A NNALES DE L ’I. H. P., SECTION A
H. R AUCH
Quantum measurements in time dependent neutron interferometry
Annales de l’I. H. P., section A, tome 49, n
o3 (1988), p. 355-368
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355
Quantum Measurements
in Time Dependent Neutron Interferometry (*)
H. RAUCH
Atoministitut der Osterreichischen Universitaten, A-1020 Wien, Austria
Ann. Inst. Henri Poincare,
Vol. 49, n° 3, 1988, Physique theorique
ABSTRACT. 2014 The
perfect crystal
neutron interferometer has been usedcontinuously
for test measurements on quantum mechanics. Polarized neutrons were used toperform
the quantum mechanicalspin-superposition experiment
on amacroscopic
scale. Thisexperiment
was continued with two resonance coils in thebeams,
in which the coherencepersisted,
evenif an energy
exchange
occurred withcertainty
between the neutron and the resonator system. A quantum beat effect was observed whenslightly
different resonance
frequencies
wereapplied
to both beams. In this case,an
extremely high
energysensitivity
of 2.7 x10 -19
eV was achieved.Neutron spectroscopy is thus able to cover time domains from micro-
scopic
tomacroscopic
scales. All the results obtained until now are inagreement
with the formalism of quantum mechanics and stimulate discus- sion about theinterpretation
of this basictheory.
RESUME. - L’interferometre a neutrons a cristal
parfait
a servi sansdiscontinuer a faire des mesures tests en
mécanique quantique.
Des neu-trons
polarises
ont ete utilises pour effectuer uneexperience
desuperposi-
tion de
spins quantique
a l’échellemacroscopique.
Cetteexperience
futreprise,
eninterposant
deux solinoides resonnants dans les faisceaux et la coherence montreepersister
même si unechange d’energie
s’effectuait de maniere certaine entre Ie neutron et Iesystème
resonnant. Un effet de battementquantique
a ete observequand
desfrequences
de resonancelegerement
différentes sontappliquees
aux deux faisceaux. Dans ce cas une sensibilite enenergie
extremementgrande (2,7
x10 -19 ct)
a ete(*) This article is an abridged and slightly modified version of the article « Quantum
measurements in Neutron Interferometry » published in the Proc. 2nd Int. Symp. Founda-
tions of Quantum Mechanics, Tokyo, 1986.
Annales de l’lnstitut Henri Poincare - Physique theorique - 0246-0211
Vol. 49/88/03/355/14/$3,40/(~) Gauthier-Villars
atteinte. La
spectroscopie
de neutrons peut done couvrir des domainestemporels
allant de 1’echellemicroscopique
a l’échellemacroscopique.
Tous les resultats obtenus
jusqu’a present
sont en accord avec Ie forma-lisme de la
mecanique quantique
et suscite des discussions surl’interpré-
tation de cette theorie fondamentale.
§ 1 ~.
INTRODUCTIONThe
perfect crystal
interferometer represents amacroscopic
quantum device with characteristic dimensions of severalcentimeters.
The basisfor this kind of
X-ray
or neutroninterferometry
isprovided by
the undis-turbed arrangement of atoms in a monolithic
perfect
siliconcrystal [1 ], [2 ].
An incident beam is
split coherently
at the firstcrystal plate,
reflectedat the middle
plate
andcoherently superposed
at the thirdplate (fig. 1).
It follows
immediately
fromgeneral
symmetry considerations that thewave functions in both beam
paths,
which compose the beam in the forward direction behind theinterferometer,
areequal
= becausethey
are transmitted-reflected-reflected
(TRR)
and reflected-reflected-transmitted(RRT), respectively.
The system is based onBragg
diffraction fromperfect crystals; therefore,
the deBroglie wavelength
of the neutrons is about 1.8A
and their energy about 0.025 eV.
The whole theoretical treatment of the diffraction process is based on
the
dynamical
diffractiontheory,
which can also be found in the literature for the neutron case[3-8 ].
A
phase
shift between the two coherent beams can beproduced by nuclear, magnetic
orgravitational
interactions. In the first case, thephase
shiftis most
easily
calculatedusing
the index of refraction n[9], [10 ].
