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Investigation of the role of
10
Li resonances in the halo
structure of
11
Li through the
11
Li(p, d)
10
Li transfer
reaction
A. Sanetullaev, R. Kanungo, J. Tanaka, M. Alcorta, C. Andreoiu, P. Bender,
A.A. Chen, G. Christian, B. Davids, J. Fallis, et al.
To cite this version:
A. Sanetullaev, R. Kanungo, J. Tanaka, M. Alcorta, C. Andreoiu, et al.. Investigation of the role
of
10Li resonances in the halo structure of
11Li through the
11Li(p, d)
10Li transfer reaction. Physics
Contents lists available atScienceDirect
Physics
Letters
B
www.elsevier.com/locate/physletb
Investigation
of
the
role
of
10
Li resonances
in
the
halo
structure
of
11
Li
through
the
11
Li
(
p
,
d
)
10
Li transfer
reaction
A. Sanetullaev
a,
b,
1,
R. Kanungo
a,
∗
,
J. Tanaka
c,
M. Alcorta
b,
C. Andreoiu
d,
P. Bender
b,
A.A. Chen
e,
G. Christian
b,
B. Davids
b,
J. Fallis
b,
J.P. Fortin
a,
f,
N. Galinski
b,
A.T. Gallant
b,
P.E. Garrett
g,
G. Hackman
b,
B. Hadinia
g,
S. Ishimoto
h,
M. Keefe
a,
R. Krücken
b,
i,
J. Lighthall
b,
E. McNeice
e,
D. Miller
b,
J. Purcell
a,
J.S. Randhawa
a,
T. Roger
j,
A. Rojas
b,
H. Savajols
j,
A. Shotter
k,
I. Tanihata
c,
l,
I.J. Thompson
m,
C. Unsworth
b,
P. Voss
d,
Z. Wang
b,
daAstronomyandPhysicsDepartment,SaintMary’sUniversity,Halifax,NSB3H3C3,Canada bTRIUMF,Vancouver,BCV6T2A3,Canada
c
RCNP,OsakaUniversity,Mihogaoka,Ibaraki,Osaka5670047,Japan
dDepartmentofChemistry,SimonFraserUniversity,Burnaby,BCV5A1S6,Canada eDepartmentofPhysicsandAstronomy,McMasterUniversity,Hamilton,ONL8S4M1,Canada fDepartmentofPhysics,UniversityofLaval,QuebecCity,QBG1V0A8,Canada
gDepartmentofPhysics,UniversityofGuelph,Guelph,ONN1G2W1,Canada hHighEnergyAcceleratorResearchOrganization(KEK),Ibaraki305-0801,Japan
iDepartmentofPhysicsandAstronomy,UniversityofBritishColumbia,Vancouver,BCV6T1Z1,Canada jGrandAccélérateurNationald’IonsLourds,CEA/DSM-CNRS/IN2P3,B.P.55027,F-14076CaenCedex5,France kUniversityofEdinburgh,Edinburgh,UnitedKingdom
lSchoolofPhysicsandNuclearEnergyEngineeringandIRCNPC,BeihangUniversity,Beijing100191,China mLawrenceLivermoreNationalLaboratory,L-414,Livermore,CA 94551,USA
a
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t
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c
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a
b
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Articlehistory:
Received28December2015
Receivedinrevisedform25February2016 Accepted25February2016
Availableonline2March2016 Editor:D.F.Geesaman Keywords: Halonucleus 10,11Li Transferreaction Inversekinematics DWBA Spectroscopicfactor
Thefirstmeasurementoftheone-neutrontransferreaction11Li(p,d)10LiperformedusingtheIRISfacility atTRIUMFwitha5.7 A MeV11LibeaminteractingwithasolidH
2targetisreported. The10Liresidue
was populated strongly as aresonance peakwithenergy Er=0.62±0.04 MeV havingatotalwidth
=0.33±0.07 MeV.Theangulardistributionofthisresonanceischaracterizedbyneutronoccupying the1p1/2orbital.ADWBAanalysisyieldsaspectroscopicfactorof0.67±0.12 forp1/2removalstrength
fromthegroundstateof11Litotheregionofthepeak.
©2016TheAuthors.PublishedbyElsevierB.V.ThisisanopenaccessarticleundertheCCBYlicense (http://creativecommons.org/licenses/by/4.0/).FundedbySCOAP3.
