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Experimental Investigation of the Hydrodynamic Interactions between a Sphere and a Large Spherical
Obstacle
N. Lecoq, F. Feuillebois, R. Anthore, C. Petipas, F. Bostel
To cite this version:
N. Lecoq, F. Feuillebois, R. Anthore, C. Petipas, F. Bostel. Experimental Investigation of the Hydro-
dynamic Interactions between a Sphere and a Large Spherical Obstacle. Journal de Physique II, EDP
Sciences, 1995, 5 (2), pp.323-334. �10.1051/jp2:1995102�. �jpa-00248158�
Classification Physics Abstracts
47.90 07.60L 68.15
Experimental Investigation of the Hydrodynamic Interactions between
aSphere and
aLarge Spherical Obstacle
N.
Lecoq
(~>~,*), F. Feuillebois (~>*), R. Anthore (~>*), C.Petipas
(~>*) and F. Bostel (~>*) (~) UFR desSciences(**),
76821 Mont Saint Aignan, France(~) Laboratoire d'Adrothermique, CNRS, 4 ter route des Gardes, 92190 Meudon, France (Received 2 June 1994, received in final form 19 October 1994, accepted 24 October
1994)
Abstract. The hydrodynamic interactions between a spherical particle embedded in a very
viscous fluid and a large close spherical obstacle
are investigated experimentally. The displace-
ment of the particle is followed by laser interferometry with a 100 nm resolution. The large
obstacle is either convex, plane or concave. The experimental results for the drag coefficient on the particle
are compared to the theoretical results written as three terms expansions for small gaps, viz. the result of Cox and Brenner
(1967)
for a plane obstacle, the result of Jeffrey(1982)
and Jeffrey and Onishi
(1984)
fora convex obstacle and an extension of Cooley and O'Neill
(1969)
for a concave obstacle. Excellent agreement is found between the experimental and the theoretical results for all cases.1. Introduction
The motion of a small
particle
embedded in a viscous fluid when in theneighbourhood
of alarge
curved obstacle is of interest for variousapplications: filtration, particle
adhesion and reentrainment, etc. If smallparticles
in air orliquids
areconsidered,
theReynolds
numbers of the flow relative to theparticle
and relative to the gap between theparticle
and thelarge
obstacle may be smaller than
unity.
This system is modelledexperimentally
hereby using
rather
large (viz.
millimetersize) particles
embedded in a very viscous silicon oil.The
technique
used here is laserinterferometry.
Theexperimental
setup andprocedure
will be described in Section 2. Theapplication
ofinterferometry
to thestudy
ofhydrodynamic
interactions between a
particle
and walls in a viscous fluid has beenpresented
in apreceding
paper
by Lecoq
et al.[ii.
It was thenapplied
to thestudy
of thehydrodynamic
interactions between asphere
and acylinder
closed at both ends. Thetechnique
allows us to follow thedisplacement
of aparticle
with atypical
resolution of loo nm. Because of thispossibility,
it is(*) The authors are also members of Groupement de Recherche "Physique des Miheuz H£t£rogdnes Comple~es", CNRS.
(**) URA 808.
@ Les Editions de Physique 1995
specially adapted
to validate various theoretical results in lowReynolds
numberhydrodynamics
when
displacements
are small.The
configuration
used here consists of asphere sedimenting
in a fluid at rest towards an obstacle at rest. The gap between thesphere
and the obstacle is small ascompared
to thesphere
radius.Typical
obstacle surfaces are used:(I)
aplane; (it) spherical
surfaces with alarge radius,
viz. a convex one and a concave one.Theoretical results have been obtained in the literature for the motion of a
sphere
towardsa close
plane
and a close convex or concavespherical
obstacle on the basis of thecreeping
flowequation
of fluid motion, or Stokesequations. Expansions
of the friction factor for small gap will be used here. These results will be recalled in Section 3. Theexpansion
valid for a concaveobstacle will be extended here.
Our
experimental
results will then becompared
to the theoretical formulae in Section 4.Finally
the conclusion is in Section 5.2.
Experimental Setup
and ProcedureThe
experimental
setup is sketched inFigure
I.A
spherical particle
issedimenting
on the centerline of a closedcylindrical
cell filled up with viscous oil. Theparticle
is a steel ball manufacturedby
SNR. Its massdensity
is 7800kgm~~.
