Schr¨odinger equation (NLS)

Solitary wave soliton: the hydrodynamical soliton

A single oscillation

Typical model: Korteweg-de Vries equation (KdV)

Few-cycle optical solitons:

L∼λ

The slowly varying envelope approximation is not valid Generalized NLS equation

We seek a different approach based on KdV-type models

(9)

A transparent medium

The general spectrum of a transparent medium

1/p

12

A simple model: A two-component medium, each component is described by a two-level model

We assume that the FCP duration

τp

is such that

ω1

(1/τ

p

)

ω2

(10)

A transparent medium

The general spectrum of a transparent medium

1/p

12

A simple model: A two-component medium, each component is described by a two-level model

1/

p

1

2

We assume that the FCP duration

τp

is such that

ω1

(1/τ

p

)

ω2

(11)

A transparent medium

The general spectrum of a transparent medium

1/p

12

A simple model: A two-component medium, each component is described by a two-level model

1 / 

p

1

2

We assume that the FCP duration

τp

is such that

ω1

(1/τ

p

)

ω2

(12)

A transparent medium

A simple model: A two-component medium, each component is described by a two-level model

1 / 

p

1

2

We assume that the FCP duration

τp

is such that

ω1

(1/τ

p

)

ω2

In a first stage, the two components are treated separately UV transition only, with (1/τ

p

)

ω2

=⇒

Long-wave approximation

(13)

A transparent medium

A simple model: A two-component medium, each component is described by a two-level model

1 / 

p

1

2

We assume that the FCP duration

τp

is such that

ω1

(1/τ

p

)

ω2

In a first stage, the two components are treated separately UV transition only, with (1/τ

p

)

ω2

=⇒

Long-wave approximation

(14)

A transparent medium

A simple model: A two-component medium, each component is described by a two-level model

1 / 

p

1

2

We assume that the FCP duration

τp

is such that

ω1

(1/τ

p

)

ω2

In a first stage, the two components are treated separately UV transition only, with (1/τ

p

)

ω2

1/

p

2

=⇒

Long-wave approximation

(15)

A transparent medium

In a first stage, the two components are treated separately UV transition only, with (1/τ

p

)

ω2

1/

p

2

=⇒

Long-wave approximation

modified Korteweg-de Vries (mKdV) equation

∂E

∂ζ

= 1 6

d3k dω3 ω=0

3E

∂τ3

ncχ(3)

(ω;

ω,ω,−ω) ω=0

∂E3

∂τ

H. Leblond and F. Sanchez,Phys. Rev. A67, 013804 (2003)

(16)

A transparent medium

In a first stage, the two components are treated separately IR transition only, with

ω1

(1/τ

p

)

=⇒

Short-wave approximation sine-Gordon (sG) equation:

2ψ

∂z∂t

=

c1

sin

ψ

with

c1

=

w

wr

: normalized initial population difference and

∂ψ

∂t

=

E

Er

: normalized electric field

H. Leblond and F. Sanchez,Phys. Rev. A67, 013804 (2003)

(17)

A transparent medium

In a first stage, the two components are treated separately IR transition only, with

ω1

(1/τ

p

)

1/

p

1

=⇒

Short-wave approximation sine-Gordon (sG) equation:

2ψ

∂z∂t

=

c1

sin

ψ

with

c1

=

w

wr

: normalized initial population difference and

∂ψ

∂t

=

E Er

: normalized electric field

H. Leblond and F. Sanchez,Phys. Rev. A67, 013804 (2003)

(18)

A transparent medium

In a first stage, the two components are treated separately IR transition only, with

ω1

(1/τ

p

)

1/

p

1

=⇒

Short-wave approximation sine-Gordon (sG) equation:

2ψ

∂z∂t

=

c1

sin

ψ

with

c1

=

w

wr

: normalized initial population difference and

∂ψ

∂t

=

E Er

: normalized electric field

H. Leblond and F. Sanchez,Phys. Rev. A67, 013804 (2003)

(19)

A transparent medium

Then the two approximations are brought together to yield a general model:

The mKdV-sG equation

2ψ

∂z∂t

+

c1

sin

ψ

+

c2

∂t ∂ψ

∂t 3

+

c3

4ψ

∂t4

= 0

∂u

∂z

+

c1

sin

Z t

u

+

c2

∂u3

∂t

+

c3

3u

∂t3

= 0 with

u

=

∂ψ

∂t

=

E

Er

: normalized electric field

Integrable by inverse scattering transform in some cases:

