• Aucun résultat trouvé

This study was designed to investigate the vertical and lateral sedimentation dynamics in-fluencing Vidy Bay, Lake Geneva. The goal was to ascertain the sedimentation pathways of particle-bound contaminants and identify if sediment focusing was occurring in the bay.

The radionuclidic and sedimentological aspects of settling particles were used to describe the sedimentation process and discriminate between vertical and lateral fluxes. The vertical sedimentation model, with a lateral component, used 7Be/210Pbxs flux ratios to differen-tiate between and quantify vertical and lateral particle advections. The modelled results were in line with literature values while lending to more refined process-related and overall residence times. The model showed that process-related residence times τP and τC were the controlling factors in the overall residence time on a seasonal scale, while the process-related residence timeτBandτC were noted to be the controlling factors on an annual scale.

Sedimentological and radionuclidic aspects of settling particles evidenced that sediment fo-cusing was occurring in Vidy Bay. Sediment fofo-cusing increased with proximity to shore and was also most prominent during thermally unstratified conditions.

78

3.8 Acknowledgements

3.8 Acknowledgements

The authors are thankful and acknowledge the financial support of the Swiss Science Foun-dation (Project: PDFMP 2-123 034). They would also like to thank Damien Bouffard for his help in improving the flow of the article and thank Philippe Arpagaus for his vital assis-tance in sampling. Thanks are also extended to the fishing authority of the Canton of Vaud, Switzerland for their helpfulness in addressing potential issues in sampling.

References

Arnold, J. R. (1998). Radionuclides produced by cosmic rays: the early years. Planetary and Space Science 47 (1), 293–297.

Assainissement Lausanne (2009). Plan General d’Evacuation des Eaux Lausann. Tech. rep.

Lausanne.

Blais, J. M., Kalff, J. (1995). The influence of lake morphometry on sediment focusing.

Limnology and Oceanography 40 (3), 582–588.

Bloesch, J. (1996). Towards a new generation of sediment traps and a better measure-ment/understanding of settling particle flux in lakes and oceans: a hydrodynamical pro-tocol. Aquatic Sciences 58 (4), 283–296.

Bloesch, J., Uehlinger, U. (1986). Horizontal sedimentation differences in a eutrophic Swiss lake. Limnology and Oceanography, 1094–1109.

Bohle-Carbonell, M. (1986). Currents in Lake Geneva. Limnology and Oceanography, 1255–

1266.

Bonvin, F., Rutler, R., Chèvre, N., Halder, J., Kohn, T. (2011). Spatial and Temporal Pres-ence of a Wastewater-Derived Micropollutant Plume in Lake Geneva. Environmental Science & Technology 45 (11), 4702–4709.

Bouffard, D., Lemmin, U. (2013). Kelvin waves in Lake Geneva. Journal of Great Lakes Research 39 (4), 637–645.

Burton, G. A. (1992). Assessing Contaminated Aquatic Sediments. Environmental Science

& Technology 26 (10), 1862–1862.

Discrimination Between Vertical and Lateral Sedimentation Pathways in a Contaminated Bay

Dominik, J., Burrus, D., Vernet, J.-P. (1987). Transport of the environmental radionuclides in an alpine watershed. Earth and Planetary Science Letters.

Dominik, J., Dulinski, M., Span, D., Hofmann, A., Favarger, P.-Y., Vernet, J.-P. (1993).

Transfert de matiere et de radio-isotopes entre l’eau et les sediments dans le Leman.

Tech. rep. Comm. Int. Prot. Eaux Léman Contre Pollut.

Dominik, J., Schuler, C., Santschi, P. H. (1989). Residence times of234Th and7Be in Lake Geneva. Earth and Planetary Science Letters 93 (3-4), 345–358.

Drexler, T. M., Nittrouer, C. A. (2008). Stratigraphic signatures due to flood deposition near the Rhône River: Gulf of Lions, northwest Mediterranean Sea. Continental Shelf Research 28 (15), 1877–1894.

Dulinski, M., Dominik, J. (1992). Density corrections in gamma spectrometry of lake sed-iments. Nuclear Geophysics: International Journal of Radiation Applications & Instru-mentation Part E 6 (2), 237–242.

Fer, I., Lemmin, U., Thorpe, S. A. (2002a). Contribution of entrainment and vertical plumes to the winter cascading of cold shelf waters in a deep lake. Limnology and Oceanogra-phy, 576–580.

Fer, I., Lemmin, U., Thorpe, S. A. (2002b). Observations of mixing near the sides of a deep lake in winter. Limnology and Oceanography 47 (2), 535–544.

