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Macroscopic regime transition of a non-Newtonian fluid through porous media

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Open Archive TOULOUSE Archive Ouverte (OATAO)

OATAO is an open access repository that collects the work of Toulouse researchers and makes it freely available over the web where possible.

This is an author-deposited version published in : http://oatao.univ-toulouse.fr/ Eprints ID : 14410

To cite this version : Pierre, Frédéric and Davit, Yohan and Loubens,

Romain de and Quintard, Michel Macroscopic regime transition of a

non-Newtonian fluid through porous media. (2015) In: MAMERN'15 :

The 6th International Conference on Approximation Methods and Numerical Modelling in Environment and Natural Resources, 1 June 2015 - 5 June 2015 (Pau, France). (Unpublished)

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions In

Macroscopic regime transition of a

non-Newtonian fluid through porous media

F. Pierre

1,3,∗

, Y. Davit

1,2

, R. de Loubens

3

and M.

Quintard

1,2

1Universit´e de Toulouse ; INPT, UPS ; IMFT (Institut de M´ecanique des

Fluides de Toulouse), All´ee Camille Soula, F-31400 Toulouse, France

2CNRS ; IMFT ; F-31400 Toulouse, France

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Overview

Introduction

Context

Keys concept

Rheology

Porous medium

Permeability prediction

Numerical Results

Numerical set up

Numerical results

Model

Transition’s model

Full model

Conclusions

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Introduction

Many applications fields,

composites or paper

manufacturing,

blood flow,

polymer injection,

and others.

Fig : Pressure field in Clashach sandstone

Fig : Soulis2008, blood flow through an arterial tree

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Context

µ = µ0 ⇒ hUi = −K·∇pµ 0 ⇒ hUi ∝ k∆pk ⇒ 1

µ = µβ ˙γn−1 ⇒ hUi = −K(khUik)·∇pµ0 ⇒ hUi ∝ k∆pk1/n ⇒ 2

˙

γ

c 1 2

˙

γ

µ

Fig : Non-Newtonian rheology

hU

c

i

non-Newtonian regime 2 Newtonian regime 1

?

hUi

k

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Context

Literature: ˙γ eq = α√4hUi

8k/ǫ, with fitting parameter.

Reservoir simulators: switch macroscopic law when ˙γeq = ˙γc.

Our Goal: predict and understand the transition, hU

ci.

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Rheology

Time-independent fluids, no

Bingham, Sochi2011. Common models are, ◮ plateau + power-law, µ =    µ0 if ˙γ < ˙γc, µ0  γ˙ ˙ γc n−1 else, (1) ◮ Carreau, ◮ generalized Newtonian.

Choice of plateau + power-law

(and tried others).

This leads at a macro scale to,

hUi ∝ ( k∆pk k∆pk1/n (2) 10−410−310−210−1 100 101 102 103 104 10−2 10−1 100

˙γ/ ˙γ

c

µ

0 plateau + power-law Carreau generalized Newtonian

Fig : Different rheological model

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Porous Medium

Keywords: universal, wide panel, pore to throat ratio (PTR).

1 2 2D Array name : A ǫ = 0.72 k0 = 1.1 104 ǫ = 0.75 k0 = 1.3 104 3D Stacks name : S ǫ = 0.35 k0 = 33 ǫ = 0.44 k0 = 46 3D Bentheimer name : B ǫ = 0.18 k0 = 1.92 ǫ = 0.17 k0 = 0.82 3D Clashach name : C ǫ = 0.13 k0 = 0.27 ǫ = 0.14 k0 = 0.48

Tab : Porous medium investigated (k0 in Darcy unit, for liquid)

ǫ

ց

k

0

ց

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Permeability prediction

Porous media X-ray micro-tomography Denoising & Threholding Downsampling Meshing Solver Solution REV ? (b) Resolution ? Subjectivity ? (c) and (d) Error induced ? Grid quality Schemes accuracy (a) Workflow 0 200 400 600 800 1,000 0 0.5 1 1.5

l

(µm)

ǫ

B1 B2 C1 C2 S1 S2

(b) ǫ∗ versus cube length

(c) Thresholding 1 (d) Thresholding 2

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Numerical set up

Equations: 0 =−∇p + ∇ · [ν( ˙γ)(∇U + ∇UT)], ∇ · U = 0 .

FVM with OpenFOAM.

no-slip conditions, walls.

Grid convergence study, 80 millions meshes, 80000 hours of CPU time,

use of HPC.