,

(20)

A transparent medium

Then the two approximations are brought together to yield a general model:

The mKdV-sG equation

2ψ

∂z∂t

+

c1

sin

ψ

+

c2

∂t ∂ψ

∂t 3

+

c34ψ

∂t4

= 0 Or

∂u

∂z

+

c1

sin

Z t

u

+

c2∂u3

∂t

+

c33u

∂t3

= 0 with

u

=

∂ψ

∂t

=

E

Er

: normalized electric field

Integrable by inverse scattering transform in some cases:

,

(21)

A transparent medium

Then the two approximations are brought together to yield a general model:

The mKdV-sG equation

∂u

∂z

+

c1

sin

Z t

u

+

c2

∂u3

∂t

+

c3

3u

∂t3

= 0 with

u

=

∂ψ

∂t

=

E

Er

: normalized electric field

Integrable by inverse scattering transform in some cases:

,

(22)

A transparent medium

Then the two approximations are brought together to yield a general model:

The mKdV-sG equation

∂u

∂z

+

c2

∂u3

∂t

+

c3

3u

∂t3

= 0 with

u

=

∂ψ

∂t

=

E Er

: normalized electric field

Integrable by inverse scattering transform in some cases:

mKdV,

(23)

A transparent medium

Then the two approximations are brought together to yield a general model:

The mKdV-sG equation

∂u

∂z

+

c1

sin

Z t

u

= 0

with

u

=

∂ψ

∂t

=

E Er

: normalized electric field

Integrable by inverse scattering transform in some cases:

mKdV, sG,

(24)

A transparent medium

Then the two approximations are brought together to yield a general model:

The mKdV-sG equation

∂u

∂z

+

c1

sin

Z t

u

+

c2∂u3

∂t

+ 2c

23u

∂t3

= 0 with

u

=

∂ψ

∂t

=

E

Er

: normalized electric field

Integrable by inverse scattering transform in some cases:

mKdV, sG, and

c3

= 2c

2

.

(25)

The analytical breather solution

1 2

2 4 6

-4 -2

-6 0

-0.05 0.05

0

E

-2 0

-1

A few cycle soliton:

Not spread out by dispersion Stable

However, oscillates (breather)

H. Leblond, S.V. Sazonov, I.V. Mel’nikov, D. Mihalache, and F. Sanchez,

(26)

1

Models for few-cycle solitons The mKdV-sG equation

2 A few generalizations

General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3

Supercontinuum generation Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(27)

1

Models for few-cycle solitons The mKdV-sG equation

2 A few generalizations

General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3

Supercontinuum generation Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(28)

More than two An arbitrary number of atomic levels

UV transitions:

mKdV model generalizes without modification to a general Hamiltonian,

with an arbitrary number of atomic levels.

H. Triki, H. Leblond, D. Mihalache,Opt. Comm.285, 3179-3186 (2012)

IR transitions: Not so simple The sG model

Hence population inversion

w

is explicitly involved.

Generalization: one

w

for each transition.

(29)

More than two An arbitrary number of atomic levels

UV transitions:

mKdV model generalizes without modification to a general Hamiltonian,

with an arbitrary number of atomic levels.

H. Triki, H. Leblond, D. Mihalache,Opt. Comm.285, 3179-3186 (2012)

IR transitions: Not so simple The sG model

Hence population inversion

w

is explicitly involved.

Generalization: one

w

for each transition.

(30)

More than two An arbitrary number of atomic levels

IR transitions: Not so simple The sG model can be written as:

∂E

∂z

=

−N

ε0c

ΩQ

~∂w

∂t

=

−EQ

~∂Q

∂t

=

|µ|2Ew

identical to Self Induced Transparency equations,

but with real

E

and

Q.

Hence population inversion

w

is explicitly involved.

Generalization: one

w

for each transition.

(31)

More than two An arbitrary number of atomic levels

IR transitions: Not so simple The sG model can be written as:

∂E

∂z

=

−N

ε0c

ΩQ

~∂w

∂t

=

−EQ

~∂Q

∂t

=

|µ|2Ew

identical to Self Induced Transparency equations,

but with real

E

and

Q.

Hence population inversion

w

is explicitly involved.

Generalization: one

w

for each transition.

