A NNALES DE LA FACULTÉ DES SCIENCES DE T OULOUSE
G ONZALO G ALIANO
M ARK A DRIAAN P ELETIER
Spatial localization for a general reaction- diffusion system
Annales de la faculté des sciences de Toulouse 6
esérie, tome 7, n
o3 (1998), p. 419-441
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- 419 -
Spatial Localization for
aGeneral Reaction-Diffusion System(*)
GONZALO
GALIANO(1)
and MARK ADRIAANPELETIER(2)
E-mail : mark.peletier@cwi.nl
Nous appliquons une méthode d’energie locale pour demon- trer la localisation en espace du support des solutions d’un systeme general de reaction-diffusion. Nous démontrons que la vitesse de propagation est
finie et qu’il existe des "temps de reponse"
(waiting
times ) sous des hy- potheses faibles sur la structure du systeme. Ces hypotheses admettentdes termes de reaction additifs et multiplicatifs, une dependance en temps
et en espace des coefficients ainsi qu’un terme de convection de divergence
nulle.
ABSTRACT. - We use a local energy method to study the spatial
localization of the supports of the solutions of a reaction-diffusion system with nonlinear diffusion and a general reaction term. We establish finite speed of propagation and the existence of waiting times under a set of weak assumptions on the structural form of the system. These assumptions allow for additive and multiplicative reaction terms and
space- and time-dependence of the coefficients, as well as a divergence-free
convection term.
Introduction
In the
study
of the transport of a chemicalspecies through groundwater
flow the
following
system ofequations
arises:( *) Reçu le 21 août 1996, accept£ le 5 novembre 1996
(1) Depto. Matematicas, Fac. Ciencias, Universidad de Oviedo, E-33007 Oviedo
(Spain)
E-mail : galiano@orion.ciencias.uniovi.es
(2) Centrum voor Wiskunde en Informatica, P.O. Box 94079, NL-1090 GB Amsterdam
(Netherlands)
The unknown functions u and v represent concentrations of the
species;
theformer,
insolution,
and the latter inadsorption
on the surface of the soilparticles.
The functions~, A, B,
andf
are allsupposed given.
In Section3.1 we
give
a brief derivation of theseequations.
Our interest lies in the support of solutions
(u, v)
of( 1.1 ) .
It is wellknown that solutions of the
equation
(1.2)
can exhibit a
compact (spatial) support, provided
thenonlinearity §
isdegenerate
at u = 0. Atravelling
waveanalysis
of(1.1) (cf. [7])
shows thatsolutions with
compact support
can also existwhen §
and the diffusionoperator
arenon-degenerate;
in that case the functionf
must have adegeneracy
at u = 0. Another fact that is known from the literature is that interfaces of solutions of(1.2)
can remainstationary
for shorttime,
before
starting
to move(and
neverstopping afterwards).
This is called thewaiting
timephenomenon.
In this article we wish toinvestigate
the compactsupport
andwaiting
timephenomena
of solutions of(1.1)
in ageneral
way.A number of results
concerning
finitespeed
ofpropagation
forsystems
ofequations
are known in the literature. Diaz andStakgold [5]
consideredproblem (1.1)
with a reaction term of the formf(u, v)
=g(u)h(v),
andHilhorst,
Van derHout,
and L. A. Peletier[8]
extended this to moregeneral
reaction terms. Both works consider one-dimensional autonomous situations withsimple
initial andboundary
data. Inaddition, they heavily rely
on the existence of acomparison principle.
The method that we use, often called "the energy method for free
boundary problems",
was introducedby
Antontsev[3],
rendered in amathematically rigorous
formby
Diaz and Veron[6],
and later extended andapplied by
several otherauthors, amongst
whom Bernis[4]
and Shmarev[10].
We refer to[1]
and[2]
for agood
overview of theexisting
literatureon this
point.
The method has twoprincipal
features. On onehand,
itis a local method: it operates in subsets of the domain without
taking
into account
global
information likeboundary
conditions or boundedness of the domain. On the otherhand,
it has a verygeneral setting, allowing
toconsider,
forinstance, problems
in any spacedimension, (x, t)-dependence
of the different terms of the
equations,
andanisotropy.
In addition we donot
require
acomparison principle.