The
sphere
radius is 3.175 mm.Departure
fromsphericity
issmall, typically
less than 5 ~Jm.The surface
roughness
observed under ascanning
microscope is less than 0.5 ~Jm.The viscous fluid is silicon oil
(Rhodorsyl
47 V100000)
with kinematicviscosity
u= 0.I
m~s~~ and mass
density
pp= 978
kgm~~
at 25 °C. Silicon oil was chosen for its very small variation of viscosity with temperature. The verylarge
viscosity was chosen so that fluid inertia effects would be quitenegligible
ascompared
to viscous effects. As a matter offact, calculating
theReynolds
number based on thesphere
radius and Stokes sedimentationvelocity
of the
particle settling
in unbounded fluid at rest, we find that it is of the order of10~~.The measurement cell C is a closed
cylinder
with innerheight
40 mm and inner radius 25mm. The axis of the
cylinder
is vertical. Onecylinder
end is closedby
aplane glass
window GMr
DATA
M ~
D Lz
G
s
Li Se
M M
Fig. I Experimental setup. Li, L2' Lens; Mf: Fixed mirror; M, Mr: Mirrors; S. Beam splitter; D:
Diaphragm; G: Plane glass window; Sc: Curved surface, C: Measurement cell; P: Particle
of
optical quality
with thickness 3.00 + 0.02 mm. The other end is closedby
a curved(either
convex or
concave) surface,
that is a lens ofoptical quality (made by Newport),
with radius51.68 mm. Both outer end
planes
of the cell are madeparallel
to within a tolerance of 5 minutes of arc. This cell arrangement allows us tostudy
the motion of asphere
towards aplane
and a curved surfacesuccessively by turning
the cellupside
down.Alternatively,
thecurve surface may be used before the
plane
one; this choice does not affect the final resultsince the characteristics of the fluid do not vary
during
the experiment.First,
there is no temperature variationduring
theexperiment:
theabsorption
of laser energy is very small and the heatdissipated by
viscous stresses is small as well.Secondly,
the oil iscomposed
ofdimethyl
siloxane chains of variouslengths
so that even if somelarge
chains are brokenby
theparticle
motion, the overall distribution of chains is not much affected.Before
starting
theexperiment,
the steel ball is maintained at the upper side of the container with a magnet located outside the cell, on top of it. At thebeginning
of theexperiment,
the magnet is taken away and the ball startssettling.
Thedeparture
of the ball was found to bequite smooth,
because of the low sedimentationvelocity, especially
near the wall.A 15 mW He-Ne laser beam with
wavelength
1= 632.8 nm is focused at the center of the cell with a lens
Li
It is then dividedby
a beamsplitter
into two separate beamshaving roughly
the same power. Both beams are then deviatedby
successive reflections onto mirrorsM, following symmetrical paths.
In thepreceding
version of theexperiment [ii,
the two beamswere reflected
by
theparticle;
it was then necessary for the beams to followsymmetrical paths
withnearly equal lengths.
In the present version of theexperiment, only
one of the beams is reflectedby
theparticle
in motion. The other beam is a fixed reference one. Since this reference beam may inprinciple
have anylength,
we chose asimple
setup in which it is reflectedby
afixed
plane
mirror Mf attached to the other end of the cell. This choice allows us to switch from one setup to the other when necessary,by simply changing
the cell.Both reflected beams then follow the same
paths
in the reversedirection,
up to the separator wherethey
combine to form interferencefringes.
Theresulting
beam is extracted from theinterferometer
by
the mirrorMr.
It is thenstopped
down and focused onto the end of anoptical
fibercoupled
to aphotomultiplier.
The use of anoptical
fiber makes it easier to select the useful central part of the reflected beam.The
displacement
of theparticle
results in ashifting
of the interferencefringes
which appearas concentric clear and dark
rings. Shifting
from a dark to the next clearfringe (or conversely)
is characteristic of a
displacement
/hz of theparticle
such that~~
4n ~~~
in which n is the index of refraction of the
liquid
for thegiven wavelength
1= 632.8 nm, that is
n = 1.404 for the silicon oil. Thus the absolute resolution of the apparatus, that is the smallest
displacement
which can be measured with agood confidence,
is /hz ci loo nm.Note that in the setup used in
iii
thecylinder
was closedby plane optical
windows at both ends. Then both beams were reflectedby
theparticle
so that thesensitivity
was1/(8n)
ci50 nm that is two times smaller. The twofold increase in the
sensitivity
whenchanging
to the present setup is in a sense theprice
to pay forusing
any type of obstacle.The
signal intensity
detectedby
thephotomultiplier
varies as a function of theparticle displacement
zaccording
to thefollowing
formula1
= Io
cos
~~~ ~~)
~
(2)
where
#
is an unknown constantphase
shift whichdepends
on the various reflectionsapplied
to both beams.