(32)

More than two An arbitrary number of atomic levels

IR transitions: Not so simple

The sG model for 2 transitions (4 level), generalises to:

∂E

∂z

=

−NΩ

ε0c

(Ω

1Q1

+ Ω

2Q2

)

~

∂wj

∂t

=

−EQj, j

= 1, 2

~∂Qj

∂t

=

j|2Ewj, j

= 1, 2 Hence population inversion

w

is explicitly involved.

Generalization: one

w

for each transition.

(33)

The above system reduces to

∂u

∂z

+

c1

sin

Z τ

udτ0

+

qc1

sin

ν Z τ

udτ0

= 0

−→

a generalized double sine-Gordon equation Both admit breather solutions:

H. Triki, H. Leblond, D. Mihalache,Phys. Rev. A86, 063825 (2012)

(34)

The above system reduces to

∂u

∂z

+

c1

sin

Z τ

udτ0

+

qc1

sin 2

Z τ

udτ0

= 0

−→

a generalized double sine-Gordon equation

Under certain conditions: the double sine Gordon equation (ν = 2).

Both admit breather solutions:

H. Triki, H. Leblond, D. Mihalache,Phys. Rev. A86, 063825 (2012)

(35)

The above system reduces to

∂u

∂z

+

c1

sin

Z τ

udτ0

+

qc1

sin

ν Z τ

udτ0

= 0

−→

a generalized double sine-Gordon equation Both admit breather solutions:

0 10

20 30

Z

-0.5 -1 0.5 0

1.5 1

T

-30 -20 -10 0 10 20 30

ψ

0 5

10 15

20 25

Z

-1 -1.5 0 -0.5

1 0.5

T

-30 -20 -10 0 10 20 30

ψ

Left:ν= 2,q= 0.2; right:ν=

3,q= 0.4.

(36)

1

Models for few-cycle solitons The mKdV-sG equation

2 A few generalizations

General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3

Supercontinuum generation Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(37)

Complex mKdV

Consider UV transitions only, and vectorial electric field (U

,V

) Two coupled mKdV equations

(normalized form)

:

UZ

=

UTTT

+

U2

+

V2 U

T

VZ

=

VTTT

+

U2

+

V2 V

T

Setting

f

=

U

+

iV,

reduce to

fZ

=

fTTT

+

|f|2f

T,

(1)

−→

The complex modified Korteweg-de Vries (cmKdV) equation.

Avoid confusion with

fZ

=

fTTT

+

|f|2

fT.

(2)

Eq. (2) is completely integrable while Eq. (1) is not.

Eq. (1): cmKdV I; Eq. (2) cmKdV II.

(38)

Complex mKdV

Consider UV transitions only, and vectorial electric field (U

,V

) Two coupled mKdV equations

(normalized form)

:

UZ

=

UTTT

+

U2

+

V2 U

T

VZ

=

VTTT

+

U2

+

V2 V

T

Setting

f

=

U

+

iV,

reduce to

fZ

=

fTTT

+

|f|2f

T,

(1)

−→

The complex modified Korteweg-de Vries (cmKdV) equation.

Avoid confusion with

fZ

=

fTTT

+

|f|2

fT.

(2)

Eq. (2) is completely integrable while Eq. (1) is not.

Eq. (1): cmKdV I; Eq. (2) cmKdV II.

(39)

Complex mKdV

Consider UV transitions only, and vectorial electric field (U

,V

) Two coupled mKdV equations

(normalized form)

:

UZ

=

UTTT

+

U2

+

V2 U

T

VZ

=

VTTT

+

U2

+

V2 V

T

Setting

f

=

U

+

iV,

reduce to

fZ

=

fTTT

+

|f|2f

T,

(1)

−→

The complex modified Korteweg-de Vries (cmKdV) equation.

Avoid confusion with

fZ

=

fTTT

+

|f|2

fT.

(2)

Eq. (2) is completely integrable while Eq. (1) is not.

Eq. (1): cmKdV I; Eq. (2) cmKdV II.

(40)

Complex mKdV

Consider UV transitions only, and vectorial electric field (U

,V

) Two coupled mKdV equations

(normalized form)

:

UZ

=

UTTT

+

U2

+

V2 U

T

VZ

=

VTTT

+

U2

+

V2 V

T

Setting

f

=

U

+

iV,

reduce to

fZ

=

fTTT

+

|f|2f

T,

(1)

−→

The complex modified Korteweg-de Vries (cmKdV) equation.

Avoid confusion with

fZ

=

fTTT

+

|f|2

fT.

