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Theoretical aspects of magnetic fluctuations
Ronald E. Burgess
To cite this version:
Ronald E. Burgess. Theoretical aspects of magnetic fluctuations. Revue de Physique Appliquée,
Société française de physique / EDP, 1970, 5 (1), pp.77-82. �10.1051/rphysap:019700050107700�. �jpa-
00243378�
THEORETICAL ASPECTS OF MAGNETIC FLUCTUATIONS
By RONALD E. BURGESS,
Department of Physics, University of British Columbia, Vancouver 8, B.C., Canada.
Abstract.
2014The thermodynamic treatment of equilibrium fluctuations in magnetic systems
is discussed and applied to
avariety of situations. The spectral density of the magnetic
moment or flux are derived for simply-connected bodies (sphere and cylinder) and for multiply-
connected systems (loop and hollow cylinder). The material is considered to be either
anormal conductor,
asuperconductor or ferromagnetic. The results are valid in the presence of
astatic
magnetic field and also if the susceptibility is field-dependent. No abrupt change in fluctua-
tions occurs as
asuperconductor is taken through the transition temperature. The introduc-
tion of
aJosephson junction or
aresistive link in
asuperconducting loop is shown to increase the flux fluctuations markedly with
asteady increase as the link is made weaker. At high fre- quencies the fluctuation spectrum for
asuperconductor approaches that for the same system
in the normal state.
PHYSIQUE APPLIQUEZ 5, 1970,
I. Introduction.
-Fluctuations of the magnetic
moment of a solid body of arbitrary shape can be
calculated for thermal equilibrium by means of the fluctuation-dissipation theorem. Similarly the flllc- tuations of flux and magnetic field within a loop or
other hollow body may be found.
Attention is hère devoted to various configurations
of normal conductors, ferromagnetics and supercon- ductors. The results are valid in the presence of an
arbitrary static magnetic field and the field-dependence
of magnetization (which may be non-linear) enters through the differential susceptibility which is in gene- ral a complex function of frequency.
The inapplicability of the simple form of the equi- partition principle commonly used to evaluate magne- tic fluctuations in superconductors arises from the
neglect of significant components of energy additional
to the magnetic field energy.
A superconducting system customarily exhibits appreciably smaller magnetic fluctuations than a nor-
mal metal system of the same configuration and has
a smaller relaxation time. Nevertheless the fluctua- tions are continuous through the transition température
as is the magnetic polarizability.
The total mean square fluctuation (integrated spec-
trum) of the magnetic moment or flux is simply related
to the polarizabilities at 0)
=0 and oo and to the
response of the system to an infinitesimal step function
of the external field.
In dealing with superconductors it proves to be
helpful to represent the inertia of the super and normal fluid components in terms of the kinetic inductances.
Similarly the behavior of a Josephson junction can be represented by an effective inductance for small phase
fluctuations. These equivalences are adopted here to provide uniformity of notation.
In practice the fluctuations of relevance may either be the integrated spectrum (in wideband systems) or
the low-frequency portion of the spectrum (in narrow
band systems). Special attention is therefore devoted
to these limiting forms. Depending on the configura-
tion either the fluctuations of magnetic moment (for
a solid body) or of magnetic flux (for a loop or hollow body) may be of primary interest.
Throughout the sinusoidal response functions are in terms of the function exp (icôt) and parameters are expressed in e.m.u.
Spectral densities for fluctuations are defined such that the variance of a quantity is given by the integral :
II. General Relations.
-We first note some general
relations connecting the spectrum of fluctuations and the integrated variance with the response function of the system to an external magnetic field.
If the magnetic moment of a body is m exp (Í6Jt) in
response to a small sinusoidal magnetic field H exp (Í6Jt)
their ratio is denoted by m/H
=rl(6J) where ce(m) is
the complex polarizability. This function is analytic
in the lower half of the 6J-plane and it follows by
contour integration that :
where oc
=a’
-ia". The dissipative part ce"(ce) is
a non-negative odd function of frequency which va-
nishes at ce
=0 and cc.