It is worthnoting
that the method isessentially qualitative,
in the sense that it does notprovide,
ingeneral,
quantitative
estimates of the evolution of the support.Let us start
by giving
the definitions of theproperties
of system(1.1)
that we will prove in this article:
DEFINITION 1.1. -
(Finite speed
ofpropagation, FSP) If (u, v)
is asolution such that
u( ~ , 0)
andv(
~0)
both vanish on a ballB(xp, po),
thenthere exists an instant
to
> 0 and a continuousfunction
p :[0, t0 ]
~R, p(0)
= pp, , such thatu( ~ , t)
andv( ~ , t)
vanish almosteverywhere
inp(t)) for
all t to.DEFINITION 1.2.-
(Waiting times, WT) If (u, v)
is a solution such thatu( ~ , 0)
andv( ~ , 0)
both vanish on a ballB(xp, po)
andsatisfy
aflatness
condition in an annulus
B(xp, pl) ~ B{xp, po),
then there exists an instant t* > 0 such thatu(
~, t)
andv(
~, t)
vanish almosteverywhere
inB(xo, po)
Two remarks are due.
First,
we have notyet
defined the notion of asolution;
wepostpone
this to Section 2.2.Second,
the flatness condition that the defintion of the WTproperty
refers to isunspecified;
inpractice,
the
precise
conditiondepends
on theassumptions
that we make about thecomponents
of(1.1).
This will become clear in what follows.1.1 Statement of results
Let us state our
hypotheses.
We consider theproblem
on a domain
Q
= Qx(0 , T],
where Q is a bounded domain Solutionsto this
problem
are defined in Definition 2.1. Thefollowing hypotheses
shallhold
throughout
thisarticle,
even when not statedexplicitly:
(1)
u0, Vo E(2) 4J, A, B,
andfare Caratheodory functions;
(3) m1up+1
for all u >0,
where the function 03A6 isgiven by
(4) A~’ ~ ~ ~ ~ ~~)’ ~ >_ ~2I~~2~ ~ E ~N~
{5) ~A( ’ ~ ’ ~ ’ ~ ~) ~ _ m3I~ I ~ ~ E ~~~
(6)
B satisfies eitherB=0
or
B = w ~ ’0~(u) , (1.5)
where w E
II~~)
and div w = 0.(7) f
isLipschitz
continuous in the second variable:)/(~~~~)-/(~~~~2)t~L!~-~! ~ (1.6)
for all u, vi u2 E
1i8,
and(x, t)
EC~.
Here 0
p
1 and the numbers mi arepositive
constants. In view ofproperties
FSP and WT definedpreviously
we fix once and for allxo E S2
and po > 0 such that
Bpo - B(xo, po)
c S2 and u0 = v0 = 0 onBpo .
Inaddition,
forproperty
WT we assume that pi > po andBp~
C Q. We shalluse the
not ation " B p "
forB ( xo , p)
.We shall use the
following hypotheses
in the formulation of the different theorems:(HI)
There exists a number 0~
oo and anon-negative
function~ : ~ [0,
that~u - ~(v)) t,
u~v) >-
0for all u ~ 0, 0 ~ v , x ~ B03C1 and for all t > 0.
Herejo
> 03C10and,
ifappropriate, p
> pi . If v oo then we set~(t;)
= oo for all~ ~
6.(H2) 0 ~ f( .
, . u,0) ~
for all u >0;
(H3) ~2u~’ f ( ~ , ~ ,
, u,0)
forall u >
0.Here the
exponent
p is the same as above and the exponent y is free to be chosen in(0,1). The ki
arepositive
constants. Wheneverpossible
weshall omit the variables x, t in
expressions
of the typeA( x,
tu,’Du).
Although
at firstsight hypothesis (HI)
may seemfar-fetched,
it arises ina natural way in the derivation of the model
underlying (1.3).
InAppendix
3.1,
we thereforegive
an outline of the derivation of the model and its relation to thishypothesis.
To make clear what we shall state from
hypothesis (H2)
and(H3)
let usassume for a moment that
f (u, 0, ~ , ~ )
is apower-like
functiondepending only
on u,f(u,O)
=ug,
and that u, v ELOO(Q).
Then we can restrict ourattention to the case
0 u, v
1 for which we shall prove the FSP and WTproperties
in thefollowing
range ofparameters
p, q:Therefore,
we shall arrive at the desired resultsby
the naturalhypothesis
ofeither
strong absorption (even
withoutparabolic degeneracy
of ourPDE),
or
parabolic degeneracy
without restriction in theabsorption.