(2)

Eq. (2) is completely integrable while Eq. (1) is not.

Eq. (1): cmKdV I; Eq. (2) cmKdV II.

(41)

fZ

=

fTTT

+

|f|2f

T,

Linearly polarized solitons:

f

=

f0

(Z

,T

)e

, with

f0

solution of mKdV (real) and

φ

constant.

U

=

f0

(Z

,T

) cos

φ, V

=

f0

(Z

,T

) sin

φ

More interesting would be a circularly polarized soliton:

f

=

u(T −wZ

)e

i(ωT−kZ).

If

u

=

ae

,

U

=

a(T −wZ

) cos(ωT

−kZ

+

φ(T −wZ

))

V

=

a(T −wZ

) sin(ωT

−kZ

+

φ(T −wZ

))

However no

exact, even numerical, steady state solution of this type,

but very robust

approximate

ones.

(42)

fZ

=

fTTT

+

|f|2f

T,

Linearly polarized solitons:

f

=

f0

(Z

,T

)e

, with

f0

solution of mKdV (real) and

φ

constant.

U

=

f0

(Z

,T

) cos

φ, V

=

f0

(Z

,T

) sin

φ

More interesting would be a circularly polarized soliton:

f

=

u(T −wZ

)e

i(ωT−kZ).

If

u

=

ae

,

U

=

a(T −wZ

) cos(ωT

−kZ

+

φ(T −wZ

))

V

=

a(T −wZ

) sin(ωT

−kZ

+

φ(T −wZ

))

However no

exact, even numerical, steady state solution of this type,

but very robust

approximate

ones.

(43)

fZ

=

fTTT

+

|f|2f

T,

Linearly polarized solitons:

f

=

f0

(Z

,T

)e

, with

f0

solution of mKdV (real) and

φ

constant.

U

=

f0

(Z

,T

) cos

φ, V

=

f0

(Z

,T

) sin

φ

More interesting would be a circularly polarized soliton:

f

=

u(T −wZ

)e

i(ωT−kZ).

If

u

=

ae

,

U

=

a(T −wZ

) cos(ωT

−kZ

+

φ(T −wZ

))

V

=

a(T −wZ

) sin(ωT

−kZ

+

φ(T −wZ

))

However no

exact, even numerical, steady state solution of this type,

but very robust

approximate

ones.

(44)

fZ

=

fTTT

+

|f|2f

T,

Linearly polarized solitons:

f

=

f0

(Z

,T

)e

, with

f0

solution of mKdV (real) and

φ

constant.

U

=

f0

(Z

,T

) cos

φ, V

=

f0

(Z

,T

) sin

φ

More interesting would be a circularly polarized soliton:

f

=

u(T −wZ

)e

i(ωT−kZ).

If

u

=

ae

,

U

=

a(T −wZ

) cos(ωT

−kZ

+

φ(T −wZ

))

V

=

a(T −wZ

) sin(ωT

−kZ

+

φ(T −wZ

))

However no

exact, even numerical, steady state solution of this type,

but very robust

approximate

ones.

(45)

T

Z

-40

-20 0 20

40

0 0.5 1 1.5 2 2.5 3 3.5 4

Linear propagation

(46)

T

Z

-40

-20 0 20

40

0 2 4 6 8 10 12

The circularly polarized FCP: amplitude

|u|

(47)

T

Z

-40

-20 0 20

40

0 2 4 6 8 10 12

The circularly polarized FCP:

Ex

=

Re(U

)

(48)

The circularly polarized FCP is unstable in subcycle range

(forωτp<1.4)

Initial (Z = 100): breather withω= 1,τp= 1,|f|;, U=Re(f).

Final (Z = 10000):, |f|; ,U;, V =Im(f).

Black: fit of final|f|by a fundamental soliton of real mKdV.

H. Leblond, H. Triki, F. Sanchez, D. Mihalache,Phys. Rev. A83, 063802 (2011)

(49)

1

Models for few-cycle solitons The mKdV-sG equation

2 A few generalizations

General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3

Supercontinuum generation Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(50)

One IR transition, for a vectorial field (U,V ).

Excited state for

x-polarization differs from excited state for y-polarization

−→

two population differences

w1

and

w2

. No reduction to sG, but a complicated system

UZ

=

−PT PT

=

−M −iUK MT

=

wU−sU

KT

=

Im

(U

P

)

sT

=

UM

wT

=

−3Re

(U

M) U =u+iv: electric field;P=p+iq: polarization density w = (w1+w2)/2,s= (w2−w1)/2−iS: population differences K real,M complex

(51)

One IR transition, for a vectorial field (U,V ).

