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Magnetoresistance in NiPt multilayers with perpendicular and in-plane magnetizatio

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Journal of Mignetism and F&guetic Materials 14.0-144 (1995) so3-

Magnetoresistance in Ni-Pt multilayers with and in-plane magnetization

B. Ahneida a, LB. Sousa ay * , R. Krishnan b, pi. Lassri b, A%. Porte b,

a IFIiUUP and CFUP, FaculaMe Cihcias, Uniuersialadk Porte, Pr. Gumes Teireira, 4&W Porto, Pormgd b Laboratoire Magne~dsne et Mat. Magdqw, CNRS 921195, Me&ion, France

Abstract

High resolution magnetoresistance (Ap/p) measurements were made on have shown the dominance of perpendicular spontaneous magnetization (Y) in-plane) our Ap/p results show the usual Smitt anisotropy with respect t while for thin Ni-layer (M petpendicuiar) Ap/p is always negative. In mechanisms leads to an anomalous minimum in Ap/p at Iow gelds, when Wll I.

It is known that systems like Co-Pt [l] and Fe-p1 [2]

can develop a perpendicular magnetic anisotropy, which makes them interesting for magneto-optical storage appli- cations. Previous studies on Ni,Pt,, A multilayers de- posited on silicon substrates at 200°C have shown [3] that Z-P! multilayers also exhi!it perpendicular anisotropy, for thin Ni-layers (X I 17 A!, whereas for large n the spontaneous magnetization M, is in-plane.

To investigate this problem further we performed high resoIution magnetoresistance (Ap/p) measurements onoa set of Ni,-Ptz, A samples, with x = 9, 16, 19.5 and 39 A.

The number of Ni/Pt bilayer repetitions was 20, 12, 15 and 8, respectively. They were prepared 131 by sequential evaporation in ultrahigh vacuum, with a base pressure of 5 X lCt-’ Torr. Their thickness was monitored by an in-situ quartz oscillator, calibrated with a profiometer. The sam- ples were deposited on a silicon zubstrate at 2tWC, having a 100 A Pt buffer and a 30 A Pt top layer, with the exception of the Ni,,, @, A and Ni,, &,, A which had no buffer. The magnetoresistance measurements were made from 20-300 K with the magnetic field (HI applied in the plane of the films, either parallel or perpendicular to the electrical current (I).

Our samples can be divided in three main groups:

Ni 39 APt, A with in-plane magnetization, Ni, bPt, A and Ni r6 opt, ji with perpendicular anisotropy (the second one at Iow temperatures only) and Ni ,9,5 opt, A as a transition case [3].

In the sample with thick Ni layers (X = 39 A> Ap/p is positive for H I] I and negative for H II, as shown in Fig. 1. In aII cases, magnetic saturation is easily reached

l

Corresponding author. Fax: +351-Z-319267.

with &r = loo0 Oe. This hehaviour is to observed in buM Ni, and attributed to the Smitt [4]. In this mechanism the resi

6 between the current I a,td the ma magnetoresistance A p/p = A dependence has been confirmed in

giving A = -3.92 x 10-3 and B = 10.6x 1W3, as shown in Fig. 2 for T = 1757 K.

-0.OO6 ’ i- 1

Hrl

0304-8853/95/.$09.50 8 19!J5 Elsevier Science B.V. All rights reserved

SW 0304-8853(94)01540-6

(2)

’ ’ * ’ ’

0 0.2 0.4

0.6

cm’8 0.3 I

v&es of (Apjp),, 1755 K tic energy. This could enhance the

r tbis model we could under-

get much larger. As a aI .q&disorder scattering de-

a mametoresistive behaviour

ximately zero [3] (near balance in-pkme M6 orientation), the iwr gets rncwe ~m~Iex hecause this sample

rvgd in the temperature derivatives sides of the transition point

e tbe normal Smitt with ~Ip/p> 0 for This suggests that in

-0.002 : I I-

HHI

-a.004 \. :

. .

296.7K-

-0.001 -1

27.3K -

Fig. 4. Magnetoresistance of the Nil,,5 rlPtt,, A sampIe, both fos HIlland HII.

At high temperatures (T > T * ) we systematically ob- serve a negative magnetoresistance, suggesting that & is perpendicular to the film plane in this case. This new behaviour may be due to a small change in K, near zero, altering its sign, which could be easily caused by the structural transition at T *.

At temperatures near I”, where strong competition exists between perpendicular and in-plane M,, we observe a superposition of both effects, as clearly shown by the Ap/p curve at T= 199.3 K (see Fig. 4) obtained with H parallel to the electrical current (when the Smitt mecha- nism has opposite sign to that of the perpendicular anisotropy effect). Accordingly, Ap/p first decreases with H, indicating the initial dominance of the perpendicular anisotropy effect, and then starts to increase when the Smitt mechanism takes over. Due to this interplay a mini- mum is observed in Ap/p at low fields. When H 1 Z we do not observe any competing hehaviour, since the Smitt and the perpendicular anisotropy effect both lead to Ap/p

< 0 under such arrangement.

Ackmvkdgements: One of us (B.A.) gratefully ac- knowledges a Ph.D. grant by JNICT-Junta National de Investiga$o Cientifica e Tecnol6gica from Portugal. This work bas been partially supported by STRDA/C/CEN/

522/92 and Brite-Euram, Project BREU/0153/CXm).

[l] P.F. Garcia, A.D. Meinhaldt and A. Suna, Appl. Phys. Lett. 47 (1985) 178.

[2] S. Iwata, S.S.P. Parkin, H. Nuri and T. Suzuki, Mater. Res.

Sot. Symp. Proc. 232 (1991) 85.

[3] R. Krishnan, H. Lassri, S. Prasad, M. Porte and M. Tessier, J.

Appl. Phys. 73 (1993) 6433.

[4] J. Smitt, Physica 16 (1951) 612.

ES] Y. Yafet and E.M. Gyorgy. Phys. Rev. B 38 (1988) 9145.

[6] 2. Shi, J. Phys. Condens. Matter 4 (1992) L 191.

[7] R. Allerspach, M. Stampanoni and A. Bishof, Phys. Rev. Leu.

65 (1990) 3344.

[Sl R.P. Pinto, B. Almcida, M.E. Braga, J.B. Sousa, R. Krislman,

H. Lassry and M. Tessier, 14th EPS Conference on Condensed

Matter Physics, March 28-31, Madrid (1994).

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