This interferometric
signal
is converted into an electricsignal by
thephotomultiplier;
this apparatus manufacturedby
Hamamatsu has a bandwidth inwavelength
300 nm < 1 < 850nm. The
analog signal
is transformed into adigital
one with a converter board installed ina PC
compatible microcomputer.
Dataacquisition
programs are written in Clanguage
withsome parts in assembler
language
to increase data acquisitionfrequency.
The results in
[ii
were relative to the motion of aspherical particle along
its wholetrajectory
inside the cell. The present article is
only
concerned with theapproach
of aparticle
to a wall.Thus the data
acquisition
is started when thesphere
comes close to thewall,
at a distance of the order of 200 ~Jm from it. Thebeginning
of theacquisition
of the electricsignal
issynchronized
with the value 300 Hz of the shiftfrequency
of the interferencefringes.
Atypical signal
ispresented
inFigure
2~ Itcorresponds
to asphere approaching
a concave obstacle.5
Is
t
Fig. 2. Example of an interferometric signal for a spherical particle approaching a concave obstacle.
The beginning of the signal corresponds to a particle velocity of the order of 3 pm
Is.
The recorded
signal
is thenprocessed
in themicrocomputer
as follows. The average line is calculated first. The successive times at which thesignal
crosses this average line are then obtained. The difference between two such times is theelapsed
time interval lit for theparticle
to move a distance
/hz, Equation (I).
Theparticle velocity
is thensimply
calculated as wp = /hzlint.
Because of the small size of /hz and of the excellent precision on the measurement of time, it was found that this
simple
method is sufficient toprovide
asmoothly varying velocity.
As indicatedabove,
the dataaquisition
is started for the value 300 Hz of the shiftfrequency
of the interferencefringes;
thiscorresponds
to asphere velocity
of 67.10 ~JmIs.
The contact
position
for which theparticle velocity
vanishes isclearly
visible on thesignal
curves. it is obtained with a loo nm
precision.
This contactposition
is taken as theorigin
of the
sphere-to-wall
distances. Theexperimental
gap between theparticle
and the obstacle based on thisorigin
is then reconstructed at the end of each experiment.Thus,
apractically
continuous set ofparticle
positions and velocities can be recorded.The present setup is
adapted
tostudy
thepurely
one-dimensional motion of a spherealong
the vertical. Theverticality
of the upper beam isadjusted by forming
an autocollimation of the beam on a surface of mercury. The lower beam isadjusted by superimposing
it to theupper one. The cell is then made horizontal
by
autocollimation of the upper beam on anoptical
mirror attached to the upper side of the cell. That is, the setup isdesigned
in such a way that any horizontal motion would be quitesmall,
and if present, would beimmediately
detected: interferences with three waves would then form and the
signal
would be unusable.In the case of a concave
or a convex
wall,
the axis of symmetry has to beexactly
vertical andcross the
sphere
centreduring
its motion. Theperfect verticality
of the axis of symmetry ismade
possible by precise
construction of thecell,
as detailed above. Fora concave
wall,
thesphere
if off axis is thenmoving
towards the axis of symmetry. This observation agrees with the theoretical prediction of Falade and Brenner [2].Conversely
for a convexwall,
in the case of a badalignment,
the closer thesphere
from thewall,
thelarger
thediscrepancy.
Thesphere
is then
rapidly moving
out of the beam and the interferometricsignal
is lost. It is thus easy to ascertain theposition
of thesphere
so as to measure its verticalvelocity.
3. Theoretical Formulae for Two Close
Converging Spherical
Surfaces3.I. PROBLEM AND NOTATION.