FIG. 1. - Sketch of the standard o symmetric perfect crystal interferometer.
Annales de l’lnstitut Henri Poincaré - Physique " theorique "
QUANTUM MEASUREMENTS IN TIME DEPENDENT NEUTRON INTERFEROMETRY 357
As in
ordinary light optics
thechange
of the wave function is obtainedas follows :
Therefore,
theintensity
behind the interferometer isgiven by
The
intensity
of the beam in the deviated direction follows fromparticle
conservation :
Thus,
the intensities behind the interferometer vary as a function of the thickness D of thephase shifter,
theparticle density
N or the neutronwavelength
~,.The
magnetic
interaction is causedby
thedipole coupling
of themagnetic
moment of the neutron ~c to a
magnetic
field B(H
= - jM’B). Therefore,
the
propagation
of the wave function isgiven by
. where a represents a formal
description
of the Larmor rotationangle
around the field B
(IX
=(2 /h) J Bdt = J Bds).
This wave function
shows the
typical 4~-symmetry
of aspinor
whereas
203C0-symmetry
existsonly
for theexpectation
valueThe
47r-periodicity
becomes visible in interferometerexperiments,
aspredicted theoretically [11-13 ],
and has been verifiedexperimentally
inearly
neutron interferometricexperiments [14 ], [7J],
where theintensity
for
unpolarized
incident neutrons was found to beB "/
These results are
widely
debated in the literature. It should be mentioned that this4~-symmetry
canalways
be attributed to real rotations in thecase of fermions
[16 ], [17 ]. Today,
the mostprecise
value for theperiodicity
factor is ao = 715.87 ± 3.8
degrees [18 ].
This valueprovides only
a smallmargin
forspeculation
aboutSU(2)-symmetry breaking,
but a new andmore
precise
determination of ao is recommended. The403C0-periodicity
effect has been observed for
unpolarized
as well aspolarized
neutrons,3-1988.
which demonstrates the intrinsic feature of this
phenomenon
and theself-interference
properties
involved in these kinds ofexperiments.
Under reasonable
experimental
parameters, the action of thegravita-
tional field on the neutron is
comparable
to the nuclear andmagnetic
interaction. On the surface of the earth the pure
gravitational
term andthe Coriolis term due to the earth’s rotation have to be considered as
where g
is thegravitational acceleration,
r the space vetor from the centreof the
earth,
úJ the earth’sangular
rotationvelocity
and L = r theangular
momentum of the neutron relative to the centre of the earth.This
gravitational
interaction causes thefollowing phase
shifts[79-27] ]
resulting
in thefollowing intensity
modulationA is the area enclosed
by
the coherentbeams,
() is theangle
of deviationof this
plane
from thehorizontal, 0L
is the colatitudeangle
of theplace,
where the
experiment
isperformed,
and 8 is the rotationangle
around thevertical direction.
Experiments performed by
aUS-group [19 ], [22], [2~] ]
have shown
complete
agreement betweenexperiment
andtheory. Recently,
the Dortmund interferometer group has extended these kinds of
experiments
to observe interferences in noninertial frames
[24 ].
All the results of interferometric measurements obtained until now can be
explained
well in terms of the wavepicture
ofquantum
mechanics and thecomplementarity principle
of standardquantum
mechanics.Nevertheless,
one should bear in mind that the neutron also carries well- definedparticle properties,
which have to be transferredthrough
the inter-ferometer. These are : its mass of m =
1.6749543(86)
x10 - 2’ kg,
itsspin h/2
and associatedmagnetic moment
= -1.91304308(54) K,
its effec- tive radius of about 0.7fm,
and internal structureconsisting
of one « up »and two « down »
quarks. Therefore,
neutrons seem to be a proper tool fortesting
quantum mechanics of massiveparticles,
where the wave-particle
dualism becomes obvious.All neutron interferometric
experiments pertain
to the case of self-interference,
whereduring
a certain timeinterval, only
one neutron isinside the
interferometer,
if at all.Usually,
at thistime,
the next neutron has notyet
been born and is still contained in a uranium nucleus of the reactor fuel.Although
there is no interaction between different neutrons,Annales de l’lnstitut Henri Poincare - Physique theorique
QUANTUM MEASUREMENTS IN TIME DEPENDENT NEUTRON INTERFEROMETRY 359
they
have a certain commonhistory
withinpredetermined
limits whichare
defined,
e. g.,by
the neutron moderation process,by
their movementalong
the neutronguide tubes, by
the monochromatorcrystal
andby
thespecial
interferometer set-up.Therefore,
any real interferometerpattern
containssingle particle
and ensembleproperties together.