Thenuclear halo,discovered three decadesback [1,2], contin-uesto be an intriguing object of study posinga great challenge tounderstandfromfirstprinciples.Particularlyunusualstructures arethe Borromean neutronhalo nuclei, whichare weakly bound states of three components, a core nucleus plus two neutrons
*
Correspondingauthor.E-mailaddress:ritu@triumf.ca(R. Kanungo).
1 Presentaddress:InhaUniversityinTashkent,Tashkent,Uzbekistan.
[1,2]. Here anytwo sub-components taken together are neutron-unbound. Borromean two-neutron halos have been identified in 6He, 11Li, 14Be, 17,19B [3]and22C [4].The challengeto achievea completeunderstandingoftheBorromean halorelatestothe cur-rent limited knowledge on the structure and interactions of the pair-wisesub-components.Whilethesub-componentsareneutron unbound,someofthemcanexistasresonances,suchasthe core-neutronsystems,10Li,13Be,16,18B and21C.
The wavefunctionof11Licanbe expressedby a superposition ofdifferent resonancestatesof10Liplus a neutronthat occupies
http://dx.doi.org/10.1016/j.physletb.2016.02.060
482 A. Sanetullaev et al. / Physics Letters B 755 (2016) 481–485
therelevantmatchingorbital,intotalgivingthe11Ligroundstatea spinof3
/
2−.Inordertounderstandthedominating10Listatethat constitutesthegroundstate of 11Li, we reportthe first measure-mentofaone-neutronpickupreaction11Li(p,d)10Li,thattransfers neutronfrom11Lipopulatingthestatesin10Li.Theunboundstatesof10Lihavebeenexploredthroughvarious techniques,butmostofthesedonotrelatetothewavefunctionof 11Li. 10Liisjustbeyondthedrip-lineofthe N
=
7 isotones where it is known that the intruder 2s1/2 orbital maybe energetically lower than the 1p1/2 orbital causing a breakdown of the N=
8 shell closure. The first observation of a 10Li identified through the 9Be(9Be,8B)10Li reaction [5], found a peak at resonance en-ergy Er=
0.
80±
0.
25 MeV;=
1.
2±
0.
3 MeV (=
full width at half maximum). Thiswas later understood not to be the ground state.A subsequentstudythroughthe11B(π
−,9Li+
n)preaction[6] showeda broadstructure at Er=
0.
15±
0.
15 MeV that was as-sumedtoresultfromalarges-waveamplitude.Thisassumptionis supportedby observationofan l=
0 resonanceat0.
1±
0.
1 MeV (=
0.
4±
0.
1 MeV)inthe11B(π
−,p)10Lireaction[7].A resonant state unboundto neutrondecay by atleast100 keV, andwitha possibles-waveorp-wavestructurewasidentifiedfromastudyof the11B(7Li,8B)10Lireaction[8].The presence of a neutron s-wave in the lowest state of 10Li wasfurtheraffirmedfromseveralfragmentationexperiments.The relative-velocityspectrumofthe9Li-nsystemfromfragmentation of18O was peakedatzeroindicativeofthes-wavenature[9,10], witha scatteringlength, as
<
−
20 fm[10].Momentum distribu-tionsofone protonandone-neutronremovalfrom11Be [11] and 11Li [12], respectivelywere rather narrowwhich indicates that a neutroninthe 10Ligroundstatehasa strongs-wavecomponent. The invariant mass spectrum froma 9Li-n coincidence measure-ment,following neutronremovalfrom11Li, whenanalyzed using a Breit–Wigner distribution showsthe lowest resonanceat Er=
0.
21±
0.
05 MeV;=
0.
12−+00..1005 MeV[13].Theneutronremoval re-actionssuggestthes-wavevirtualstatetohaveascatteringlength varyingintherangeas∼ −
22 to−
30 fm[14,15].Severalstudies havesuggestedthefirstexcited stateof10Lito be ap1/2 resonance.The9Li(d,p)reaction [16] exhibitsapeak at Er
∼
0.
38 MeV interpretedas this resonance.This peak is much lower in energy than that in Ref. [5]. 10Be(12C, 12N)10Li is the onlyothermeasurement[17]whichshowedanevenlowerenergy peakat0.
24±
0.