Fitzgerald, S. A., Klump, J. V., Swarzenski, P. W., Mackenzie, R. A., Richards, K. D. (2001).

Beryllium-7 as a Tracer of Short-Term Sediment Deposition and Resuspension in the Fox River, Wisconsin. Environmental Science & Technology 35 (2), 300–305.

Froehlich, K. (2009). Environmental radionuclides: tracers and timers of terrestrial pro-cesses. Vol. 16. Amsterdam: Elsevier.

Gandais, V. (1989). Origines et variations spatio-temporelles des flux de matière particulaire au centre du Léman. Doctoral dissertation. Genève: University of Geneva, Institute F.-A.

Forel.

Gandais, V., Vernet, J.-P. (1987). Determination des Flux de Nutriments Sous Forme Partic-ulaire dans le Leman a l’aide de Trappes a Sediments. Tech. rep. Comm. Int. Prot. Eaux Léman Contre Pollut.

Gascon Diez, E., Garcia Bravo, A., Porta, N., Masson, M., Graham, N. D., Stoll, S., Akht-man, Y., Amouroux, D., Loizeau, J.-L. (2013). Influence of a wastewater treatment plant on mercury contamination and sediment characteristics in Vidy Bay (Lake Geneva, Switzerland). Aquatic Sciences 76 (S1), 21–32.

Goldscheider, N., Haller, L., Poté, J., Wildi, W., Zopfi, J. (2007). Characterizing Water Cir-culation and Contaminant Transport in Lake Geneva Using Bacteriophage Tracer Ex-periments and Limnological Methods. Environmental Science & Technology 41 (15), 5252–5258.

Haller, L., Amedegnato, E., Poté, J., Wildi, W. (2009a). Influence of Freshwater Sediment Characteristics on Persistence of Fecal Indicator Bacteria. Water, Air, and Soil Pollution 203 (1-4), 217–227.

80

References Haller, L., Poté, J., Loizeau, J.-L., Wildi, W. (2009b). Distribution and survival of faecal indicator bacteria in the sediments of the Bay of Vidy, Lake Geneva, Switzerland. Eco-logical Indicators 9 (3), 540–547.

He, Q., Walling, D. E. (1996). Use of fallout Pb-210 measurements to investigate longer-term rates and patterns of overbank sediment deposition on the floodplains of lowland rivers. Earth Surface Processes and Landforms 21 (2), 141–154.

Klump, J. V., Edgington, D. N., Waples, J. T., Szmania, D. C., Brown, B. E., Orlandini, K. A.

(2004). Sampling Methods and Approaches Using Radionuclide Tracers in the Study of Sediment Resuspension and Cross Margin Transport in Nearshore of the Laurentian Great Lakes. International Journal of Sediment Research 18 (2), 266–277.

Lazzarotto, J., Nirel, P., Rapin, F. (2006). Évolution Physico-Chimique des Eaux du Léman (Éléments Majeurs) - Physical-Chemical Changes in the Waters of Lake Geneva (major-elements). Tech. rep. Comm. Int. Prot. Eaux Léman Contre Pollut.

Lazzarotto, J., Quetin, P., Klein, A. (2013). Évolution Physico-Chimique des Eaux du Lé-man (Éléments Majeurs) - Physical-Chemical Changes in the Waters of Lake Geneva (major-elements). Tech. rep. Comm. Int. Prot. Eaux Léman Contre Pollut.

Le Thi, A. D., De Pascalis, F., Umgiesser, G., Wildi, W. (2012). Structure thermique et courantologie du Léman (Thermal structure and circulation patterns of Lake Geneva).

Archives des Sciences 65, 65–80.

Lemmin, U., Mortimer, C. H., Bäuerle, E. (2005). Internal seiche dynamics in Lake Geneva.

Limnology and Oceanography, 207–216.

Loizeau, J.-L., Arbouille, D., Santiago, S., Vernet, J.-P. (1994). Evaluation of a wide range laser diffraction grain size analyser for use with sediments. Sedimentology 41 (2), 353–

361.

Loizeau, J.-L., Pardos, M., Monna, F., Peytremann, C., Haller, L., Dominik, J. (2004). The impact of a sewage treatment plant’s effluent on sediment quality in a small bay in Lake Geneva (Switzerland-France). Part 2: Temporal evolution of heavy metals. Lakes and Reservoirs: Research and Management 9 (1), 53–63.

Loizeau, J.-L., Rozé, S., Peytremann, C., Monna, F., Dominik, J. (2003). Mapping sediment accumulation rate by using volume magnetic susceptibility core correlation in a contam-inated bay (Lake Geneva, Switzerland). Eclogae Geologicae Helvetiae 96, S73–S79.