Excited state for

x-polarization differs from excited state for y-polarization

−→

two population differences

w1

and

w2

. No reduction to sG, but a complicated system

UZ

=

−PT PT

=

−M −iUK MT

=

wU−sU

KT

=

Im

(U

P

)

sT

=

UM

wT

=

−3Re

(U

M) U =u+iv: electric field;P=p+iq: polarization density w = (w1+w2)/2,s= (w2−w1)/2−iS: population differences K real,M complex

(52)

One IR transition, for a vectorial field (U,V ).

Excited state for

x-polarization differs from excited state for y-polarization

−→

two population differences

w1

and

w2

. No reduction to sG, but a complicated system

UZ

=

−PT PT

=

−M −iUK MT

=

wU−sU

KT

=

Im

(U

P

)

sT

=

UM

wT

=

−3Re

(U

M) U =u+iv: electric field;P=p+iq: polarization density w = (w1+w2)/2,s= (w2−w1)/2−iS: population differences K real,M complex

(53)

If we set

U

=

fe

, with

φ

constant, i.e. we look for a linearly polarized pulse:

The system reduces to sine-Gordon.

We look for a circularly polarized FCP.

No exact solution

An approximate solution valid in the SVEA:

U

=

bei

h k−b2k

ω2

Z−ωTi

sech

b

T

+

k ωZ

.

Stable in the SVEA limit

But unstable in the sub-cycle range

(54)

0 20 40 60 80 100 500 140

0.4 0.5 0.6 0.7 0.8 0.9 1 1.1

z

max

/ z

disp

Number of cycles

The lifetime of the circularly polarized FCP,

(Red: numerical data. Light blue: exponential fit)

(55)

T

Z

0

20

40

60

80

100

0 100 200 300 400

The circularly polarized FCP decays into orthogonally polarized single-humped pulses.

= 5,b= 2)

(56)

Polarization vector (Re(U ),Im(U )) Time profiles of

Re(U)

and

Im(U)

H. Leblond, H. Triki, D. MihalachePhys. Rev. A84, 023833 (2011)

(57)

-1 -0.5 0 0.5 1 1.5 2

-2 -1.5 -1 -0.5 0 0.5 1 1.5

v

u

Polarization vector (Re(U ),Im(U))

Initial, 1 circularly pol. pulse, Final, 2 linearly pol. pulses.

-2 -1 0 1 2

0 20 40 60 80 100

±

|( u,v )|, u

T

Time profiles of

±|U|

and

Re(U)

H. Leblond, H. Triki, D. MihalachePhys. Rev. A84, 023833 (2011)

(58)

1

Models for few-cycle solitons The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3 Supercontinuum generation

Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(59)

1

Models for few-cycle solitons The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3 Supercontinuum generation

Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(60)

Supercontinuum generation

An intense laser pulse launched in a fiber (photonic crystal fiber especially) turns into white coherent light

The usual theory uses a generalized NLS model, i.e. slowly varying envelope.

In principle, SVEA assumes a narrow spectral width!

Our models may account for supercontinuum generation

(61)

Supercontinuum generation

An intense laser pulse launched in a fiber (photonic crystal fiber especially) turns into white coherent light

The usual theory uses a generalized NLS model, i.e. slowly varying envelope.

In principle, SVEA assumes a narrow spectral width!

Our models may account for supercontinuum generation

(62)

Supercontinuum generation

An intense laser pulse launched in a fiber (photonic crystal fiber especially) turns into white coherent light

The usual theory uses a generalized NLS model, i.e. slowly varying envelope.

In principle, SVEA assumes a narrow spectral width!

Our models may account for supercontinuum generation

(63)

The mKdV equation:

∂u

∂z

+

c2

∂u3

∂t

+

c3

3u

∂t3

= 0 Input is a Gaussian pulse:

u(0,t) =A

sin(ωt )e

−t22.

Normalized (dimensionless),

c2

=

c3

= 1 Optical period 2π

ω

and pulse duration

τ

: same as a 100 fs long pulse,

λ

= 1µm.

Numerical resolution...

(64)

z

ν

50

40

30

20

10

00 1 2 3 4 5

-160 -140 -120 -100 -80 -60 -40 -20 0 (dB)

mKdV, input withFWHM= 100,ν= 0.3,A= 0.7.