04 MeV togetherwithapeakat0.
53±
0.
06 MeV which are both l=
1 resonances. The latter resonance energy seemsconsistentwiththeobservationfromthe 9Be(9Be,8B) reac-tionreportinganl=
1 resonanceat0.
50±
0.
06 MeV[18],butnot consistentwiththe 0.8 MeVstate inRef. [5].Theresonances ob-servedat0.
54±
0.
06 MeV inthe 11B(7Li,8B)10Lireaction [8],and at0.
7±
0.
2 MeV inthe11B(π
−,p)reaction[7],arealsoin agree-ment with the above. The two-proton removal from 12B reports threepositiveparityresonancesat0.
1±
0.
04 MeV,0.
5±
0.
1 MeV and1.
1±
0.
1 MeV[19].The decayspectrumisdominatedbythe 0.
5±
0.
1 MeV resonanceexhibitingapeakbuttheothertwo com-ponentswererequiredinordertofittherisingandtrailingedges ofthe spectrum.Recently, stoppedπ
− absorption reactions with 14C target reported peaks for 10Liat Er
=
0.
70±
0.
05 MeV and 0.
78±
0.
15 MeV[20].Whileall ofthe abovementioned reactions canprobethe ex-cited resonance spectrum of 10Li, they do not convey informa-tionontheroleoftheseresonances inthegroundstatestructure of 11Li. This can be investigated via neutron removal orneutron transferreactionsfrom11Li.Severalneutronremovalreactions ex-hibitedpeaksatEr
=
0.
61±
0.
10 MeV[13],0.
68±
0.
10 MeV[23], 0.
510±
0.
044 MeV [15] and 0.
566±
0.
014 MeV [14]. The reso-nanceenergieswere obtainedfromBreit–Wigner fitsofthe9Li-n decayenergyspectra,withasumofcontributionsfromresonancesFig. 1. (a)Aschematiclayoutoftheexperiment.Theparticleidentificationusingthe (b)YY1-CsI(Tl)array(c)S3E−E array.
whose widthsdepend on thedecay energyandangular momen-tum.Thisledtoanunderstandingofthel
=
1 natureofthepeak whilethelowerenergyspectrumshowsastrongandnarrow con-tributionfromthel=
0 virtualstate.Thesemeasurementshowever donotprovideanyinformationonthespectroscopicfactorthatis necessarytodefinethegroundstateof11Li.A neutrontransfer re-actionisadecisivewaytoascertainboththeangularmomentum andthe spectroscopicstrengthfromthemeasured angular distri-bution. The mainmotivation ofthe investigationreported inthis articleis tostudytheneutronpickup reaction 11Li(p,d)10Li, since nosuchstudyhasyetbeenperformed.The first measurement of this one-neutron transfer from 11Li using the IRISfacility [21] atTRIUMF, Canada isreported inthis letter.The11Libeamwithanaverageintensityof2800 pps, accel-erated toan energyof6 A MeV using thesuperconducting LINAC attheISACIIfacility,interactedwithasolid H2 targetatIRIS.The beamintensitywasdeterminedusingalow-pressure transmission-type ionizationchamber operatedwithisobutanegasat19.5 Torr placedbefore theH2 target.Theenergy-lossspectrum ofthe ion-izationchamberalsorevealedthattherewerenoisobaric contam-inantsinthebeam.
The solid H2 target was formed by spraying H2 gas onto a 5.4 μmthickcooledAgfoil.Thefoiladherestoacoppertargetcell framecooled to4 K.Thetargetthicknesswas measuredusingthe Ag(11Li,11Li)Ag elastic scattering peak energy of 11Li detected in theS3siliconarray.Thiswas donesimultaneously while measur-ingthe(p,d)reaction.Thedifferenceinenergyofthiselasticpeak withoutandwithH2 providesameasureofthesolidH2thickness fromtheenergylosswithinit.Itwascrucialtohaveacontinuous thicknessdeterminationbecausethetargetwasfoundtogradually evaporateafterseveralhours.A continuousthicknessmeasurement thereforeallowed usunambiguous determinationofcross section usingthethicknessmeasuredateachinstanttogetherwiththe re-spectivenumberof reactionevents.When thethickness dropped below a certain level the target was re-furbished by adding H2. The average thickness was
∼
60 μm varying from∼
30 μm to∼
130 μm with time. In order to restrict the radiative heating ofthe H2 target, the target cell is surrounded by a copper heat shieldwhichiscooled to∼
30 K.The openingoftheheat shield forthescatteredparticlesledtoanangledependentgeometric ef-ficiencyforthe Yd1-CsI(Tl)detectorarray since the shieldmasks partsofthisarray.Thisgeometricefficiencywasdeterminedby a Monte Carlosimulation.ThebackgroundreactionsfromtheAgfoil emittingdeuteronswere negligiblysmallasfoundfrom measure-ment without the H2 layer. The beam energy atmid-target was 5.