Typical
obstacles chosen in theexperiment
are aplane
and a
spherical
surface with alarge
radius.Consider then
(Fig. 3)
asphere
with radius amoving
withvelocity
wp towards alarge spherical
obstacle at rest. Let [a2( be the radius of theparticle
and let ~=
-ala2,
Bydefinition,
a2 > 0, ~ < 0 for a convexobstacle,
and a2 < 0, ~ > 0 for a concave obstacle. Letz be the axis
along
the line of centers of thespheres.
Let ea be the gap between the surfaces of thespheres.
We assume e < I.Solving
Stokescreeping
flowequations
of fluid motion, theexpression
for thedrag
force on thesphere
is obtained as linear function of thevelocity
wp in the formFz =
-6xa~Jwp f$ (3)
The force is
along
zby
symmetry, as indicatedby
thesubscript
z.f£
is the friction coefficientrelating
the force in the z direction to the translationalvelocity
in thez direction. ~J is the
dynamic viscosity
of the fluid.3.2. PLANE OBSTACLE. An exact theoretical result for
f£
for the motion of asphere
towards a
plane
was derivedindependently by
Brenner [3] and Maude [4]using
the method ofbipolar
coordinates. A three termexpansion
of this result for small gaps(e
<I)
was laterobtained
by
Cox and Brenner [5] andindependently by Cooley
and O'Neill [6]:f£
=
loge
+0.9713(4)
Note that other terms
involving
the fluid inertia were also derivedby
Cox and Brenner [5], but these terms will beneglected
here. There is a smalldiscrepancy
between the twoquoted
papers in that Cox and Brenner obtained the more
precise
value 0.971264 for the constant term, whereasCooley
and O'Neill obtained the value 0.971280. Since the next term in theexpansion
is of orderflog
e, the difference between both values would besignificant only
ifif log
e[ < 10~~ which occurs for e < 10~~. For ,particle
with a radius of the size of a few millimeters, the gap would then be of the order of a few nanometers. Such small gaps are not considered in the presentexperiment
since thesensitivity
is loo nm. The value 0.9713 whichwe use in
Equation (4)
iscompatible
with the results of Cox and Brenner [5] andCooley
and O'Neill [6] and it is sufficient forexperimental
purposes.It is also of interest to compare
expansion (4)
to the exact result of Brenner [3] and Maude [4].As shown in [6] the two results differ
by
less than 0.3% when e= o.12763 which is above the non-dimensional gaps used in the
experiment.
Thus the expansion(4)
is sufficient for our purposesa
W~ ~~~°
a
~ - w
-
~
j j
az >o
z
z
Ca ca
Fig. 3 Notation for a spherical particle moving towards a large spherical obstacle. In the experi- ment, a = 3 175 mm, [a2( #
(a/~[
= 51.68 mm.
3.3. SPHERICAL CONVEX OBSTACLE.
Cooley
and O'Neill [6] also obtained anexpression
for the friction coefficient on a
sphere
moving towards a closespherical
obstacle at rest. Their result is in the form of a two-termexpansion
for small gaps:~~ (l
lG)2f ~5(~~ )~~~
~~~~ ~
~~~~
~~~Note that there is a
misprint
inEquation (7.12)
of [6].This result was later
generalized
for a convex obstacle of radius-a/~,
with ~ <0, by
Jeffrey
(7] who derived an expansion up to orderO(e) (his Eq. (5.9)).
For our purpose ofTable I. Vanes
of K(~).
~ 0 0.1 0.2
K(~)
0.9713 1.1378 1.504comparing
with the presentexperiments,
we retainonly
terms up to orderO(1):
~~ (l
~lG)2f ~5(~~ )~~~
~~~~ ~
~~~~
~~~The function
K(~),
obtainedby matching expansion (6)
with the exact solution for twospheres,
was tabulated
by Jeffrey
and Onishi (8]: see their Table II in which I is -~ andAL
is K.Interpolating
between these values, we obtain K= 1.0192 for the value ~
= -0.0615 used in the
experiment.
3.4. SPHERICAL CONCAVE OBSTACLE.
Expansion (5)
obtainedby Cooley
and O'Neill (6]is also valid for a
sphere
and a close concave obstacle of radiusa/~
with~ > 0.
Following
then theapproach
ofJeffrey
[7] with now ~ > 0,expansion (6)
still holds. The functionK(~)
will be obtainedby fitting expansion (6)
to the exact solution for twospheres.