In this
article,
recent results obtainedby
our groupduring
theperiod
1984-1987 will be
presented [25 ],
but noepistemological interpretation
will be
given.
In this respect, the reader should refer to his ownpicture
orto the related literature.
§ 2.
SPIN STATE INTERFEROMETRYWe
already reported
on theexperimental
verification of the quantum mechanicalspin superposition
law on amacroscopic
scaleby
means ofneutron
interferometry [25 ], [27], [28 ].
Theprinciples
of theseexperiments
and the most
important
results are summarized infig.
2. Moreexperimental
details can be found in the references mentioned above. There is a marked difference between the action of a static
flipper
and a resonanceflipper,
which has to be discussed in more detail.
In the first case
(static flipper
the wave function ischanged by
theflipper according
to eq.( 1. 4),
which has to beapplied
forpolarized
incident neu-trons:
The rotation of the
polarization
vector around they-axis
has beenpostu-
lated to be 7T[29 ]. Thus,
two wave functions withopposite spin
directionsare
superposed
at the thirdplate
aswhich
corresponds
to the situationproposed by Wigner [30 in
1963 toverify
the quantum mechanicalspin superposition
law. In this case theintensities in the 0- and H-beams are
equal
and the beams arepolarized
in the
(x, y) plane,
i. e.,perpendicular
to both the initialspin
directions.The
angle
of thepolarization
in the(x, y)-plane
isgiven by
the nuclearphase
shift :
Thus,
a pure initial state is transferred to a pure final state. The interferencepattern
appearsonly
if apolarization analysis
isperformed
inthe |x >-
Vol. 49, n° 3-1988.
FIG. 2. - Sketch of the static (above)
and the time-dependent (below) spin superposition experiment with characteristic results.
or
the y>-direction.
If theanalyzer
is set inthe |z )- (or
- z)-) direction,
nointensity
modulation is observed. Theintensity
is in this caseexactly
the sameas when
the ! -z )- (or
z)-)
beamthrough
the interferometer was blocked.Nevertheless,
thequestion
whether the neutrons transmittedthrough
a!
z)-setting
of theanalyzer originate
fromthe
z)-beam
inside the inter-ferometer,
remains anepistemological question
not answeredby
the forma-lism of quantum mechanics. If this were not the case new
possibilities
fordelayed-choice experiments
would open up, where a decision about beamAnnales de l’lnstitut Henri Poincare - Physique theorique
QUANTUM MEASUREMENTS IN TIME DEPENDENT NEUTRON INTERFEROMETRY 361
path
or interference detection could be made after the beam haspassed
the interferometer device.
The second version of the
spin superposition experiment
wasperformed
with a
Rabi-type
resonanceflipper
which is alsocommonly
used inpola-
rized neutron
physics.
This kind of interaction istime-dependent and,
inaddition to the
spin-inversion,
anexchange
of the resonance energyEHF
= occurs between the neutron and the resonator system, which has to be considered in the interferometricexperiment.
This energyexchange
was observed in a
separate experiment,
where the energy resolution ðE of the apparatus was better than the Zeeman energysplitting (DE EHF) [31 ].
For a
complete spin
reversal thefrequency
of the field has to match theresonance condition and the
amplitude B 1
has to fulfill the relationI B1l/hv
= 7T, where l is thelength
of the coil.Oscillating
fields are usedinstead of
purely
rotational fieldsand, therefore, only
onecomponent
contributes to the resonance which causes aslight
shift in the resonancefrequency
from the Larmorfrequency
=2 |B0/h
due to the Bloch-Siegert
effect = +(Bi/16Bo)]) [32 ], [33 ]. Thus,
the wave functionof the beam with the
flipper changes according
toTherefore,
aspin-up
and aspin-down
state aresuperposed
at theposition
of the third
plate.
