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HAL Id: jpa-00246927

https://hal.archives-ouvertes.fr/jpa-00246927

Submitted on 1 Jan 1994

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Stéphane Roux, Alex Hansen

To cite this version:

Stéphane Roux, Alex Hansen. Interface roughening and pinning. Journal de Physique I, EDP Sciences,

1994, 4 (4), pp.515-538. �10.1051/jp1:1994157�. �jpa-00246927�

(2)

Classification Pllysics Abstracts

61A3H 64.60A 68.45G 61.72L

Interface roughening and pinning

Stéphane

Roux

(1)

and Alex Hansen (~>*)

(1) Laboratoire de Physique et Mécanique des Milieux Hétérogènes

(**),

Ecole Supérieure de

Physique et Chimie industrielles, 10 rue Vauquelin, 75231 Paris Cedex 05, France

(~) Groupe Matière Condensée et Matériaux, URA CNRS 804, Université de Rennes 1, Campus

de Beaulieu, 35042 Rennes Cedex, France

(Received

27 September1993, accepted in final form 24 December

1993)

Résumé Nous étudions un modèle simple pour analyser l'accrochage d'une interface

sur des

impuretés et le décrochage sous l'effet d'une pression appliquée, dans une limite quasi-statique.

Ce modèle est très voisin du modèle '~Robin Hood" introduit par Zaitsev. Il s'applique en parti-

culier à l'invasion d'un fluide mouillant

(imbibition)

dans un milieu poreux hétérogène contenant

un fluide immiscible. Nous discutons les relations entre ce modèle et d'autres approches propo- sées pour décrire

ce phénomène. Le front d'invasion acquiert une structure auto-affine, avec

un développement de la rugosité selon une loi de puissance du volume injecté. La valeur de l'exposant de

rugosité

apparent se compare bien avec des mesures expérimentales, mais nous

montrons que l'exposant réel est hors de portée des méthodes d'analyse habituelles. La distribu-

tion,

f(d, Al),

des distances, d, entre pores envahis à un intervalle de temps Al peut être décrit par une loi d'échelle

f(d, Ai)

=

d~~~(dllù).

Cette loi peut être obtenue

en identifiant une structure hiérarchique de "bouffées" dans le signal de pression. Ces "bouffées" sont qualitative-

ment similaires à celles observées lors du drainage

(invasion

d'un fluide non

mouillant),

dans un

régime de percolation d'invasion.

Abstract. We study a simple model for the pmning of an interface by impunties with

random strengths, and the depinning due to the applied pressure, m a quasi-static propagation limit. The model is very close to the so called "Robin Hood" model introduced by Zaitsev.

It is designed to describe e-g- the invasion of a wetting fluid

(imbibition)

in a heterogeneous

porous medium

containmg

a second immiscible fiuid. The relation between this model and

other previously proposed approaches is discussed. The front of the mvaded domain is shown to

develop a self-affine structure with an increase of the roughness as a power-law of the injected

volume. The value of the apparent roughness exponent can be favorably compared to some

expenmental measurements although we argue that the true roughness exponent is out of reach of commonly used methods. We show that the distribution

f(d,

Al) of distances d between

discrete local invasions at a time interval Al can be described by a scaling law

f(d, Al)

=

d~~~(dllù).

This form

can be obtained from the identification of a hierarchical structure of ~'bursts"

m the pressure signal. Those ~'bursts" are qualitatively similar to those observed

in quasistatic drainage, (1.e. invasion percolation), although charactenzed by dilferent scaling indices.

(*) Also at Institutt for Fysikk, NTH, N-7034 Trondheim, Norway.

(**) URA CNRS 857.

(3)

1 Introduction.

The geometry and trie

dynarnics

of trie

propagation

of interfaces in a

heterogeneous and/or noisy

environment is a

problem

which occurs in a

variety

of fields. Much progress bas

recently

been achieved

through

trie

quantitative analysis

of trie fluctuation of trie interface both in a number of

experimental examples,

and

through

trie

development

of various models which have revealed very

general scaling

laws

iii.

in various

growth models,

it has been realized that the

roughness

of the front can be described

by scaling laws,

which accounts both for a self-

afline geometry below a characteristic

length

scale the correlation

length

and the time

development

of this correlation

length.