From the fluctuation-dissipation theorem (Landau
and Lifshitz, 1958), it may be deduced that the ma-
gnetic moment fluctuation spectrum is :
If the significant frequencies in the dispersive beha-
vior of (X( (0) lie below kT/~, the spectrum simplifies to
the classical form :
The total variance of the moment fluctuations inte- grates to :
Article published online by EDP Sciences and available at http://dx.doi.org/10.1051/rphysap:019700050107700
78
Now the function ce(m) is related to the response function for an abrupt change of magnetic field. If
the applied magnetic field is increased by an infini-
tesimal step 8H at t
=0 and 3m(t) is the resulting
time variation of the magnetic moment, the incre- mental response function is defined as :
This is in general a tensor but we shall only consider
cases where it is a scalar by making the coordinate
axes coincide with the principal axes of the system.
The Fourier transform relation connecting r(t) and et. ( (0) is :
The prompt and the final steady state response functions are related to ce(ce) by :
The variance of a Cartesian component of the ma- gnetic moment is thus :
where r(t) is function applicable to the component of the moment considered. This result can be further
generalized to give the autocorrelation function for the moment component :
For a normal conductor r( oo) = 0 if [J.
=1 and
r( oo) > 0 if y > 1 while for a superconductor r( oo) 0 corresponding to diamagnetic behavior.
For all systems r(0+) 0 and is simply related to
the geometry of the system.
One situation of practical interest is that of a long
solenoid enclosing the magnetic body which can be
of arbitrary shape. The magnetic moment of the body m in the direction of the solenoid axis sets up in the solenoid a flux :
where no is the number of turns per unit length of the
solenoid. This flux is independent of the dimensions of the solenoid so long as its length is large compared
with its radius.
The observable would be the EMF induced in the solenoid by variations of the magnetic moment. If
the body is in thermal equilibrium at temperature T the spectrum of the induced EMF is :
This is just (kT/03C0) times the resistance induced in the solenoid by the presence of the body, as is indeed required by the general thermodynamic validity of Nyquist’s theorem.
III. Simply-Connected System.
-III.1. SPHERE.
-
The sphere exemplifies the case of a simply-connec-
ted body with an isotropic demagnetization coefficient
so the polarizability tensor is particularly simple.
A sphere of radius a, normal conductivity a and permeability [L = 1 has polarizability :
where z
=Ka
=a(47ti(ù(j)1/2 and K is the wave
constant.
Thus oc 0
=0 and cc(oo) == - 1 a3 gives :
The low-frequency moment spectrum is :
If however the sphere is ferromagnetic with permea-
bility p,., these results become modified to :
where f ( z) = z-1 coth z
-z- 2 and now :
The limiting values are :
As expected the final steady state response :
is not zero but has the positive value appropriate to
a polarizable sphere of permeability f1. taking account
of the demagnetization effect. The variance and the low frequency spectrum of the magnetic moment are
greater than those for a non-ferromagnetic sphere :
We discuss the variance of the magnetic moment
instead of its mean square value since for a ferromagne-
tic system there may be some steady magnetization
upon which the fluctuations are superimposed. The permeability 03BC here must be interpreted at the static
differential permeability (dB/dH) taken at the value
of the steady magnetization.
Some ambiguous results can arise if the sphere
with 03BC > 1 be assumed to have zero conductivity
i.e. an ideal ferromagnet. The value of x(0) is unchanged but the evaluation of z(oo) and hence
of tl( (0) for zero conductivity is indeterminate. In this situation and others of similar character it must
be recognized that the conductivity of a real ferro- magnet may be very small but positive for eu > 0.
Thus in evaluatingf( (0) to obtain ce (0) we let m - aJ
and 03C3 ~ 0+ which again leads to the value found above for oc ( oo ) .
A further factor is that the permeability itself will
in general be a complex function of frequency due to
the inevitable inertia of the spin motion in a varying magnetic field. Thus in evaluating ce oo) it is relevant that not only is f (z) frequency dependent but so also
is [.L. These considerations are without effect if f ( 00 )
is taken as 0, yielding again the above expression for
var m even when there is dispersion of 03BC.
It is important to remember that the conductivity 03C3(03C9) is complex and bounded at high frequency. For
a normal conductor in which the electrons can be
considered to have a momentum relaxation time Tn :
where nn is the (normal) electron density. Thus as
(ù -+ oo the wave constant :
where 11n
=m/nne2.