We shall now state our main results. The first one extends a known result for the
"porous
mediumequation" (1.2): if p 1, then,
under a weakcondition on
f, system (1.3)
hasproperty
FSP.Besides,
an advection termof the form
(1.5)
does notchange
thisproperty.
THEOREM A.- Let
hypothesis (Hl)
besatisfied. If
p 1 and the condition on the advective term(1.5) holds,
thenproblem (l.~l~
hasproperty
FSP.For the theorem on
waiting
times we introduce anauxiliary
function:where 1/;
isgiven by (H1).
If s > v, then is takenequal
toinfinity.
THEOREM B. - Let
hypothesis (HI)
besatisfied
and suppose that B = 0.If
p 1 thenproblem (1.3)
hasproperty
WT. Theaccompanying flatness
condition reads:
Here
,Q
isgiven by (,~.10).
It was
already
known from atravelling
waveanalysis [7]
that if the func- tionf
satisfies a certain kind ofdegeneracy,
then finitespeed
ofpropagation
can occur even for
regular (i.e., Lipschitz continuous)
nonlinearities~.
Thefollowing
theorem makes this statementprecise.
THEOREM C. - Let either
of
thefollowing
conditions besatisfied:
(H2)
with p 1 or(H~3)
with y 1. .Set ~ = p
for
and ~ = yfor (H3). Then,
(1) if
the advection condition(1.5)
issatisfied,
thenproblem (1.3)
hasthe
property FSP;
(2J if
B =0,
thenproblem (1.3)
also has theproperty
WT under theassumption of
theflatness
condition:Here
,Q
isgiven by (,~.10~ for
andby ~,~.,~5~ for (H3).
1.2 A
comparison
with the method oftravelling
wavesIn many cases results of the type of Theorem A
(finite speed
of propa-gation)
areproved by comparing
the solution withtravelling
waves. Thisallows the often detailed information that can be obtained on
travelling
waves to be transferred to
general
solutions.For this method to
apply
it is however necessary that theproblem
is autonomous,i.e.,
invariant under translations.Although
thestudy
of suchequations
andsystems
can lead to valuableinsight,
manyapplications explicitly require
results that remain valid when thisspatial
invariancecondition is relaxed. A
typical example
is the model of transport of chemical substancesthrough
a porous medium that is derived in Section 3.1. Even if the medium itself issupposed homogeneous, together
with its characteristics such as thefunctions §
andf, then
thedispersion
coefficient D willgenerally
depend
on space andtime,
because itdepends
on thedischarge
field w.Simply stated,
D is a tensor that "has the value" in the direction ofw and
03B1T|w|
in the other directions. Note that such adispersion
coefficient does notonly bring
space- andtime-dependence
into theproblem,
but alsoanisotropy.
The
price
to bepaid
for thegain
ingenerality, however,
isobvious;
forinstance,
while for thetravelling
wave solutions(necessarily
inhomogeneous media)
that were examined in[7]
a veryprecise
characterization could begiven
of the occurrence and non-occurrence of bounded supports, in thegeneral
case wejust
obtain the one-sided results of TheoremsA,
B and C.For the
travelling
wave method it is also necessary that theproblem satisfy
acomparison principle.
It is not difficult to see that if B = 0 and $is an
increasing function, system (1.1)
satisfies acomparison principle
if andonly
iff
isincreasing
in u anddecreasing
in v. Acomparison principle
is avery
important tool,
notonly
inproving
existence anduniqueness,
but alsoin
proving
finitespeed
ofpropagation (property FSP)
or its converse,by comparing
the solution withtravelling
waves.Generically,
the information about thetravelling
wavesimmediately
carries over to the fullproblem.
Therefore it is
important
to note that the conditions that we set onf
allow for
non-monotonicity. Indeed, they
could be said toimply
a form of"weak
monotonicity" :
a functionf
that isincreasing
in u anddecreasing
inv
automatically
satisfies condition(HI)
as well as therequirement f(u, 0)~0
for all u > 0which is
part
of(H2)
and(H3).
As a second
point
ofdifference,
we should note that ingeneral
atravelling
wave
comparison
method can not prove the existence ofwaiting times,
sincetravelling
wavesmostly
have non-zerospeed.