A few selected works

focusing

on this property have been collected in a recent book [2].

However, despite

this progress, some situations still

display

features which cannot be con-

vincingly

described

by existing

models without

resorting

to some additional

hypotheses (e.g.

long

range correlation [3],

singular

distribution of noise [4], or even

inhomogeneous spatial

distribution of

pinning

centers with a

power-law dependence

on the distance from an

injection

side [Si

...)

whose

physical

foundation remains unclear. More

recently,

the rote of

pinning

has been outlined in a series of model [5-10] we will discuss further.

One such

example

of interface

propagation

which is

lacking

a proper

understanding

is trie structure of imbibition fronts even in trie

simplifying

limit of

quasistatic

fiow. Imbibition is trie invasion of a

wetting

fiuid in a porous media filled with another immiscible less

wetting

fiuid. We will in trie

following

use this

problem

to derive trie rules of trie model we

study,

and to

highlight

its relation with a model called trie "Robin Hood" model RH model in trie

following

introduced

recently by

Zaitsev

[loi

and later studied

by Sneppen

[9]. Albeit we will

essentially

refer to the imbibition

problem,

the RH model and results may be

applied

to other cases.

Among

other fields of

application,

one may quote trie

growth

of bacteria

colony [11],

trie motion of vortex lines in

superconductors

[12], of dislocations in

crystals [loi,

or

even trie

roughening

of crack fronts in fracture [13]. In addition trie RH model shares some

similarities with other models

proposed

in trie context of solid friction [14] or

earthquakes [15],

of avalanches in

granular

media

[16j.

It should also be

emphasized

that trie motivation for

studying

those

problems

is not

simply

to bave a proper statistical

description

of trie geometry of trie

interface,

but also to

gain

some

insight

into trie

global pinning

and

propagation

of an interface. In trie domain of

wetting,

heterogeneities

are

responsible

for trie occurrence of a

hysteretic

behavior of trie

(macroscopic)

contact

angle

between two fiuids [17].

Understanding

and

quantifying

this

hysteresis

is still a

major challenge.

It bas been

recognized

[18j

long

ago

that,

m trie case of a

non-wetting invading fiuid,

trie sc-called

~'drainage"

case, trie

development

of trie interface between trie two fluids in a porous medium could be

accurately

described

by

an "invasion

percolation"

model.

Experiments

[19j bave confirmed trie

validity

of this limit. Trie case of

~'imbibition",

1-e- when trie

invading

fiuid is

wetting,

is a

question

which bas been addressed much more

recently

in terms of statistical

analysis.

Trie

development

of imbibition fronts bas been studied

expenmentally recently

in two or quasi-two dimensional

geometries by

dilferent groups

[20-23]

and trie results they bave

obtained are

quite comparable (although

trie very precise value of trie

roughness

exponent

they

measured bas been

slightly

controvers1al

[22]).

However, these values are much

larger

than

initially expected

from theoretical models.

One of trie most celebrated models in trie field of interface

growth,

trie

Kardar,

Parisi and

Zhang equation

[24], which

appeared

a

priori

to be a reasonable

description

for such a

problem

bas led to

quantitative

dilferences with respect to observed

expenmental

data.

Attempts

to

(4)

modify

this model in order to match trie measured

properties, through

trie introduction of

a

power-law

noise distribution [4], or a

long

range time or space correlated noise [3] or non

homogeneous spatial

distribution of

pinning

centers [Si seem to be difficult to

justify

for trie

experimental

systems which bave been studied

although

some

analysis

bas been carried in this direction [25]. Other

proposais

bave been made such as trie

suggestion

that directed

percolation

or vanants [26, 27] may

provide

a suitable frarnework.

However,

at present, trie

justification

of such models is

mostly

based on trie numerical agreement between measured and

proposed

exponents.

A much more

promising approach

bas been

independently proposed by

Kessler et ai. [7] and Parisi [8] who bave both noted that

taking

into account a

quenched

noise leads to a

change

of trie

scaling

exponents of trie

original

KPZ

equation. However,

both studies bave been carried out in

regimes

such that trie new

scaling

which could be

favorably compared

to trie

experiments

was

only

of a limited

validity. Sneppen

[9] bas shown that a

simple

modification of trie above

proposed

models with

quenched

noise reveals

naturally

trie

required scaling properties by keeping

trie

driving

force on trie interface

exactly

at its

depinning threshold,

in a

spirit

similar to invasion

percolation.