Fig : Slice of grid over over S1

10−4 10−3 10−2 10−1 100 10−1 100 101 102

N

10

0

×

h U i− h UN ∗= 1 i h UN ∗= 1 i S C B A

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Numerical results - Two regimes

To quantify the transition, we define an dimensionless number, N ,

N = hUi hUci . (3)

10

−10

10

−9

10

−8

10

−7

10

−6

10

−5

10

−4

10

−3

10

−2

10

−1

10

0

10

1

hU

co

i

hUi m.s

−1

k

Fig : Dimensionless permeability k∗ = k/k

0 versus hUi. Here n = 0.75 and ˙γlim = 1s−1.

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Numerical results - Varying n

Varying n: k ∝ khUik1−n is equivalent to hUi ∝ k∆pk1/n.

10−10 10−9 10−8 10−7 10−6 10−5 10−4 100 101 slope = 1 −n hUi m.s−1 k ∗ n = 0.75 n = 1.15

Fig : Dimensionless permeability k∗ = k/k0 versus hUi for the C1 case.

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Numerical results - Varying ˙

γ

c

Varying ˙γc: hUci ∝ ˙γc. This leads to, hUci = ǫ × ˙γcℓeff .

Rheology: embedded in ˙γc.Topology: embedded in ℓ eff. ◮ Use of ǫ. 10−9 10−8 10−7 10−6 10−5 10−4 10−3 100 hUi m.s−1 k ∗ ˙ γc = 100s−1 ˙ γc = 101s−1 ˙ γc = 102s−1

Fig : Dimensionless permeability k∗ = k/k0 versus hUi for the C1 case.

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Numerical results - Microscopic Phenomenology

hUi = 0.1cm.D

−1

hUi = 1cm.D

−1

hUi = 8cm.D

−1

hUi = 22cm.D

−1

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Numerical results - Microscopic Phenomenology

Identify a critical pore throat volume with PDF.

Media ǫ k0 VPT A1 0.72 1.1 104 8 A2 0.75 1.3 104 11 S1 0.35 33 2.9 S2 0.44 46 5.2 B1 0.18 1.92 1.8 B2 0.17 0.82 1.6 C1 0.13 0.27 0.4 C2 0.14 0.48 0.5

Tab : Medium description ( k0 in Darcy

unit, and VPT in % of volume)

0 0.2 0.4 0.6 0.8 1 10−7 10−6 10−5 10−4 10−3 10−2 10−1 100 ˙γc∗ % VPT ˙γ∗ P D F

Fig : PDF of ˙γ∗ at N = 1 for media C1.

Legend : for ˙γc = 100s−1, for ˙γc = 101s−1,

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Transition’s model

Our goal: predict hU

ci = ǫ × ˙γcℓeff.

Equivalent to: predict ℓ

eff.

Validation by comparison between hU

ci and hUcoi.

Medel for ℓeff :

Use ofk

0. For Newtonian fluids, √k0 is a pure topological parameter

(even if PDE are needed). We have tried: p8k0/ǫ, p32k0/ǫ, pk0/ǫ,

√ k0.

Use of Kozeny-Carman formulation and equivalent diameter,

DuPlessis1994,Kozeny1927,Sadowski1963.

Use of volume or surface of the medium (Vpart, V

medium, Spart),

Li2011,Ozahi2008.

Best results using simply ℓeff = √k0. Leading to:

hUci = ǫ × ˙γc

p

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Full model

10−1010−910−810−710−610−510−410−310−210−1 100 101 hUcoi hUi m.s−1 k ∗

Fig : Dimensionless permeability k∗ = k/k

0 versus hUi. Here n = 0.75 and ˙γlim = 1s−1.

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Full model

Relevant dimensionless non-Newtonian number, N = hUi

hUci =

hUi ǫ× ˙γc√k0.

Proof of model validation.

Analytical model, hUi = −K ∗ · ∇p µ0 , K∗ = (1− f (N ))K0 + f (N )K(khUik). (5) 10−4 10−2 100 102 104 0 0.5 1 f( N ) 10−2 10−1 100 101 102 103 100 101 N k ∗

Fig : k∗ versus N . A1, A2,

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

Conclusions & Applications

Studying the transition of a non-Newtonian fluid through porous media.

Model this transition using rheological and topological parameters, ˙γ

c

and ℓeff.

Definition of a dimensionless non-Newtonian number N , which

characterizes the regime. Many applications can be seen,

Regime verification in core-flood experiments,

Estimation of critical distances characterizing the regime transition in

petroleum and environmental engineering.

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions This work was performed using HPC resources from CALMIP (Grant 2015-11).

This work was supported by Total.

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fluids through porous media F.Pierre Introduction Context Keys concept Rheology Porous medium Permeability prediction Numerical Results Numerical set up Numerical results Model Transition’s model Full model Conclusions

References

Figure

Fig : Non-Newtonian rheology
Fig : Predict hU c i ⇒ R c ?
Fig : Permeability prediction issues
Fig : Slice of grid over over S1
+7

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