Thus K and z do not tend to infinity in this limit,
and the corresponding characteristic length :
for a typical metal is about 2 X 10-6 cm. Thus except for very small particles we may take z(co) > 1
as m - oo and thus f( (0)
=0 as assumed above.
This limit is equally valid for a ferromagnetic con-
ductor.
If however our concern is with very small spheres
the earlier expressions for the variance of the magnetic
moment must be modified to take account of the finite value of K( oo) and becomes :
In discussing superconducting bodies we shall use
the approximation of London (London, 1961).
The results for a superconducting sphere can then be
derived from those of a normal conductor of the same
configuration by a simple procedure using the two-
fluid approach.
The wave constant K used above for steady-state periodic excitation at frequency m in a normal conduc-
tor with unity permeability is :
For a superconductor we modify this to include the contributions of both the super and normal fluids :
where 11s
=m/ns e2 with ns
=superfluid number den-
sityand À is the London penetration depth
=(As/41t)1/2.
The limiting values of the wave constant K(to) are
then :
where n = ns --+- nn and A -1
=As’ + An’.
The essential difference between the normal and
superconducting spheres is that for the latter z(O) is
not zero but 2/À.
Thus in calculating the low frequency spectrum
care is needed in approximating since z(w) is not necessarily small (as for the normal sphère). Indeed
if the radius of the sphere is large compared with the
London penetration depth :
so the low-frequency moment spectrum is :
which is smaller by the factor (45/2) (03BB/a)3 than the
low frequency moment fluctuations in the corres-
ponding normal sphere.
If a/03BB is small compared with unity we recover the
result found for the normal sphere at low frequency :
The presence of the superfluid does not therefore
manifest itselfin the magnetic fluctuations for particles
small compared with h.
Since the penetration depth 03BB increases as T in-
creases to Tc, it is seen that the fluctuation spectrum increases rapidly and steadily with temperature and joins smoothly to the value for a normal conductor
at T
=T,. This is a general inference for an arbi- trary shape of the conductor since K((ù) varies conti- nuously with temperature through T,.
The integrated spectrum of the moment fluctuations in a superconducting sphere also has two limiting
forms depending on whether the radius is large or
small compared with À.
For a » h the moment variance is smaller by the
factor 3(h - h’) la compared with the same sphere
in the normal state :
where 03BB’
_(A/4n) . For a ~ 03BB’ :
which is determined by the normal fluid and corres-
ponds to the result for the normal sphere with p.
=1.
It is a general result that for superconducting bodies
with dimensions small compared with À the relevant electron density is that of the normal fluid in deter-
mining the magnetic moment fluctuations.
III.2. LoVG CYLINDER.
-A long cylinder of a
normal conductor with unity permeability has pola- rizability in the axial direction given by :
where a is the radius and 1 the length of the cylinder
and z
=a( 4ni(j(ù) 1/2 as for the sphere.
Thus (x(0)=0 and oc ( oo) _ - a2 lj4 for the cylinder radius large compared with the skin depth :
The low frequency spectrum of the moment fluc- tuations is :
If the cylinder is ferromagnetic the polarizability
becomes :
where the first term represents the induced magnetiza-
tion and the second term the diamagnetic effect of the
eddy currents.
The variance and low frequency spectrum are now :
where fL === fL’ - ifL".
If the cylinder is superconducting we make the same
modification to the wave constant K as we did for the sphere. For a » h the variance of the magnetic
moment is :
80
which is 2 (h
-À’) la times the variance for the cylinder
in the normal state whereas for a radius small compared
with the London penetration depth :
A generalization of the moment variance for a solid
superconducting body of arbitrary shape and having
all dimensions large compared with X is :
where S. is the surface area of the body and D is the demagnetization coefficient in the direction of the observed component of the moment (e. g. for a cylin-
der D
=0, for a sphere D
=1/3).
III .3. MEDIUM COMPOSED OF A LATTICE OF MAGNE-
TIC PARTICLES.
-Here we consider a medium with
macroscopic polarizable particles distributed in a cubic array and for simplicity of isotropy we consider the
particles to be spherical. The magnitude and orien-
tation of the particle moment is determined by the
local field.