A very broad spectrum is reached quickly.

(65)

1

Models for few-cycle solitons The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3 Supercontinuum generation

Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(66)

Question: generation of frequencies lower than

ω?

We solve numerically the mKdV, sG and mKdV-sG models starting with a 100 fs pulse,

λ

= 1µm

−→

Compare the evolution of the spectrum

(67)

Comparison between

mKdV,sG, andmKdV-sG

models

Forz= 0, 6, 12, and 16.

sG

extends first towards

Stokes

side,

mKdV

extends first towards

anti-Stokes.

mKdV-sG

model lies in between.

(68)

Recall that

mKdV accounts for UV transitions, and sG for IR transitions.

Usual Raman broadening yields extension of the spectrum towards low frequencies at the beginning of the process and is due to IR

transitions.

Although Raman effect itself

is not taken into account by sG model,

the corresponding spectral broadening is.

(69)

Recall that

mKdV accounts for UV transitions, and sG for IR transitions.

Usual Raman broadening yields extension of the spectrum towards low frequencies at the beginning of the process and is due to IR

transitions.

Although Raman effect itself

is not taken into account by sG model,

the corresponding spectral broadening is.

(70)

Recall that

mKdV accounts for UV transitions, and sG for IR transitions.

Usual Raman broadening yields extension of the spectrum towards low frequencies at the beginning of the process and is due to IR

transitions.

Although Raman effect itself

is not taken into account by sG model,

the corresponding spectral broadening is.

(71)

1

Models for few-cycle solitons The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3 Supercontinuum generation

Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(72)

A quasi monochromatic wave

u

=

U

(z,t)e

i(kz−ωt)

+

cc

+

u1

(z,t), (3)

U

: fundamental wave amplitude;

u1

: small correction.

Neglect dispersion, and disregard third harmonic generation:

U

=

A

2 exp

i

c1

3

+ 3ωc

2

A2

4

z

.

(4)

Self phase modulation.

−→

broadening of the spectrum

with typical oscillations of the spectral density.

(73)

A quasi monochromatic wave

u

=

U

(z,t)e

i(kz−ωt)

+

cc

+

u1

(z,t), (3)

U

: fundamental wave amplitude;

u1

: small correction.

Neglect dispersion, and disregard third harmonic generation:

U

=

A

2 exp

i

c1

3

+ 3ωc

2

A2

4

z

.

(4)

Self phase modulation.

−→

broadening of the spectrum

with typical oscillations of the spectral density.

(74)

A quasi monochromatic wave

u

=

U

(z,t)e

i(kz−ωt)

+

cc

+

u1

(z,t), (3)

U

: fundamental wave amplitude;

u1

: small correction.

Neglect dispersion, and disregard third harmonic generation:

U

=

A

2 exp

i

c1

3

+ 3ωc

2

A2

4

z

.

(4)

Self phase modulation.

−→

broadening of the spectrum

with typical oscillations of the spectral density.

(75)

Numerical

mKdV

vs analytical

self-phase modulation, Eq. (4)

0 30 60

0.28 0.3 ν 0.32 0.34

0 20 40

0.28 0.3 ν 0.32 0.34

0 15 30

0.28 0.3 0.32 0.34

spectrum ν

0 15 30

0.28 0.3 ν 0.32 0.34

0 10 20

0.28 0.3 ν 0.32 0.34

FWHM= 100,ν= 0.3,A= 0.7, forz= 0, 2, 4, 10, 20.

Then

actual broadening

becomes asymmetric, while

analytic formula

remains symmetric.

The very beginning of the broadening process

is due to self phase modulation.

(76)

Numerical

mKdV

vs analytical

self-phase modulation, Eq. (4)

0 30 60

0.28 0.3 ν 0.32 0.34

0 20 40

0.28 0.3 ν 0.32 0.34

0 15 30

0.28 0.3 0.32 0.34

spectrum ν

0 15 30

0.28 0.3 ν 0.32 0.34

0 10 20

0.28 0.3 ν 0.32 0.34

FWHM= 100,ν= 0.3,A= 0.7, forz= 0, 2, 4, 10, 20.

Analytic envelope approximation OK until

z '

4, Then

actual broadening

becomes asymmetric,

while

analytic formula

remains symmetric.