In fact trie model studied

by Sneppen

had

originally

been introduced

a little earlier in a dilferent context,

namely

trie

propagation

of dislocation

lines, by

Zaitsev

[loi.

Trie "Robin Hood" model was trie name chosen in trie latter reference and thus we will

use it in trie

folllowing.

Cieplak

and Robbins

[28-30]

bave introduced a two dimensional model hereafter referred to as trie CR model for

finding

static

equilibrium configurations

of an interface between two

wetting

immiscible fiuids in a

simple

geometry. Their

analysis

leads to two very distinct

regimes depending

on trie value of trie contact

angle

between trie

invading

and trie

defending

fluid with respect to a threshold value. On trie

non-wetting

side

(for

trie

invading fiuid),

one encounters an invasion

percolation regime

characterized

by

a fractal geometry of trie invaded pores, above

a lower cut-off scale which

depends

on trie contact

angle.

On trie

wetting

side of trie transition, trie invaded domain is compact, but trie interface

displays

a self-affine

roughness.

Trie latter

regime

thus appears to be a natural candidate for

modelling

trie above mentioned imbibition

experiments

and a

quantitative

comparison bas revealed

good

agreement with

experimental

data

[29].

However,

trie CR model is both very precise m its

definition,

and very ricin in trie diflerent types of basic processes at

play

in trie local

displacement

of trie interface. A very careful

analysis

of trie dilferent types of

possible

restructuration of trie interface bas to be done in order to find

a new

position

of

equilibrium.

It is thus of uttermost

importance

to try to

single

out in trie

complex interplay

of trie basic local mechanisms trie essential features which determine trie

"universality

Mass" and thus trie

scaling

properties of trie

problem.

In trie

following

we will discuss a very crude

simplification

of trie CR model aimed ai pre-

serving

trie few

ingredients

that we believe are essent1al to

reproduce

trie imbibition

regime.

We will show that one encounters

naturally

trie RH

model,

and indeed trie

scaling

properties of

trie invasion are

correctly reproduced.

Trie

simphcity

of trie RH model allows us to

investigate

in detail many of trie statistical features which can be accessed

experimentally.

We focus our attention on two aspects: 1) trie

geometrical

features of trie

front,

and ii

)

trie pressure

signal.

Trie

analyses

we

perform

are based on trie usual

description

of front

growth

[31] as well as on

geometrical analyses

of trie interface. We also

study

trie fluctuations of trie pressure

signal

in terms of

"bursts",

a concept

brought

forward for trie

non-wetting

invasion

percolation regime [32-34].

(5)

2. Trie CR mortel.

Before

presenting

trie RH

model,

we recall

briefiy

trie model introduced

by Cieplak

and Robbins

[28-30].

Trie

starting point

is trie

description

of trie geometry of trie porous medium in two

dimensions. It is

represented by

an array of disks whose centers are on trie sites of a

regular triangular lattice,

and whose radii are

randomly

distributed. Trie latter rule

provides

trie

only

randomness of trie model which is otherwise deterministic. Trie model is static in trie sense that trie pressure in each fiuid is assumed to be

homogeneous.

Across trie interface there exists a pressure

discontinuity

due to

capillary

forces which is related to trie curvature of trie

menisci,

which is thus constant for all pores. As a

result,

trie interface between trie two fluids thus consists of a series of circular menisci of

equal

radii

connecting

trie disks. An additional

parameter is needed for

determming

trie front geometry for a

given

pressure

drop, namely

trie contact

angle

which

gives

trie direction of trie tangent to trie minuscus with respect to trie tangent to trie disk at trie contact

point. Being given

trie pressure

drop

and trie contact

angle,

it is thus a

simple

exercice to compute trie location of a meniscus between two

disks,

and to check that trie obtained meniscus does not

overlap

with a

neighbouring

disk or another meniscus.

Let us also note that for a

given pair

of disks

(a pore),

there exists a maximum pressure above which no stable solution can be found. This allows one to construct an admissible

position

of trie interface step

by

step.