2. Main results
2.1 An outline of the method
As was mentioned in the
Introduction,
animportant
aspect of this energy method is itsapplicability
to verygeneral equations
and systems.The other side of the coin is that
proofs
tend to be very technical andobscure the
underlying
ideas. We therefore start with an introduction to themethod,
aimed atconveying philosophy
rather thanmathematically
correct statements. After this introduction we shall prove Theorems
A,
Band C in full
rigor.
We shall discuss the method
applied
to asimplified
version of(1.3) :
The result we seek is that of Theorem
A, i.e., if p 1
andf
satisfies(HI),
then
system (2.1)
hasproperty
FSP.The
key
idea is to derive anordinary
differentialinequality
from thissystem
ofpartial
differentialequations
and to concludeby
means of thestudy
of thisinequality. Following
the definition ofproperty
FSP we assume that the initial data uo and vp both vanish in the ballBpo
=B(.CQ) po).
Wemultiply
the firstequation
of(2.1) by
the solution u andintegrate by parts
on a ball
Bp
centered in xo with radius p po. We obtainBy integrating
over(0, t)
for some 0 tT,
We now define the
non-negative
functions bandE,
which represent gener- alizedenergies (whence
the term"energy method" ):
Both are
non-decreasing
with respect to p;using
it follows from the Holder
inequality
thatUsing
this in(2.3)
we find thatThe next
step
consists inusing
aninterpolation-trace inequality (see Appendix 3.3)
to derive the estimatewhere
It is
important
to remark here that K >1/2
if andonly if p
1. Thereforethe
arguments
that follow canonly
be executedif p 1,
sincethey require
that 03BA >
1/2.
This is thepoint
in thereasoning
where thedegeneracy
ofthe
nonlinearity
is essential.Applying Young’s inequality
we obtain from(2.5)
thatwhere 0 6’
p/(p+ 1)
andBy combining (2.6)
and(2.9)
we obtainwhere
Ci
andC2
collect all the different constants.In the
rigorous proofs
we shall show how to handle the second term onthe
right-hand
side in(2.11) depending
on theassumptions
onf.
For themoment we assume that it is
non-positive, allowing
us to find anordinary
differential
inequality
for the function E:which holds for all 0 p po and 0 t T. . For such
ordinary
differentialinequalities
it is not difficult to prove thefollowing lemma,
which is aspecial
case of Lemma
3.1, part
2.LEMMA. - Let v > 0 and
03B2 1,
andlet 03C8
EC([0, T) x [ 0 , 03C10])
be anon-negative function
such thatfor
almost every p E{0, pa)
andfor
all t E~0 , T ~.
. Then there exists a timet*
T and a continuousfunction
r :j 0 ,
t*~
--~ 1I8 withr(0)
= po such that~(p, t)
= 0for
all p and t such that pr(t)
.We conclude from this Lemma that in the
region
p~ r(t)
the functionE(t, p),
and therefore also the functionb(t, p),
isequal
to zero. Therefore system(2.1)
possesses property FSP.As we said
above,
this is not more than an intuitive outline of ageneral
method which can be
proved
in fullrigour. Many
steps areonly formal,
andthe treatment of the function
f
has beencompletely neglected.
In Sections2.2,
2.3 and2.4,
we shallgive
the details which are necessary to render the ideaspresented
aboverigorous.
2.2 Proof of Theorem A
Even for the
simple system (2.1)
theproof
of Theorem Agiven
above isnot
complete.
The steps that were omitted were:(1)
the definition of a solution of theproblem;
(2)
thejustification
ofequations (2.2)
and(2.4)
and estimate(2.5).
Thisdepends strongly
on the choice of the function space to which asolution
(u, v)
shouldbelong;
(3)
the treatment of the termt0B03C1 u f (u, v).
Besides,
in order tocomplete
theproof
forsystem (1.3),
we need toconsider the more
general
functions~, A, B,
andf
instead of theirsimple counterparts
in(2.1).
We shall discuss thesepoints
oneby
one.The
definition of
a solution. - This first omission iseasily
remedied.DEFINITION 2.1.- A
pair of
measurablefunctions (u, v) defined
inQ
= 52 x(0 T ~
is a weak solutionof (1.3)
with initial data(uo, vo) if
the
following
conditions aresatisfied:
(I)
u E and v EL°°(Q)s
(2)u>0 andv>0;
(3 ) at . , .