The finalpolarization
of the beam in the forward directionis
given by
, , ,and lies
again
in the(x, y)-plane
but now rotates within thisplane
withthe resonance
(Larmor) frequency
withoutbeing
drivenby
amagnetic
field.
Therefore,
astroboscopic
method was needed for the observation of this effect. The direction of thepolarization
in the(x, y)-plane depends
on the status
(phase)
of the resonance field and has to be measured syn-chronously
with thisphase.
The observed interference pattern
(fig. 2)
demonstrates that coherencepersists, although
a well defined energyexchange
between the neutronand the apparatus exists.
Thus,
an energyexchange
is notautomatically
a
measuring
process. As we will see later on, theexchanged photon
cannotbe used for a quantum nondemolition measurement
[34 ].
In ourexperi-
ment, the
following
argument based on differentuncertainty
relations canbe used :
First,
onesingle
absorbed or emittedphoton
of the resonatorcannot be detected because of the
photon number-phase uncertainty relation,
which can be written in the form[35 ], [~6] ]
Vol. 49, n° 3-1988.
where Sand C can be
expressed by
the creation and annihilationoperators,
C =
(a-
+a+)/2
and S =(a- - a + )/2i,
whose matrix elementscouple
coherent Glauber states. For our purpose this relation can be used in its
simpler
formThe
uncertainty
of thephoton
number of the resonator is minimized fora coherent state resonator
by [37] and, therefore,
the lower limit for thephase uncertainty
becomes A0 ~~/2~/( N ).
Because in this kind ofspin-superposition experiment
thephase
determination of theflipper
field isrequired
to be better than 01/2
for thestroboscopic method,
it isimpossible
to observe asingle
absorbed or emittedphoton (ON > 1).The argument
has to bechanged
ifsqueezed
states of the electro-magnetic
field areconsidered,
where iB() canapproach
a limit ofA0 ~
1/2 (N) [38 ], [39].
Anexplanation,
which is not based on thenumber-phase uncertainty relation,
can be found in the literature[34 ].
A second version of the beam
path
detection may be based on the obser- vation of the energychange
of the neutron. This canonly
beachieved,
if the energy resolution of the instrument fulfills the relation2,uBo.
On the other
hand,
thestroboscopic measuring
methodrequires
timechannels
1/2vHF
=/~! Bo,
whichprovides
another constrainton the
experiment.
Both conditions cannot be fulfilled withrespect
to theenergy-time uncertainty
relationconcerning
the beamparameters
~/2. Therefore,
we conclude that a simultaneous detection of the beampath through
the interferometer and of the interferencepattern
remainsimpossible.
It has been
argued by Vigier’s
group[40 ], [~7] that
new information about theparticle-wave duality
can be obtained with resonator coils in both coherent beams.They
calculated the quantumpotential
and thebeam
trajectories [42 ], [~3] ]
within the frame of the causal stochastic view of quantum mechanics.Unfortunately
the results of these calculationsare identical with the results of
ordinary
quantum mechanicsand, therefore,
to discern between both
points
of view remains anepistemological problem.
The
corresponding experiments
will be discussed in the next section.§3
DOUBLE COIL EXPERIMENTSThe
experimental arrangement
for the double coilexperiment
is shownin
fig.
3[44 ], [45 ].
The finalpolarization
lies inthe |- z>
direction and the energy transfer can be smaller orlarger
than the energy resolution iBE because this information can not be in any way associated with a beampath
detection. Thelay-out
for thisexperiment
followed theproposal
Annales de l’lnstitut Henri Poincaré - Physique théorique
QUANTUM MEASUREMENTS IN TIME DEPENDENT NEUTRON INTERFEROMETRY 363
FIG. 3. - Sketch of the double resonance coil experiment.
ofVigier’s
group[40 ], [41 ]. According
to ourprevious
considerations thechange
in the wave functions with the resonanceflippers
tuned to theresonance
frequency
can be written forpolarized
incident neutrons(!
