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III. A further application of localized white-light fringes of superposition

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Submitted on 1 Jan 1950

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III. A further application of localized white-light fringes

of superposition

S. Tolansky

To cite this version:

(2)

III. A FURTHER APPLICATION OF LOCALIZED WHITE-LIGHT FRINGES OF SUPERPOSITION

By

S. TOLANSKY.

Sommaire. 2014 Les

franges de superposition localisées qui apparaissent en lumière blanche dans un dispositif à franges de Fizeau sont utilisées pour mettre en évidence de faibles inclusions et changements

d’indices dans le mica. On coupe en deux une feuille de mica argentée sur les deux faces et l’on utilise

les deux morceaux pour produire un système de franges. Une différence de marche de 2,5 A seulement

pent être détectée à l’0153il. Cette technique se recommande par sa simplicité.

LE JOURNAL DE PHYSIQUE ET LE RADIUM. I TOME

It,

JUILLET

4930,

PAGE 4:1().

Introduction. - The

principle

of

superposition

of

fringes

has been

long

in use, since in fact their

discovery

early

last

century

by

Brewster. Two

types

can be

used,

either

fringes

of

equal

incli-nation or

fringes

of

equal

thickness,

and

they

can be used either with two beams or with

multiple’

beams. The Brewster and Jamin

fringes

are

typical

two beam

arrangements

and the classical

super-position

system

of

equal

inclination

fringes

used

by

Fabry,

Perot and Buisson in the metre

deter-mination was the first use of

multiple-beams

for such

fringes.

More

recently

Sears and Barrell determined the refractive index of air with a

closely

similar

optical

arrangement.

By

far the

larger

number of studies

using

multiple-beam

fringes

of

superposition

have been made with

the

fringes

of

equal

inclination,

and

apart

from

very brief mention

by

Fabry

in his book " Les

appli-cations des

interfirences

lumineuses "

very little use of the

system

using fringes

of

equal

thickness appears to have been made.

It is the purpose of this Note to describe such an

application, highly specific

it is

true,

yet

none the

less of much interest because of its

great

power

and

simplicity.

The method is

applied

to

studying

"

invisible "

inclusions in mica sheets. The illus-trations used were taken for me

by

my

assistant,

Miss Austin.

Experimental. -

The

arrangements

are ~of

the

simplest

possible.

The mica is cleaved and silvered

on both sides

(reflectivity

go -

g5

per

cent).

The

piece

of mica is cut in

two,

and the

pieces

held

close

together,

i. e.

effectively parallel.

This is

illuminated with a

parallel

beam of white

light

from an arc or

pointolite

and

following

the mica

is a lens of focal

length

25 -~ 5o cm. On

placing

the eye at the

principal

focus localised white

light

fringes

of

superposition

are seen.

The results are

striking.

If the mica had consisted

of a

truly parallel-sided

sheet,

then one would

only

have seen a

uniformity

of illumination. But in

general,

mica sheets have minute

steps

on

them,

cleavage

steps,

and it has

already

been established that these are

integral

multiples

of . the

crystal

lattice

spacing

20

Á,

often

only

a

single

lattice

spacing (see

M. B.

I.) yet

possibly

extending

over

quite large

areas. Thus in the field of view one

sees

beautifully

tinted areas,

separated

by

cleavage

lines. Plate 5 is a

photograph

of such a

region

and

gives only

a very poor

impression

indeed of

what the eye

actually

sees, for the different

regions

have

great

purity

of colour and are also very

brightly differently

coloured,

e. g. green,

red,

blue,

etc.

~

PL 5.

It is

immediately

obvious from the

superposition

principle

that that in effect one has

white-light

multiple-beam

interference over the

path

lengths

which are the minute

differences

in thickness between the two mica

sheets,

i.e. over the

cleavage

areas. It has been shown elsewhere

by

the author

(see

M. B.

I.)

that when

using

single

parallel-sided

stepped

films

(in

the 11

crossed Fizeau

fringe

tech-nique

")

a

change

of

height

of but one

crystal

lattice

spacing

in mica can make a 5 o per cent

change

in the

intensity

of transmission.