, u, E~N)
andB(
. , . , ~,vu)
Er,l(~);
~4~ limt-.o ~~’~~ ~ ., t)~
=~(uo)
andlimt-,o v~ ’ ~ t)
= vo in(5) for
any~
E C°°([
0, T ~
we haveWe
emphasize
that we leave aside allquestions
ofuniqueness,
as well asexistence under
given boundary
conditions. Thearguments
that followonly
require
the existence of a solution in the local sense of Definition 2.1.Non-zero convection. - In order to accommodate non-zero convection
(condition (1.5))
we shall use a domain ofintegration
that is not thecylinder Bp
x(0, T)
but a truncated coneKp,t
={ (x, r)
E S2 x(0, t)
:~x~ g(p, T)}
,(2.14)
where
g(p, T)
:= p-aT and a > 0 shall be fixed later. For ageneral
function~,
we introduce the notationand
similarly
for theboundary integrals.
It can
easily
be verified that thefollowing identity
holds for smoothfunctions (:
By
atruncation-regularization
scheme such as in[1]
or[6],
we can combinethis formula with
equation (2.13) (for 1/; = u)
to obtain for all 0 p po and for all 0 tT,
When p is allowed to take values in the interval
( po , p1 )
, as is necessaryfor property
WT,
theright-hand
side of(2.16)
contains the extra termB03C1 03A6(u0).
Equation (2.16)
is theequivalent
of(2.2)
forgeneral
functions~, A,
and B. . Observe thatby choosing a
=the
second term on theleft-hand side becomes
non-negative.
Remark. - The use of a cone instead of a
cylinder
has a verysimple physical interpretation.
When a = thespatial boundary
ofthe cone
(i . e . ,
moves inward with time with avelocity
that isas least as
large
as the maximumvelocity
of the flow field. Thereforethe convection term will not introduce any material from
outside
into theintegration domain;
the occurrence or non-occurrence of zero sets is then determinedby
theinterplay
between the timederivative,
the diffusion term, and the functionf,
as is the case when convection is absent.Justification of equation (2.4) and estimate It follows from
Fubini’s theorem that for u E
H1 (S2)
and po such thatBPo
CS2,
the functionis defined for almost every p E
(0, po).
Since the domain ofintegration
is acone, we now define the functions band E in the
following
way:Definition 2.1
guarantees
that theseexpressions
are well-defined. It then follows that for almost every p E(0, po),
We can then combine this with
(2.16)
to obtain,-. - . /
This
inequality
is therigorous counterpart
of(2.6)
.Handling of
the termK uf( u, v).
- Let us now consider the last termp,t
in
(2.17). Hypothesis (Bl)
ensures the existence of a functiono. By multiplying
the secondequation
in(1.3) by 9(v)
andintegrating
we findthat
for all 0 p po . Note that since
hypothesis (HI)
allows the function to assume the value oo for some valuesof s,
the twointegrals
written abovemight
both be infinite. Now we add thisinequality
to(2.17)
to obtainHypothesis (HI)
now ensures that the second term on the left-hand side isnon-negative
and the last term on theright-hand
side isnon-positive.
Thisalso ensures that both sides of the
inequality
have finite values. We are left withFrom here onwards the
proof
is the same as in the formaldiscussion,
withthe one
exception
that Lemma 3.1 should now beapplied
to a truncatedcone instead of a
cylinder.
2.3 Proof of Theorem B
Throughout
theprevious
section the variable p took valuesin [0 ,
po).
For values outside of this range,
i.e.,
for pE ~ [ po , pl ), essentially
the samearguments
hold. The main difference is that whenintegrating
over thecylinder (that is,
the passage from(2.2)
to(2.3))
the terms at t = 0 do notnecessarily
vanish. Theequivalent
ofinequality (2.18)
then readsThe first term on the
right-hand
side is handled asbefore,
and theproof
ofTheorem 1.2 is concluded
by
theapplication
of Lemma 3.1.2.4 Proof of Theorem C
The essential difference between Theorem C and the two other theorems lies in the
assumptions
on thenonlinearity f.
We shall thereforeonly
discussthis part of the total
argument.