Mabit, L., Benmansour, M., Walling, D. E. (2008). Comparative advantages and limitations

Discrimination Between Vertical and Lateral Sedimentation Pathways in a Contaminated Bay

Ozen, B., Thorpe, S. A., Lemmin, U., Osborn, T. R. (2006). Cold-water events and dissi-pation in the mixed layer of a lake. Journal of Physical Oceanography 36 (10), 1928–

1939.

Pardos, M., Benninghoff, C., De Alencastro, L. F., Wildi, W. (2004). The impact of a sewage treatment plant’s effluent on sediment quality in a small bay in Lake Geneva (Switzer-land–France). Part 1: Spatial distribution of contaminants and the potential for biological impacts. Lakes and Reservoirs: Research and Management 9 (1), 41–52.

Perga, M.-E., Laine, L. (2012). The Zooplankton of Lake Geneva. Tech. rep. Comm. Int.

Prot. Eaux Léman Contre Pollut.

Poté, J., Goldscheider, N., Haller, L., Zopfi, J., Khajehnouri, F., Wildi, W. (2008a). Origin and spatial–temporal distribution of faecal bacteria in a bay of Lake Geneva, Switzer-land. Environmental Monitoring and Assessment 154 (1-4), 337–348.

Poté, J., Haller, L., Loizeau, J.-L., Garcia Bravo, A., Sastre, V., Wildi, W. (2008b). Effects of a sewage treatment plant outlet pipe extension on the distribution of contaminants in the sediments of the Bay of Vidy, Lake Geneva, Switzerland. Bioresource Technology 99 (15), 7122–7131.

Razmi, A. M., Barry, D. A., Bakhtyar, R., Le Dantec, N., Dastgheib, A., Lemmin, U., Wüest, A. (2013). Current variability in a wide and open lacustrine embayment in Lake Geneva (Switzerland). Journal of Great Lakes Research 39 (3), 455–465.

Rimet, F. (2012). The Phytoplankton of Lake Geneva. Tech. rep. Comm. Int. Prot. Eaux Léman Contre Pollut.

Savoye, N., Benitez-Nelson, C., Burd, A. B., Cochran, J. K., Charette, M., Buesseler, K. O., Jackson, G. A., Roy-Barman, M., Schmidt, S., Elskens, M. (2006). 234Th sorption and export models in the water column: A review. Marine Chemistry 100 (3-4), 234–249.

Thorpe, S. A., Keen, J. M., Jiang, R., Lemmin, U. (1996). High-frequency internal waves in Lake Geneva. Philosophical Transactions of the Royal Society of London. Series A -Mathematical, Physical and Engineering Sciences 354 (1705), 237–257.

Wan, G. J., Chen, J. A., Wu, F. C., Xu, S. Q., Bai, Z. G., Wan, E. Y., Wang, C. S., Huang, R. G., Yeager, K. M., Santschi, P. H. (2005). Coupling between 210Pbex and organic matter in sediments of a nutrient-enriched lake: An example from Lake Chenghai, China.

Chemical Geology 224 (4), 223–236.

Wieland, E., Santschi, P. H., Beer, J. (1991). A Multitracer Study of Radionuclides in Lake Zurich, Switzerland 2. Residence Times, Removal Processes, and Sediment Focusing.

Journal of Geophysical Research 96 (C9), 17067–17080.

82

C HAPTER 4

B OTTOM BOUNDARY LAYER HYDRODYNAMICS AND SEDI

-MENT FOCUSING : IMPLICATIONS FOR A CONTAMINATED BAY

This chapter investigates the hydrodynamics of the bottom boundary layer of Vidy Bay. This is necessary for a rounded, more complete, picture of sediment entrainment and transport dynamics and, in such, an understanding of particle-bound contaminant fate. This study was designed to investigate how the hydrodynamic conditions of the bottom boundary layer affect Vidy Bay in terms of sediment resuspension and transport dynamics and how these hydrodynamic conditions relate to the sedimentation pathways, lateral advections, and con-taminant transport discovered in the previous chapter.

Bottom boundary layer hydrodynamics and sediment focusing: implications for a contaminated bay

Bottom boundary layer hydrodynamics and sediment focus-ing: implications for a contaminated bay

Neil D. Graham*1, Damien Bouffard2, Jean-Luc Loizeau1

1Institute F.-A. Forel, Earth and Environmental Sciences Section, University of Geneva Route de Suisse, 10, 1290 Versoix, GE, Switzerland

2Physics of Aquatic Systems Laboratory — Margaretha Kamprad Chair, ENAC École Polytechnique Fédérale de Lausanne (EPFL), Lausanne, Switzerland

*Neil.Graham@unige.ch

An article of form similar to this chapter will be submitted for publishing.