Indeed,

it

requires

only

the

remarkably

small alteration

of

3.5 A

in

optical path

difference to

produce

a

detectable 10 per cent

change

in

intensity

of illu-mination. Thus even with a

single

double-silvered

film,

and monochromatic

light,

a

single

lattice

change

is

easily

detected

providing

one

adapts

the

angle

of

incidence to

give

correct

transmission,

as has been

already fully

discussed.

Now it is well know from the

theory

of the

(3)

437

compound Fabry-Perot

interferometer

(see Tolansky,

High

Resolution

Spectroscopy,

Methuen that

the

fringe

width of a double

interferometer,

both

identical,

is

/

times that of either alone. Hence

V2

the

sensitivity

of the

fringes

of

superposition

to small

changes

in

path

is

V 2

times as

great

as in the

case of a

single

mica film.

Furthermore,

one

always

finds a suitable colour

available,

and in

addition,

the eye is

certainly

far more sensitive to a

slight

colour-lint alteration than to a

slight

intensity

alteration.

Pl. 6.

One

recognises

therefore that the

sensitivity

of the method is such that one should be able to detect

optical

path

differences of

only

2.5

A,

i.e.

1 /2

ooo th of a green

light

wave. This

being

so, even very

slight

variations in chemical compo-sition of mica should show up.

Any

11

invisible" inclusions should be revealed with very

great

contrast if

they

have a refractive index

differing

even

slightly

from that of mica. In

plate 5

a mass of

unsuspected

secondary

inclusions appear. These cannot be seen

normally.

Plate 6 shows

typical

11

invisible "

inclusions. Two features may be remarked upon,

namely, (a)

the

fringe

sharpness, (b)

the

reproduction

is

only

in monotone and

gives

a very

inadequate

picture

of what is

actually

seen

by

the eye.

Plate 7

is another characteristic

example.

Here

one sees that the inclusions have often a small

crystalline

nucleus,

and one

notices,

too,

the

revealing

secondary

structure

surrounding

the nucleus. On other

plates

continuous variations appear in

patchy

areas,

indicating

secondary changes

in chemical

composition.

Pl. 7.

Conclusion. -- The method has

many obvious

applications

to the

study

of thick and thin films.

For

example,

if films are

put

down in a selected

piece

of mica and then

silvered,

a means for

stu-dying

film

uniformity

becomes available. This

should find

application

in

evaporated

films,

grown

films,

even

crystalline deposits

and

probably organic

monolayers.

It also becomes a means of

matching

thick

optical

specimens

for exact

equality (or equating

two

equal

Fabry-Perot interferometers),

for it is the differential

effect which leads to the

interference,

but with thick

specimens

collimation will

be.

critical. The fact that a

special

monochromatic source ’is not

needed is a considerable attraction.

The

rapidity

and

simplicity

of the

technique

has

much to commend it. White

light

sources

(arcs)

are so

bright

that one can tolerate

quite

heavy

silverings

and thus obtain maximum

sensitivity.

With thin

specimens

very crude collimation can be used with little loss in

sensitivity.

It is

re-emphasised

that the monotone

repro-ductions

given

here fail

entirely

to

give

an idea of the real

sensitivity

a colour

reproduction

reveals.

Intervention de M. 0. S. Heavens. The limit to the

sharpness

of the

fringes

of

equal

chromatic order would appear to be set

by

the statistical fluctuations in thickness of the

deposited

silver film.

This will in turn set a limit to the

magnification

which may be used between the interferometer

and the

dispersing

system.

Intervention de M. Kuhn. This beautiful method of

detecting

local

inclu-sons and variations in refractive index

is,

of course,

closely

related to the interference

microscope.

These

fringes

which are of the Brewster

type

are,

however,

entirely

different from those used in the double interferometer. In the latter

instrument,

no interference takes

place

of any two rays which

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