7 A MeV.Fig. 2a shows the measured energy-angle scatter plot of deuteronsbytheYY1-CsI(Tl)telescope.Forenergiesbelow4.5 MeV, the deuterons stop in the silicon layer and therefore cannot be identifiedbytheprocedurementionedabove.Thoseeventsplotted below4.5 MeVincludeallparticlesstoppedintheYY1detectorin coincidencewith9LiintheS3telescope(Fig. 2a).Inorderto min-imizethenon-resonant backgroundtheazimuthal anglebetween thedeuteronsandthe9Liwasrestrictedto180◦
±
60◦.Theregion outsidethisselectiondoesnotexhibitanyresonancepeak.Theresonanceenergyspectrum (Fig. 2b)of10Liisconstructed in the missing mass technique using the measured energy and scattering angle of the deuterons. A very prominent resonance peakis seenat Er
=
0.
62±
0.
04 MeV andfull width=
0.
33±
0.
07 MeV isobtainedfromfittingthespectrumwithaVoigt func-tionwithan energydependent Breit–Wignerfunctionwidth[22]. Theaverage(Gaussian)excitationenergyresolutionovertherange of angles used in this fit isσ
∼
0.
31 MeV based on simulation thatreproduceselasticscatteringpeak width.Theresonancepeak width extracted is consistent throughout the angular range. The resonance energy is consistent with that reported in Refs. [7,8, 14,15,17,19,23].The intrinsicwidthofthe peakis ingood agree-ment with observations from multinucleon transfer reactions [8, 17,18]andconsistentwithin large uncertainties withneutron re-movalreactions [15,14]. The widths reportedin Refs. [13,23] are muchlargerandthatinRef.[7]ismuchsmaller.The spectrum does not exhibit any other resonance peak(s) such as at Er
=
0.
24 MeV [17], 0.35 MeV [16] although they wouldbe within the detectoracceptance. A higher energy reso-nancesuch as Er∼=
1.
49 MeV discussed in [15] is also within thedetectoracceptancebutitsabsencesuggeststhatitcouldonly bea smallcomponentinthegroundstate of11Li.The remaining partofthe spectrumis estimatedwithnon-resonant background fromthethree-body phase space of11Li+
p→
d+
9Li+
n consid-eringanisotropic emissionof theproducts inthecenter-of-mass (cm) frame. The simulated shape of this non-resonant contribu-tionfoldedwiththe (Gaussian)experimental resolutionisshown by the dotted (red)curve inFig. 2b. This simulatedcontribution describes fairly well the spectrum with energy higher than the peak region. In addition, there can be background from mixing ofother particles for eventsstopping in the YY1 detectorwhichFig. 2. (a)Thecorrelationofenergyofdeuteronsasafunctionoflaboratory scat-teringangle.Theblackcurveshowsthecalculatedkinematiclocusfor10Liatthe 9Li+n threshold(i.e. for E
r=0 MeV).The regionbelow the dashed horizontal
lineareeventsthatstopintheYY1detector.(b) Theresonanceenergyspectrum reconstructedfromenergyandscatteringanglemeasuredforthe deuterons.The dottedcurveshowsthecalculated9Li+n+dthree-bodynon-resonantphasespace.