From the
linearity
of Stokesequations
of fluid motion, the exact expression for the force on thesphere moving
withvelocity
wp towards the obstacle at rest is obtained as the sum of the forces for thefollowing
two cases:(I)
the force on thesphere moving
withvelocity wp/2
towards the obstaclemoving
with anequal
andopposite velocity
-wp/2;
(it)
the force on thesphere moving
withvelocity
wp/2
when the obstacle moves with the samevelocity wp/2.
As remarkedby Cooley
and O'Neill [6], this is a solidbody
motion(the
fluid is at rest in the frame
moving
withvelocity
wp/2)
so that the force on either wall is zero.The
required
force is thenFz
=-6xa~J(wp/2)Fi (7)
in which Fi is the friction coefficient for case
(I).
This coefficient is tabulatedby Cooley
and O'Neill [6] in their Table III. Thus from(3)
the exact value of the friction coefficient for asphere moving
towards a close concave obstacle is obtained asf£)ex
=
Fi/2.
The function
K(~)
is then obtainedby fitting expansion (6)
to the exact solutionf£)ex,
that is,
denoting f£)ap
the sum of the first two terms in(6),
Kl'G)
"lf$)ex lf$)ap.
18)The result is given in Table I.
By interpolating
these values, we obtain K= 1.0499 for the value ~
= 0.o615 used in the
experiment.
3.5. RELATIVE IMPORTANCE oF THE TERMS IN THE EXPANSIONS.
Rewriting expansion
(6)
for small gaps asf£
=
~~~~
+
L(~) loge
+K(~) (9)
e
the relative
significance
of these three terms ispresented
inFigure
4by plotting
/ jT
zz
, ,' , , , ,
, ,
' , ,
, ,
' ' / ,
, , ,
, / /
, , , '
' , ,
, ,
, ,
, ,
, , ,
/
/
'
a-al 0 02 0.03 0 04 0.05 0 06
Fig. 4 Plot of
II f$
showing the relative significance of the terms in expansion (9) off$,
for thethree cases of a convex surface with ~
= -0.0615
(top
threelines),
a plane(middle
threelines),
anda concave surface with ~ = 0.0615
(bottom
three lines). The solid lines represent the first term in theexpansions, the dash-dotted lines represent the first two terms and the dashed lines the three terms.
.
@j (solid line),
.
@
+L(~) log j
~(dash-dotted line),
.
ifi
+L(~) loge
+K(~) (dashed line)
~
versus the non-dimensional gap e. These
plots
areprovided
for the three cases of aplane,
aconvex surface with ~
= -0.0615 and a concave surface with ~
= 0.06.
4. Results and Discussion
Using
theexperimental velocity
wp of theparticle,
andintroducing
itsweight
andbuoyancy together
with expression(3)
for thedrag
force into Newton's law of motion, the experimental friction coefficientf$
is obtained. Theparticle inertia,
which is of the same order as the fluidinertia,
isnegligible
for the smallReynolds
numbers considered here.The
experimental
friction coefficientf£
for the motion of asphere
towards aplane
wall isrepresented
versus the non-dimensional gap e inFigure
5 as alogarithmic plot
for ea <200 ~Jm. The agreement with the theoretical
expansion (4)
is excellent. The fluctuations due1os
'
fT
zz
ioi
lUr5 lo~ lo~3 lo~~ lo'~
e
Fig 5. Logarithmic plot of the friction factor versus the non-dimensional gap for a sphere moving towards a plane wall and in a close vicinity to it; experiment and theory.
to temperature variations are
negligible.
The smalldiscrepancy
observed for the smallest gaps is the consequence of the presence of a smallroughness
on thesphere.
It can be checked that for the small e for which thediscrepancy
occurs, ea is of the order of theroughness.
It isestimated here to be 0.5 ~Jm,
equal
to the maximumroughness
0.5 ~Jm observed under thescanning microscope (Sect. 2).
Defining
the Stokes sedimentationvelocity
of theparticle
in unbounded fluid at rest as~°~~
~a~J
~~~~
the non-dimensional
particle velocity
is obtained asI
=
( (ii)
Wps
fzz
The results can be
alternatively plotted
in terms of the non-dimensionalvelocity
wp/wp~
versusthe non-dimensional gap e.