The very beginning of the broadening process

(77)

Numerical

mKdV

vs analytical

self-phase modulation, Eq. (4)

0 30 60

0.28 0.3 ν 0.32 0.34

0 20 40

0.28 0.3 ν 0.32 0.34

0 15 30

0.28 0.3 0.32 0.34

spectrum ν

0 15 30

0.28 0.3 ν 0.32 0.34

0 10 20

0.28 0.3 ν 0.32 0.34

FWHM= 100,ν= 0.3,A= 0.7, forz= 0, 2, 4, 10, 20.

Analytic envelope approximation OK until

z '

4, Then

actual broadening

becomes asymmetric,

while

analytic formula

remains symmetric.

The very beginning of the broadening process

(78)

Numerical

mKdV

vs analytical

self-phase modulation, Eq. (4)

0 30 60

0.28 0.3 ν 0.32 0.34

0 20 40

0.28 0.3 ν 0.32 0.34

0 15 30

0.28 0.3 0.32 0.34

spectrum ν

0 15 30

0.28 0.3 ν 0.32 0.34

0 10 20

0.28 0.3 ν 0.32 0.34

Then

actual broadening

becomes asymmetric, while

analytic formula

remains symmetric.

The very beginning of the broadening process

is due to self phase modulation.

(79)

1

Models for few-cycle solitons The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3 Supercontinuum generation

Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4

Few cycle solitons in supercontinuum generation The sG model

The mKdV model

(80)

A lot of high harmonics are created and involved in the process The SVEA does not account for high harmonic generation

z

ν

4.5 4 3.5 3 2.5 2 1.5 1 0.5

00 2 4 6 8 10 12 14 16 18

-160 -140 -120 -100 -80 -60 -40 -20 0 20

(dB)

Up to 15 harmonics can be seen

FWHM= 80,ν= 0.375, andA= 5, sG model.

(81)

Spectral width of harmonics

Assume a Gaussian profile

u

=

Ae

−t2 τ2 e−iω0t.

Its Fourier transform is ˆ

u

= 2

√ π Aτ e

−(ω−ω0)2τ2

4 .

The

nth harmonic is then un

=

Ae−nt

2

τ2 e−inω0t,

and its width is

τ

√n

. Consequently its Fourier transform is

(u

dn

) = 2

√ nπ Aτ e

−(ω−nω0)2τ2

4n .

Hence the spectral width of the

nth harmonic is

2

√ n τ

; it increases as

n.

(82)

Spectral width of harmonics

Assume a Gaussian profile

u

=

Ae

−t2 τ2 e−iω0t.

Its Fourier transform is ˆ

u

= 2

√ π Aτ e

−(ω−ω0)2τ2

4 .

The

nth harmonic is then un

=

Ae−nt

2

τ2 e−inω0t,

and its width is

τ

√n

. Consequently its Fourier transform is

(u

dn

) = 2

√ nπ Aτ e

−(ω−nω0)2τ2

4n .

Hence the spectral width of the

nth harmonic is

2

√ n τ

; it increases as

n.

(83)

Spectral width of harmonics

Assume a Gaussian profile

u

=

Ae

−t2 τ2 e−iω0t.

Its Fourier transform is ˆ

u

= 2

√ π Aτ e

−(ω−ω0)2τ2

4 .

The

nth harmonic is then un

=

Ae−nt

2

τ2 e−inω0t,

and its width is

τ

√n

. Consequently its Fourier transform is

(u

dn

) = 2

√ nπ Aτ e

−(ω−nω0)2τ2

4n .

Hence the spectral width of the

nth harmonic is

2

√ n τ

; it increases as

n.

(84)

Spectral width of harmonics

Assume a Gaussian profile

u

=

Ae

−t2 τ2 e−iω0t.

Its Fourier transform is ˆ

u

= 2

√ π Aτ e

−(ω−ω0)2τ2

4 .

The

nth harmonic is then un

=

Ae−nt

2

τ2 e−inω0t,

and its width is

τ

√n

. Consequently its Fourier transform is

(u

dn

) = 2

√ nπ Aτ e

−(ω−nω0)2τ2

4n .

Hence the spectral width of the

nth harmonic is

2

√ n τ

; it increases as

n.

(85)

Spectral width of harmonics

Assume a Gaussian profile

u

=

Ae

−t2 τ2 e−iω0t.

Its Fourier transform is ˆ

u

= 2

√ π Aτ e

−(ω−ω0)2τ2

4 .