The
following
lemma combines some technical estimations.LEMMA 2.2.- Let
f satisfy (H2)
or(H3).
Thenfor
all e > 0 and0 t
T,
.where ~7 = p
for (H2)
and r~ = yfor (H3),
andHere p takes values in
(0, po) for property
FSP and in(0, pl) for property
WT.We first continue the
proof
of Theorem C and prove this lemma after- wards.Let us first tackle the case of
property
FSP underhypothesis (H2).
Inthat case the
integral
isequal
to zeroby assumption.
Fixq = p.
Using
thenon-negativeness
of the termu f(u, 0)
stated in(H2)
weobtain from
(2.21)
Now, combining (2.17)
and(2.22)
weget
By choosing 6’
and t* smallenough,
Then
(2.23)
becomesand we conclude
by
a combination of Theorem 3.2 and Lemma3.1,
in thesame way as in the
proof
of Theorem A.For
property
WT we considercylinders Bp
x(0, t)
where p now takesvalues in
(0,/?i),
which introduces two extra terms in(2.24):
The result follows in the same way as in the
proof
of Theorem B.When we trade
hypothesis (H2)
forhypothesis (H3)
we introduce a newenergy,
Using (H3)
and(2.21), inequality (2.17)
becomesFor property FSP the last term
disappears,
and we choose 6; and t* such thatC(~, t) 1~2 /2
for all0 t
t* . .Then, applying
Theorem 3.2 with parameter y insteadof p,
we obtainwhere
K, 0
and(3
all have the same values as in(2.7), (2.8)
and(2.10)
withp
replaced by y,
andNotably, ,Q
has the valueand therefore
/3
1 if andonly if y
1.Property
WT is handledanalogously.
We conclude with the
proof
of Lemma 2.2.Multiply
the secondequation
in
(1.3) by vq-1, where q
> 1 will be fixed later.Integrating
overand
using
formula(2.15)
we obtainNow,
if we writeand use the
assumption
ofLipschitz continuity
off
in vtogether
with either(H2)
or(H3)
-depending
on which one is valid - we findand with
Young’s inequality
withexponent q
we obtainwhere:
~ for
(H2)
we set r~ = p and C =k1,
ande for
(H3)
we set ~ = 03B3 and C =k3.
By
Gronwall’s Lemma it follows that(setting C’ = (q - 1)C)
Using
this estimate on v, we estimate theintegral
ofu f (u, v)
whichappears in
(2.17). Again using
thedecomposition f (u, v)
=f (v, 0)
+~ f (u, v) - f (u, 0)~ ,
theLipschitz continuity,
andYoung’s inequality,
weobtain for any é >
0,
where we are
writing again ~
forg(p, r).
Now if we use(2.27)
with~==(~-t-l)/~we
obtainand
by rearranging
the different terms,This proves the lemma. D
3.
Appendices
3.1
Physical background
One of the
major hypotheses
that we use in this paper(hypothesis (HI))
has a
mathematically
unusual form. Wheninterpreted
inphysical
terms,however,
thishypothesis
is very natural and even arisesdirectly
in themodel derivation. We therefore feel that the reader may benefit from a brief
discussion of the
physical background
of(1.1).
Since our interest lies in thestructure,
not thedetails,
of the derivation of themodel,
we shallsimply explain
theunderlying
ideas withoutaspiring
tophysical completeness.
We are interested in the
transport
of ahydrophobic
chemicalthrough groundwater
flow. This chemical substance can be found in either of two states: dissolved in the water and adsorbed on the surface of the soilparticles.
Let C and S denote the concentration of the chemical in dissolved and adsorbedform, respectively.
It is common in thehydrological
literatureto assume
incompressibility,
div w =
0,
and conservation of mass,
(C
+ +div(Cw - D~C)
=0 ,
,(3.1)
where w is a
given discharge
field and D is a combineddispersion/diffusion
tensor. In
(3.1)
theassumption
isimplicitly present
that the chemical substanceonly
moves in dissolved state.The behaviour of the concentrations C and S is
mainly
determinedby
the choice of the interaction between them. A
typical assumption
isSt
=k f (C, S)
,(3.2)
where
f
is called the rate function and k > 0 is a rateparameter.
It is alsocommon to
distinguish
between differenttypes
ofadsorption
sites on thesurface of the soil
particles.