Thesolid(red)lineshowsthelinearbackgroundshapeconsideredinthecross sec-tionevaluation.ThepinkcurveisthefittothepeakusingBreit–Wignerresonance foldedwithexperimentalresolutionandthelinearbackground.(Forinterpretation ofthereferencestocolorinthisfigurelegend,thereaderisreferredtotheweb versionofthisarticle.)
were notidentifiedasdeuterons.Suchbackgroundeventsand ef-fects of the experimental resolution contribute to the spectrum extendingbelowEr
=
0 MeV.Inordertoestimatetheuncertainty duetothe assumedbackgroundprofilewe havealsoused a sec-ond method where the spectrum was fitted by a Breit–Wigner peak folded with the resolution plus a linear background shape (solid red line, Fig. 2b) around the peak region. The uncertainty inbackgrounddeterminationfromthesedifferentmethodsis20% andisincludedinthetotaluncertaintyoftheangulardistribution data. The background countsunder the resonance peak are sub-tractedinordertoget thenumberofscattereddeuterons forthe 11Li(p,d)10Li∗ reaction.The cross section data presentedbelow isfromlinearbackgroundsubtractionincludingeffectsofthe three-bodyphasespacebackgroundas20%uncertainty.
484 A. Sanetullaev et al. / Physics Letters B 755 (2016) 481–485
Table 1
Opticalpotentialparametersfor11Li+pfromafitofelasticscattering.
V0 (MeV) r0 (fm) a0 (fm) WV (MeV) rI (fm) aI (fm) WD (MeV) rD (fm) aD (fm) Vso (MeV) rso (fm) aso (fm) 95.93 1.00 1.10 15.00 0.65 0.50 11.90 0.67 1.1 10.70 0.80 0.75
Fig. 3. Theelasticscatteringangulardistributiondatafor11Li(p,p)11Li
gs.Thecurve
showsopticalmodelcalculationswiththebestfitopticalpotentialparameters. crosssection an additional20% uncertainty fromthebackground estimationisincluded.
Fig.4showstheangulardistributionforthe11Li(p,d)10Li reac-tion.ThedetectionefficiencyshownintheinsetofFig. 4isbased on simulation with the 10Li resonance decaying isotropically in its cm frame into 9Liand neutron. It includes the geometric ef-fect of the heat shield of the target as well as the coincidence efficiencyof d and9Li detectionforthe forward
θ
cm angles.The curves in Fig. 4 are DWBA calculations using FRESCO [24]. The exit channel optical potential was considered to be the same as that extracted from the 11Li(d,d) elastic scattering [25]. The sin-gleparticleformfactorshaveaneutronboundtotheprotonina Woods–Saxonpotential. The potentialis chosen to reproducethe bindingenergy,rootmeansquareradius,andD0 ofthedeuteron. TheparametersforthepotentialareV0
=
165.
54 MeV,r0=
0.
4 fm anda0=
0.
6 fm. Theseare thequantities that affectthetransfer crosssections.A Woods SaxonformfactorhasbeenusedinDWBA calculationsinRefs.[26,27].A comparisonofthisformfactorwith aReidSoftcorepotentialformfactoryields∼
5% changein spec-troscopicfactorforthe11Li(p,d)10Lireaction.11Liisdescribedasa boundstateofa10Listate+
aneutronwithaWoods–Saxon bind-ingpotentialwheretheeffectiveseparationenergyis=
0.
98 MeV. Thepotential hasarealandspin–orbitpartwithsamegeometry, r0=
1.
15 fm anda0=
0.
6 fm.Thedepthofthespin–orbitpartis Vso=
6 MeV whilethedepthoftherealpartisV0=
49.
6 MeV for a1p1/2neutron.IntheDWBAcalculations,weconsiderthreedifferent possibil-ities ofneutron configurationof 11Liforthe resonance observed. The solid (red) curve (Fig. 4) showsneutron transfer with angu-larmomentuml
=
1.Thedistributionhassameshapefortransfer fromthe1p1/2 or1p3/2 orbital.Weconsiderthisneutrontransfer tobedominatedbytransferfromthe1p1/2 forthediscussion be-low.ThisconsiderationissupportedbypredictionsfromtheTensor OptimizedShellModelframeworkthatsuggestsonly2.5% compo-nent of(
p3/2)
2 neutrons in 11Li[28].Neutron transfers fromthe 2s1/2 orbital and 1d5/2 orbital in 11Li are shown by the dotted (black) and dashed (blue) curves, respectively (Fig. 4). The data clearlydemonstratethattheresonancepeakobservedisassociated withneutron transfer from the 1p1/2 orbital. Theχ
min2 value forFig. 4. Theangulardistributiondatafor11Li(p,d)10Li
Er=0.62 MeV.Thecurvesshow
the DWBA calculations.The solid(red)curve/dashed (blue)curve/dotted (black) curverepresentsoneneutrontransferfromthe1p1/2/1d5/2/2s1/2orbital.The
in-setshowsthedetectionefficiency.
thep-orbital is
∼
0.