The relation between the local field H1 and magne- tization M assumed to be given by the Lorentz relation :
where Ho is the external field.
If 03B11(03C9) is the polarizability of each particle and
n is the particle density :
A long cylindrical sample of the medium (of vo-
lume V) thus has polarizability :
Hence if the particles have static differential per-
meability lL :
where F
==4na3/3 is the particle filling factor.
The variance of the axial magnetic moment of the cylinder is : -.
For a given filling factor F the variance increases
by the factor 3/ (1 - F) as p. goes from 1 to cc. It may be inferred that the filling factor is of more
significance than the particle permeability in deter- mining the fluctuations.
IV. Ring or Hollow Cylinder.
-IV.1. NORMAL
CONDUCTOR. - The elementary multiply-connected
systems of interest are the planar loop and the long
hollow cylinder. In both cases the magnetic pro-
perties are simple if the thickness of the conductor is small compared with the other dimensions and the field penetration depth.
We first consider a planar loop of normal conductor with impedance Z(co) and area A. Then the pola- rizability in the direction normal to the plane of the loop is :
The fluctuation spectra of the loop flux (D is :
where L is the inductance of the loop.
We shall express the results for hollow systems in
terms of the flux spectrum since this would usually be
the observable of most direct interest.
Now the impedance is composed of the magnetic
and the electron contributions :
where Ln
=(mlnn e2) (piS) and Rn = Ln/Tn while p
and S are the perimeter and cross-sectional area of the loop conductor. Provided that this representation
is valid up to frequencies of the order of Rn/L so that
skin effect and radiation impedance are not important
the fluctuation of the flux is :
and the-mean total energy is :
’
,
which signifies that the magnetic energy and the electron kinetic energy (which both depend on 12) together correspond to one degree of freedom in formulating the equipartition result.
In practice Ln will customarily be very small com-
pared with L. Thus for a circular loop of radius a
and circular cross-section radius b :
which will be negligible for a metallic loop unless b
is less than about 10-6 cm.
The long thin hollow cylinder is very similar to the
loop for equilibrium fluctuation properties. The flux
fluctuation spectrum is still (kTL2j1t) Re (11Z) where
Z is now the impedance for a current sheet with peri- meter p = 2a and S = 1 d :
where a is the radius of the cylinder, l its length and
d the wall thickness which is assumed to be small.
Accordingly the mean square flux fluctuation is
k TL2/ (L + L.) as for the loop. The ratio LJL of
kinetic to magnetic inductance is :
If this is small compared with unity the mean square axial magnetic field at any point within the hollow
region is given by : -.
which is the value corresponding to equating the ave-
rage field energy to (1/2)kT.
IV. 2. SUPERCONDUCTOR.
-For a superconducting loop or hollow cylinder the impedance Z(cù) can be
written in the first approximation for the two-fluid model :
where Lg
=(mlns e2) (piS) is the effective inductance associated with the kinetic energy of the superfluid component while Rn
=L.1-r. is the resistance asso-
ciated with the normal fluid. Here Tn is the momen-
tum relaxation time of the normal electrons.
The spectrum and variance of the flux fluctuations
are :
where Q
=L(LS + Ln) + Ls Ln.
It is seen that the flux fluctuation for a given loop
or hollow cylinder is much smaller in the superconduc- ting state than in the normal state if L is large compared
with L, and Ln. Then for the superconducting loop :
Nevertheless it must be stressed that the fluctuations do not undergo a discontinuous change at the tran-
sition temperature, since as this temperature is approa- ched from below n, tends to zero, Ls tends to infinity
and (D2 uniformly tends to the value kTL2/(L + Ln)
for the normal state.
The reason for the large decrease of D2 below Tc is
that the kinetic energy terms (1/2)Ln I2n and (1/2)Ls I2s
for the normal and superfluids considerably exceed
the magnetic term ( 1 /2) L12
=03A62/2L. From the two-
fluid model it is readily found that the energy ratios
are :
and :
The field fluctuations inside a hollow superconduc- ting cylinder thus decrease rapidly as the temperature is reduced; for instance in going from t
==0.9 to
t
==0.5 the RMS field is reduced approximately
sevenfold (t
=T/Tc).