This leads to a formulation of the formIn
experimental practice
it is not easy to measure the rate functionf.
However,
a very naturalquantity
to measure is the set ofpairs (C, S)
suchthat
f(C, S)
= 0. If this set can berepresented
as thegraph
of a function~O,
i.e.,
then p
is called an isotherm. The curve ,S‘ = divides theS, ~’-plane
into two parts; a common
physical
observation is thatf(C, S)
0 when >~(~’) ;
(3.3)
fCC, S)
> 0 wheny(C).
In view of
(3.2)
thisproperty
can beinterpreted
asstating
that the chemicalalways
seeks anequilibrium
distribution. In some sense it therefore is astability property.
By setting
u = C and v =S, equations (3.1)
and(3.2)
form asystem
ofthe same
type
as(1.1).
In this case thefunction §
can be taken to be theidentity.
In thesequel
we shall also be interested in cases inwhich §
has anunbounded derivative in the
origin,
and we shall thereforebriefly
show howsuch a situation follows from similar
assumptions.
Consider a model that allows for two
types
ofadsorption
sites: sites oftype
1 are considered to react on the same time scale as the advectiondynamics,
while sites oftype
2 aresupposed
to react much morequickly.
We can therefore
reasonably
assume that for sites oftype
2 theequilibrium
condition
52
=cp2(C)
is satisfied at alltime,
which allows us to substitute thisexpression
into(3.1):
(C
+~P2(C)
+ +div(Cw -
= 0 .For
Si
we retain theoriginal equation
s~t
= .By setting
u = C and v =51
we now obtain a nonlinearfunction §
that -depending
on the isotherm p2 - may or may notdegenerate
at C = 0.We now return to
hypothesis (HI). Expressed
in terms of C andSl,
thishypothesis
states that:It follows from property
(3.3)
that if the isotherm pi isinvertible,
we canchoose its inverse as the
function ~
in(3.4). Generally, experimentally
determined isotherms are monotone and therefore
invertible, although
othercases have been observed.
3.2 A nonlinear
ordinary
differentialinequality
LEMMA 3.1. -
Let 03B3
> 0 and 003B2
1 .1)
Let b > 0 and let p EC([0,
03C10 +b ]
x[0, T])
be anonnegative function
such thatfor
almost every p E[0,
03C10 + b]
andfor
all t E[0, T ).
Here ~ is anonnegative
number.If
p isnon-decreasing
in botharguments,
then there exists a time 0 t* T such that p = 0 on[0, 03C10] [0 , t*].
2~
Let be the conedefined
in(~.1l~)
with p = pp and t =T,
andlet p
EC(KPO T)
be anonnegative function
such thatfor
all t E~ 0 , T ~
andfor
almost all p E~ 0 , g(po, t) ~
. Then thereexists a continuous
function
r: ( 0 , T~ ~ II8
withr(0)
= pp such thatp(p, t)
= 0for
all p and t such that pr(t)
.Proof.
- Forpart 1),
we consider anauxiliary
function z =z(p)
thatsatisfies _
Here t* > 0 is still to be chosen. It is
easily
shown that the functionsatisfies these two conditions if
In that case t* is deduced from
(3.6):
The statement of the lemma then follows from the
monotonicity of 03C6
in tand p.
Part
2)
isproved
in thefollowing
way. Fix 0 t STand suppose thatcp is
strictly positive
on~p g(po,t)].
. Remark thatby (3.5)
the function p isnon-decreasing
in p, and thereforep(p, t)
> 0implies cp( ~ t)
> 0 on~P~ 9(Po~t)~~
Then for all pNow
integrate
over(/~ g(po,t)]:
:or
equivalently,
Clearly
thisimplies
a contradiction ifSince p
is continuous on the closed set is boundedby
a constantM > 0 and as a consequence
3.3 An
interpolation-trace inequality
As there exist some
slighty
different versions ofinterpolation-trace
in-equalities,
wepresent
here that used in thepresent
work. For further refer-ence
(see ~1~, ~9~).
We denote the norm of the space ofLebesgue integrable
functions
LP(X)
on a measure space Xby I . ’ I)
°THEOREM 3.2.- Let S2 be a bounded domain in with
piecewise
smooth
boundary
F and let u E 1 p oo. Thefollowing
inequality
holds:- 441 - where
and the constant C
depends
on SZ and theexponents.
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