84

4.1 Abstract

4.1 Abstract

Understanding the hydrodynamics of the bottom boundary layer of a lake is necessary for a more complete picture of sediment entrainment and transport dynamics, and in such an understanding of particle-bound contaminant fate. Vidy Bay (Lake Geneva, Switzerland) is the most contaminated part of the lake due to its reception of treated wastewaters. This study was designed to investigate how the hydrodynamic conditions of the bottom boundary layer affect Vidy Bay in terms of sediment resuspension and transport dynamics. The aim of the study was to uncover how local hydrodynamic conditions influence sediment focusing and the potential spread of contamination from the bay to the main basin.

Hydrodynamic measurements showed the persistent influence of a secondary gyre ex-tending down to the bottom boundary layer while just outside of the bay circulation was influenced by the seasonal patterns of the main basin. Calculated mean displacement dis-tances in the bay indicated that suspended particles can travel∼3 km per month, which is 1.5 times the extent of the Vidy Bay gyre. This results in a residence time of approximately 10 d for suspended particles and is at the upper limit of, or longer than, previously mod-elled results. The calculated mobility Shield parameter never exceeded the threshold shear stress needed for resuspension in deeper parts of the bay. In such, increased lateral advec-tions to the bay are not likely due to local resuspension but rather external particle sources.

These external suspended sediment sources coupled with an increased residence time, and decreased current velocity are the precipitating factors in sediment focusing. Contaminant spread from the bay may occur through the transport of suspended sediments in shallower zones of the bay or fine suspended sediments of the WWTP effluent by longshore littoral currents.

4.2 Introduction

Sediment focusing is the accumulation of sediments in quiescent, less energetic, zones of

Bottom boundary layer hydrodynamics and sediment focusing: implications for a contaminated bay

ecological, economic, and health impacts through the reintroduction of contaminants to the water column (Girardclos et al., 2007; Haller et al., 2009b; Herrero et al., 2013). Since sediments act as both a source and sink for many contaminants and nutrients, it is important to understand the nature of sediment transport dynamics to aid in planning and managing sustainable water reserves for the future.

Sedimentation can be studied over decadal and centurial time-scales through sediment core profiling; however, these methods provide little resolution for the relationships between sedimentation dynamics, hydrodynamics, and the physicochemical sediment characteristics.

Short-term spatial-temporal studies provide a more vivid picture of the sedimentation dy-namics at a given location. The use of sediment traps allows for the estimation of temporal and spatial variation in sedimentation rates and suspended particle composition. Analysis of sediment samples for radionuclides has proven to be useful in estimating particle residence times and identifying sedimentation pathways in various aquatic environments (Dominik et al., 1989; Muir et al., 2005; Wieland et al., 1991). However, distinguishing between sources of particles is difficult if no identifier or tag is present (Bloesch, 1994; Cornett et al., 1994).

For example, Wieland et al. (1991) were able to identify the vertical settling component to sediment traps using the pulse of137Cs recorded after the Chernobyl accident. Particles settling from the lake’s surface were labelled with137Cs, while sediments resuspended from the sediment surface were lacking this radioactive tag. A short review of other methods to identify resuspended sediments can be found in Bloesch (1994).

Ultimately, the combined use of sediment traps with current and turbidity meters is op-timal for in-situ studies on suspended particulate matter near the sediment surface (Bloesch, 1994). In this study RCM9 current meters were used to measure temporal and spatial vari-ations in hydrodynamic conditions to elucidate sediment transport dynamics in the bottom boundary layer of Vidy Bay. These results are used to help identify the source(s) of sed-iments previously shown to focus in the bay, see Chapter 3. The sediment trap study in Chapter 3 was conducted at the same sites as, and concurrent with, the use of the RCM9 current meters. In chapter 3, the use of7Be and 210Pbxs gave insight into residence times and differentiated between vertically and laterally advected sediments.

Vidy Bay is the most contaminated part of Lake Geneva due to its reception of efflu-ents from the wastewater treatment plant (WWTP) of the City of Lausanne. The spread of contamination in the sediments and in the water column of Vidy Bay have previously been investigated (Bonvin et al., 2011; Goldscheider et al., 2007; Loizeau et al., 2004; Pardos et al., 2004; Razmi et al., 2014); however, the effect of resuspension and sediment focusing have been neglected. An understanding of sediment transport in the bay is essential in

deter-86

4.3 Environmental Setting, Materials, and Methods