They
are shown inFigure
6.The
experimental
non-dimensionalvelocity
of thesphere moving
towards a curved obstacle is also shown inFigure
6. It iscompared
to the theoretical value obtained from(ii)
and theexpression
for the friction coefficient from Section 3.3 and Section 3A for a convex and concave obstacle,respectively.
The agreement between
experiment
andtheory
is excellent for theplane
as well as for the curved obstacles.It is seen in the
Figure
that the curvature of the obstaclestrongly
modifies thesphere velocity.
This is because the flow of
liquid
out of theregion
near the contactpoint
isresponsible
for thedrag
force; and thisliquid
flow isstrongly
affectedby
the curvature of the obstacle. When the surface is convex, the outside flow is made easier and thedrag decreases;
the reversehappens
o~os
w~/w~z
0.030.01 0.02 0.03 0.04 0.05 0.06
e
Fig. 6. Plot of the non-dimensional velocity versus the non-dimensional gap for a sphere moving
towards a convex spherical surface
(top),
a plane
(middle),
and a concave spherical surface(bottom).
The sphere is in close vicinity to the obstacle. Experiment
(circles)
and theory(solid lines).
when the surface is concave. It is also seen in the
Figure
that the case of aplane
obstacle is intermediate between the convex and concavesurfaces,
asexpected.
The influence ofthe surface curvature increases for small gaps: the relative difference between the
experimental
curves for the convex and concave obstacles is of the order of 20$lo for e ci5 x lo~~ and 25% for e ci 3 x lo~~.
Inspecting
the curves inFigure
6, one sees that theexperimental
results for the convex or the concave surface separatecontinuously
from those for theplane
surface.It is
interesting
to note that thevelocity
ratios (wp)~onvex/(wp)plane
and(wp)~on~ave/(wp)plane
are
practically
constant over the wholeexperimental
range. This can be understoodby
recast-ing expansion (6)
for a curved obstacle in thefollowing
form:f~
=
loge
+ 0 9713 + ~~loge
+O(K(~)
0713)j
(12)
~~
II
lG)~f 5 5
The first three terms in brackets are the expansion terms for the
plane equation (4).
The fourth term is small ascompared
to IIf
for small ~: for ~= o.0615 and e
= 0.06, we obtain
e
(~~
oge)
= 1.25%.
5
The fifth term in brackets in
(12)
isO(5
x10~~),
that is very small as compared to1le.
Thus it is seen that the three-termexpansion
of the friction factor for a curved(convex
orconcave)
obstacle with a
large
radius can be obtainedby multiplying
thecorresponding
expansion for theplane by
IIii ~)~.
The
region
of small gaps e < 0.01 isreplotted
in more detail inFigure
7. Theexperimental
Wp/Wp~
0.005
0.002 0.004 0.006 0.008 0.01
e
Fig. 7. Same as in Figure 6. Details of the region of small gaps e < 0.01. The lubrication law is also shown as dashed straight lines for the three cases of a convex
(~
<0),
plane(~
= 0) and concave
(~
> 0) obstacle.data can be
compared
to the lubricationlaw,
which is written~°~
=
ii ~)~e (13)
Wp~
using ill)
and the first term in(5).
InFigure
7 one can see that(13) only applies
for small non-dimensional gaps,roughly
e < 0.005, that is for asphere-tc-wall
distance less than orequal
to 15 ~Jm.
The relative
hydrodynamic
effects of the other walls of the cell arenegligible.
This can be checkedusing
the characteristic dimension R= 25 mm for the
cylinder
radius: the relative ef- fect of the lateral walls isO((a /R) /(I If)
for thelargest
value e = 0.06 used in theexperiment,
this is 0.76%.5. Conclusion
The
hydrodynamic
interactions of aspherical particle
with a close obstacle increeping
flow have been measured with laserinterferometry.
Thetypical
obstacles considered here are aplane obstacle,
a convex obstacle and a concavespherical
obstacle withlarge
radii. Theexperimental
results for the friction coefficient are in excellent agreement with the theoretical results written
as a three term
expansion
for small gaps.The interferometric
technique
iswell-adapted
to validate theoretical results for thedrag
ona
particle
obtained from thecreeping
flowequations, especially
for smalldisplacements
when other methods would not be so efficient.References
ill
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