z»
and for different modes of
operation
as follows.a)
Bothflippers
areoperated synchronously
without aphase
shiftbetween the
flipper
fields :This results in an
intensity
modulationwhich is
independent
of theflipper
fields.b)
Bothflippers
areoperated synchronously
with a distinctphase
rela-tion 0 v
In this case, the
intensity
modulation isgiven by
c)
Bothflippers
areoperated asynchronously
withstatistically
fluc-tuating phase
differences0(t)
which average outduring
themeasuring
interval. Then
Io
oc const.(3 . 5)
It should be mentioned in this context
that,
even in this case, coherencephenomena
can be observed if astroboscopic investigation
isperformed (Io
=The results of these related
experiments
are shown infig.
4.Complete
agreement with the theoretical
predictions
is found. The interferenceproperties
arepreserved, although
an energyexchange certainly
takesVol. 49, n° 3-1988.
FIG. 4. - Results of the double coil experiments. Above: Synchronous flipper fields with 71.90 kHz (eq. (3.2)). Middle: Two slightly fluctuating independent flipper fields
with Vr = 71.92 ± 0.02 kHz (eq. (3.5)). Below: Interference pattern as a function of the phase shift A between both flipper fields at Vr = 71.90 kHz (eq. (3.4)).
place. Only
quanta within a narrow energy band aroundh03C9r
and no othersare excited inside the
flipper
resonator.Therefore,
one could believe that thespin flip
and the energy transfer process to the neutron occurred inside one of the twocoils,
which would demonstrate that the neutron has chosenAnnales de l’lnstitut Henri Poincare - Physique theorique
365 QUANTUM MEASUREMENTS IN TIME DEPENDENT NEUTRON INTERFEROMETRY
one of the two
possible paths.
But even this rather weak statement wouldrequire
the concept ofpilot
waves, quantumpotentials,
etc.,leading
imme-diately
toquestions
about theinterpretation
of quantummechanics,
which are not the
subject
of this article. The situation with twoslightly
different resonance
frequencies
in bothflipper
coils will be discussed in the next section.§4
MACROSCOPICQUANTITIES
IN UNCERTAINTY RELATIONS
By
means ofperfect crystal
neutronoptics
the resolution in momentumor energy space can be increased to such an extent that the
conjugate quantities
reachmacroscopic
dimensions.The
experiments
have beenperformed
with monolithicmultiplate
systems
by rotating
awedge shaped
material around the beamaxis;
thisprivides
a proper control of small beam deflections in the horizontalplane,
which is the
only
sensitiveplane
forperfect crystal
reflections.Although
thewavelength
of the neutrons is smaller than the width ofthe slit
by
a factor of about108,
thebroadening
of the centralpeak
becomesvisible due to the
high angular
resolution of such systems.As an alternative to the
high
momentum resolution discussedbefore,
anextremely high
energy resolution can be achievedby
aslight
modification of the double coilexperiment
described in§ 3.
If thefrequencies
of thetwo coils are chosen to be
slightly different,
the energy transfer also becomes different(AE
=0~2))’
Thefrequency
difference can be made very small ifhigh quality synthesizers
are used for the fieldgeneration.
Theflipping
efficiencies for both coils arealways
very close to 1(better
than0.99). Now,
the wave functionschange according
toTherefore,
theintensity
behind the interferometer exhibits atypical
quantum beat effectgiven by
Thus,
theintensity
behind the interferometer oscillates between the forward and deviated beam without anyapparent change
inside the interferome-ter
[44 ], [45 ].
The time constant of this modulation can reach amacroscopic
scale which is
again
correlated to anuncertainty
relation oEOt >_~/2.
Figure
5 shows the result of anexperiment
where theperiodicity
of theintensity modulation,
T =cvr2),
amounts to T =(47.90
±0.15)s
caused
by
afrequency
difference of about 0.02 Hz. Thiscorresponds
toa mean difference of energy transfer AE between the two
beams,
AE = 8.6 x
10 -1’ eV,
and to an energysensitivity
of 2.7 x10 -19 eV,
Vol. 49, n° 3-1988.