It should be remarked that the equations derived
here incorporate the conservation and quantization
of fluxoid in the form (D + L, I,
=const.
=Nhl2e.
Quantization is not however relevant in the discussion of fluctuations unless one is concerned with transitions from one fluxoid state to another but this topic lies
outside the scope of the present paper.
IV. 3. SUPERCONDUCTING LOOP WITH JOSEPHSON JUNCTION.
-Since this problem has been discussed earlier (Burgess, 1967, 1968), it will be outlined here and the essential results presented. The Josephson junction can be conveniently represented as a parallel
combination of its capacitance C, the conductance G due to dielectric loss and quasi-particle tunneling and
thé effective inductance Li
=n/2eI1 representing the Josephson relations between voltage, phase cp and the
junction current 7j whose maximum or critical value is 11.
The conservation and quantization conditions are :
where IJ is the Josephson tunneling current in the junction. If the system is in thermal equilibrium the
fluctuation sources are given by the Nyquist relation applied to the Rn of the normal fluid in the super-
conductor and to the conductance G of the junction.
The spectral density of the flux fluctuations is then :
The mean square flux fluctuation is thence :
which is always greater than the flux fluctuation in the superconducting loop without a junction.
If L is large compared with Zg and Ln this simplifies
to :
If the junction conductance G is not too great the system can be approximated by the loop inductance L connected to the junction reactance composed of C
and L J in parallel. Then the fluctuation spectrum of the current has its maximum at the frequency :
and has its minimum at the (slightly) lower frequency equal to Josephson’s "plasma frequency" :
Thus the spectrum has its most conspicuous features
of a minimum at 0153j and a maximum at 03C9J(1 -p LJIL) 1/2
in a relatively narrow range of frequency.
For an extremely weak junction with very small Il
such that Li exceeded L the flux fluctuations approach
the value for a superconducting loop with a resistive junction discussed in the next section. If the Josephson junction is not too weak so that L is large compared
with Li we must revert to the unapproximated (D2
where we see that Lj, Ls and Ln are competing for
control of the current fluctuations which are then very much smaller than kT/L.
IV.4. SUPERCONDUCTING LOOP WITH RESISTIVE
JUNCTION.
-If a superconducting loop is interrupted by a junction (e. g. of dielectric or normal metal)
which cannot support a supercurrent the current fluctuations are markedly enhanced.
First we consider a narrow resistive region of resis-
tance R which is too wide however to permit tunneling
of a supercurrent. In this case we do not invoke the
Josephson conditions and no quantization condition
for flux and junction phase is applicable. The system behaves like a simply-connected superconductor to
which the potential difference
-IR is applied. The
two-fluid model is used for the superconductor to treat
time varying currents. There are two fluctuation
sources
-the resistance Rn associated with the normal
82
fluid in the superconductor and the R of the resistive
junction.
In terms of the notation used previously :
This spectrum as well as the response of the system
to an abrupt change of external magnetic field corres- ponds to two relaxation times 03C41 and T2 whose recipro-
cals are the roots 81 and S2 of the quadratic equation : S2 Q - 8[Rn(L + LS) + R(Ln + Ls)] + RRn
=0.
These relaxation times will be approximately (L + Ls) IR and (Ln + Ls) I Rn if Ls is small compared
with L or Ln that is for temperatures not too close to Tc.
On the other hand the superconducting loop without
a junction has a single relaxation time :
which is much smaller than the value (Ln + L)/Rn
for the normal loop but always larger than in
=Ln/Rn.
The relaxation time is continuous at T,.
The flux fluctuation is :
which is very close to that for the normal loop. Thus
when only a very small segment of a superconducting loop is resistive the flux fluctuations are greatly enhan-
ced over the value for a completely superconducting loop and approach the limiting value kTL2J(L + Ln) .
No discontinuity occurs in the flux fluctuations when the temperature is taken through Tc because :
is a constant and is equal to the value of Ln when the loop is in the normal state.
The results for the loop presented above show that there is a steady increase in the flux fluctuations pro-
ceeding in the sequence : superconducting loop
~
superconducting loop with Josephson junction
~