8 whilethoseforthed- ands-orbital are∼
4.
5 and∼
6.
7,respectivelyforthe bestfitnormalizationto thedata. The magnitude of the measured cross section compared to the DWBAcalculationprovidesthespectroscopicfactor(S)ofthis con-figuration tobe 0.
67±
0.
12 with(
dσ
/
d)
ex=
S× (
dσ
/
d)
DWBA. Here, the spectroscopic factor value refers to that of two neu-trons. Assuming that the resonance peak observed includes the complete(
1p1/2)
2 strength andhence an overlap ofthe 1+ and 2+ states of 10Li, the probability fraction of the(
1p1/2
)
2 com-ponent in the wavefunction of 11Li is S/
2=
0.
33±
0.
12, where sum of all components is unity. This is consistent with the pre-dictionsinRef.[28].Alternatively,ifthe resonancepeak observed is only one of 1+ or 2+ states of 10Li with half the p-wave strength, then the total probability fraction of the 1p1/2 compo-nent is2×
S/
2=
0.
67±
0.
12.Weconsider theformercasetobe themorelikelysituationbecausethefragmentationreactionsalso reportoneresonancepeakforthel=
1 component[14,15].In ad-dition,anequallystrongsecondresonancewellseparatedfromthe presentpeakandwithinthisexcitationenergyrangeshouldhave beenobservedinthisexperiment.If all the remaining component was only
(
2s1/2)
2, then this probability fraction would be∼
0.
67±
0.
12. Recently, 11(2)% of d-waveprobabilityhasbeenfoundinthegroundstateof11Li[29]. Therefore,considering thed-wave,thes-waveprobabilityfraction could be reduced to∼
0.
56±
0.
12. Fragmentation studies had pointedtoans-waveprobabilityfractionof0.
4±
0.
1[30].The an-gular distribution of(p,t)two-neutron transferreaction from11Li was best explained by wavefunctionmodels withs-wave proba-bility fraction in the range of 0.31–0.45 [31]. The small(
p1/2)
2 probability observedthrough the 10Liresonance andhence largethree-body model [33] finds that the B(E1) value from Coulomb dissociationis explained by a rather small s-wave probability of 25% while the charge radius was explained using a higher value of50%.Thelatterseems tobe consistentwiththeobservationin thiswork. Theoreticaldevelopmentsincludingmulti-stepreaction mechanismswouldbeusefultoinvestigateinfuture.
Insummary,thefirstmeasurementoftheone-neutrontransfer reaction11Li(p,d)10LiatE
/
A=
5.
7 MeV isreported.Theexcitation spectrumofthe10Liresidueisdominatedby astrongpopulation ofa resonance peak at Er=
0.
62±
0.
04 MeV witha width=
0.
33±
0.
07 MeV.The angulardistribution ofthisresonance ana-lyzedina one-stepDWBAframeworkconfirms ithavingan l=
1 character i.e. with the neutron occupying the 1p1/2 orbital. The measuredcrosssectionyieldsa spectroscopic factor=
0.
67±
0.
12 forthe(
1p1/2)
2 component. This defines relatively small(
p1/2)
2 fractionin11Ligs associatedwiththis10Liresonancepeak consid-eredto contain the complete
(
p1/2)
2 strength. Assuming the re-mainingprobabilityfractiontobes- andd-waves,a large(
2s1/2)
2 probabilityfraction≥
44% isdeducedforthegroundstateof11Li. Thepresentobservationwillserveasguidancefortheoretical mod-elscalculatingmoreaccuratewavefunctionsfor11Li.The authors express sincere thanks to the TRIUMF beam de-liveryteam. Thesupport fromCanada Foundation forInnovation, NSERC,NovaScotiaResearchandInnovationTrust isgratefully ac-knowledged.Thisworkissupportedbythegrant-in-aidprogramof JapaneseGovernment under the contractnumber 23224008.This workwasperformedundertheauspicesoftheU.S.Departmentof EnergybyLawrenceLivermoreNationalLaboratoryunderContract DE-AC52-07NA27344.
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