FIG. 5. - Quantum beat effect observed when the frequencies
of the two flipper coils differ by about 0.02 Hz around 71 899.79 Hz.
which is better
by
many orders ofmagnitude
than that of other advancedspectroscopic
methods. Thishigh
resolution isstrongly decoupled
fromthe
monochromaticity
of the neutronbeam,
which was x10 - 4
eVaround the mean energy of the beam
EB
= 0.023 eV in this case. It should be mentioned that the result can also beinterpreted
asbeing
the effectof a
slowly varying phase 0(t)
between the twoflipper
fields(see
eq.(3 . 4)),
but the more
physical description
is based on the argument of a different energy transfer. Theextremely high
resolution may be used forfundamental,
nuclear and solid state
physics applications.
An intrinsic lower limit for the energy width
DEi
of the neutron beam iscaused
by
itslifetime, r=
925s.According
to~/2,
3.5 xlO- 24
eV.The
decay
appears in both beampaths
and contributes an attenuation factor exp( -
= exp( - l/iv),
which is similar to those discussed in92.
It may bepossible
in a newexperiment
to observe thedecay
of theneutron inside the interferometer
by measuring
thedecay products,
whichwould make an
assignment
to a certain beampath possible.
§5
DISCUSSIONAll the results of the neutron interferometric
experiments
are welldescribed
by
the formalism of quantum mechanics.According
to the com-plementarity principle
of theCopenhagen interpretation,
the wavepicture
has to be used to describe the observed
phenomena.
Thequestion
as tohow the well-defined
particle properties
of the neutron are transferredthrough
theinterferometer,
is notmeaningful
within thisinterpretation,
but it should be an allowed one from the
physical point
of view.Therefore,
other
interpretations
should also be included in the discussion of suchAnnales de l’lnstitut Henri Poincare - Physique theorique
QUANTUM MEASUREMENTS IN TIME DEPENDENT NEUTRON INTERFEROMETRY 367
experiments.
We havealways
tried toperform
unbiasedexperiments
anddo not wish to interfere with any
epistemological interpretation
of quantum mechanics.Perhaps
in the future newproposals
forexperiments
will beformulated,
whichpermit
aunique
decision between differentinterpreta-
tions. As an
experimentalist,
oneappreciates
thepioneering
work of the founders of quantummechanics,
who created this basictheory
with solittle
experimental
evidence. Nowalthough
we have much more directevidence,
even on amacroscopic scale,
one nevertheless notices that theinterpretation
of quantum mechanics goesbeyond
human intuition in certain cases.Only
twoaspects
of theexperiments
discussed before should berepeated :
how can each neutron in thespin-superposition experiment
be transferred from an initial pure state in
the
z~-direction
into a pure state inthe
x~-direction
behind theinterferometer,
if nospin
turn occursin one beam and a
complete spin
reversal occurs in the other beampath ?
How can every neutron have information about which beam to
join
behindthe
interferometer,
when aslightly
different energyexchange
occurs inboth beams inside the interferometer and the time constant of the beat effect is
by
many orders ofmagnitude larger
than the time offiight through
the
system ?
,ACKNOWLEDGEMENTS
All the
experimental
results discussed in detail have been obtainedby
our Dortmund-Grenoble-Vienna interferometer group
working
at thehigh
flux reactor in Grenoble. Thecooperation
within this group andespecially
thecooperation
withcolleagues
from ourInstitute,
which arecited in the
references,
aregratefully acknowledged.
Personal discussions with M. M. Nieto(Livermore),
D. Petrascheck(Linz)
and J.-P.Vigier (Paris)
stimulated newexperiments.
The financial support for the expe- riments wasprovided by
Fonds zurForderung
der WissenschaftlichenForschung (contracts
P-4230 andS-4201 ).
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(Manuscrit reçu le 10 juillet 1988)
Note added : In the paper « Inelastic action of a
gradient radio-frequency
neutron
spin flipper » by
H.Weinfurter,
G.Badurek,
H.Rauch,
D.Schwahn,
to be
published
in Z.Phys.,
t. B72,1988, p.195,
wepresent
some results that show veryclearly
the energy transfer within aflipper
coil.Annales de l’Institut Henri Poincare - Physique theorique