The

nth harmonic is then un

=

Ae−nt

2

τ2 e−inω0t,

and its width is

τ

√n

. Consequently its Fourier transform is

(u

dn

) = 2

√ nπ Aτ e

−(ω−nω0)2τ2

4n .

Hence the spectral width of the

nth harmonic is

2

√ n τ

; it increases as

n.

(86)

Spectral widths of the harmonics.

mKdV

compared to

Gaussian

with width increasing as

√ n

-140 -120 -100 -80 -60 -40 -20 0 20

0 0.5 1 1.5 2 2.5 3 3.5 4

spectrum (dB)

ν

FWHM= 100,ν= 0.3, andA= 0.7, forz= 2.

(87)

Spectral broadening due to parametric interaction between the sidebands of the harmonics

and the ones of the fundamental.

ω0

: fundamental frequency. Assume a sideband

ω0

+

δω,

the third harmonics contains the sideband 3 (ω

0

+

δω).

It may interact with the fundamental

±ω0

:

−→

3 (ω

0

+

δω)−ω0−ω0

=

ω0

+ 3δω Hence

ω0

+

δω

creates

ω0

+ 3δω:

spectrum broadens

(88)

Spectral broadening due to parametric interaction between the sidebands of the harmonics

and the ones of the fundamental.

ω0

: fundamental frequency. Assume a sideband

ω0

+

δω,

the third harmonics contains the sideband 3 (ω

0

+

δω).

It may interact with the fundamental

±ω0

:

−→

3 (ω

0

+

δω)−ω0−ω0

=

ω0

+ 3δω Hence

ω0

+

δω

creates

ω0

+ 3δω:

spectrum broadens

(89)

Spectral broadening due to parametric interaction between the sidebands of the harmonics

and the ones of the fundamental.

ω0

: fundamental frequency. Assume a sideband

ω0

+

δω,

the third harmonics contains the sideband 3 (ω

0

+

δω).

It may interact with the fundamental

±ω0

:

−→

3 (ω

0

+

δω)−ω0−ω0

=

ω0

+ 3δω Hence

ω0

+

δω

creates

ω0

+ 3δω:

spectrum broadens

(90)

Spectral broadening due to parametric interaction between the sidebands of the harmonics

and the ones of the fundamental.

ω0

: fundamental frequency. Assume a sideband

ω0

+

δω,

the third harmonics contains the sideband 3 (ω

0

+

δω).

It may interact with the fundamental

±ω0

:

−→

3 (ω

0

+

δω)−ω0−ω0

=

ω0

+ 3δω Hence

ω0

+

δω

creates

ω0

+ 3δω:

spectrum broadens

(91)

Spectral broadening due to parametric interaction between the sidebands of the harmonics

and the ones of the fundamental.

ω0

: fundamental frequency. Assume a sideband

ω0

+

δω,

the third harmonics contains the sideband 3 (ω

0

+

δω).

It may interact with the fundamental

±ω0

:

−→

3 (ω

0

+

δω)−ω0−ω0

=

ω0

+ 3δω Hence

ω0

+

δω

creates

ω0

+ 3δω:

spectrum broadens

(92)

1

Models for few-cycle solitons The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3

Supercontinuum generation Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4 Few cycle solitons in supercontinuum generation

The sG model

The mKdV model

(93)

1

Models for few-cycle solitons The mKdV-sG equation

2

A few generalizations General Hamiltonian

Circular polarization - long wave Circular polarization - short wave

3

Supercontinuum generation Evidence for SC generation Stokes side

Self-phase modulation High harmonics generation

4 Few cycle solitons in supercontinuum generation

The sG model

The mKdV model

(94)

The sG equation,

∂u

∂z

+

c1

sin

Z τ

udτ0

= 0

c1= 50,A= 1 ( a change inc1results only in a change of the unit along thez-axis).

Input is a Gaussian pulse:

u(0,t) =A

sin(ωt )e

−t22.

A few FCP solitons form and tend to separate

-2

0 2

-200 -100 0 100 200 300 400 500

u

z

(95)

The sG equation,

∂u

∂z

+

c1

sin

Z τ

udτ0

= 0

c1= 50,A= 1 ( a change inc1results only in a change of the unit along thez-axis).

Input is a Gaussian pulse:

u(0,t) =A

sin(ωt )e

−t22.

A few FCP solitons form and tend to separate

-2

0 2

-200 -100 0 100 200 300 400 500

u

z

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