Trie

interesting

aspect of trie CR model is however not to generate ail or any admissible front

locations,

but rather to follow how a

given

interface will move to a new

configuration

of

equilibrium

after an increase in pressure or in

injected

volume. In order to find this transition,

a detailed

analysis

of trie local

restructuring

is needed. Three diflerent mechanisms can be identified:

a

)

Bitrst: when trie pressure exceeds trie maximum value that can be

supported by

a

given

pore,

no stable

configuration

can be found and thus its radius tends to increase until it encounters a

neighbouring

disk or

interface,

two cases which are considered below.

b)

Toitch: trie arc

connecting

two disks

(1- j)

intersects another disk

(k).

In this case, trie meniscus is broken into two arcs

(1- k)

and

(k j) (see Fig. la).

c) Ouerlap:

two arcs

(1- j)

and

(j k) overlap

on one disk

j.

In this case, trie two menisci will merge to form one

single

(1

k)

meniscus

(see Fig. lb).

Obviously,

once such a

restructuring

bas taken

place,

additional ones may again be necessary, until a stable

configuration

is found.

> w

Touch

Overlap

la) 16)

Fig. l. Schematic view of the two major mechamsms through which trie front evolves m the original model introduced by Cieplack and Robbins. The location of the front formed by the menisci is

determmed step by step by searching for the ~'touchs" (a) and "overlaps" (b) which

are the most

limitative m terms of pressure.

(6)

Clearly,

trie "burst" case is trie one which is dominant in trie invasion

percolation regime.

For trie

wetting

invasion

regime,

trie

interplay

of ail three mechanisms and

particularly

of "touches"

and

~'overlaps"

makes it diilicult to

single

out

only

one mode as discussed in reference [29].

It is important to note a

major

diflerence between trie first two cases and trie third one.

Bursts and touches are local

properties

of one

single

pore.

Although

that may not be an

efficient way of

handling

trie

problem numencally,

one could think of

assigning

to each pore

(e.g. pair

of

neighbouring disks)

an interval of pressure that con be

supported. Ignoring

trie

"overlap" mode,

trie

problem

would then reduce to an invasion

percolation problem

in trie pore space, (1.e. on a lattice dual to that of trie

disks).

On trie contrary, trie

overlap

mode cannot be

expressed

as a

single

pore property, as it involves trie interaction of two

neighbouring

pores. It thus seems

likely

that this mechanism

plays

a

determining

role in trie

regime

where compact clusters are

generated.

Trie

spirit

of trie

simple

model we will present below is to retain

only

this

mechanism,

and to

investigate

its

consequences in detail.

We will furthermore take disorder

explicitly

into account since it is

obviously

an essential

mgredient.

As a final observation

relying

on trie

reported experimental results,

we note that trie fronts

generated

in trie

wetting regime

are

rougir

but

asymptotically

flat

(trie roughness

divided

by

trie system size tends to zero for an infinite system

size).

We will use this property

by assuming

that trie interface can be considered as

being

defined

by

a

single

valued function of a coordinate axis

along

trie mean direction of trie front. Thus we will

neglect

trie occurrence of

overhangs.

As far as one is

only

interested in trie

scaling

features of trie geometry of trie front and related

properties,

trie details of trie CR model should not be relevant. Dur aim is to

simplify

but preserve trie essent1al features which determine trie

universality

Mass of trie model. In

some sense we are

looking

for a model for imbibition

playing

an

analogous

role as trie invasion

percolation

model for

quasistatic drainage.

3. Mortel definition and relation witl~ otl~er mortels.

We propose to model trie front as a

single

valued function of an abscissa

along

trie front. We

moreover discretize

it,

and represent it as a series of

heights

% where1 is a discrete index. With

this restriction, we forbid trie occurrence of

overhangs,

which are not

expected

anyway to

play

a

significant

role in trie

wetting regime.

Such would not be trie case for trie non

wetting regime.

We will see below that in fact trie conclusions we reach are in confiict with this

hypothesis.

Hence,

trie domain of

validity

of trie model we will

study

is restricted to scales small

enough

so that trie

slope

of trie front is small

compared

to 1. For

comparison

with trie CR

model,

trie

% could be

thought

of as trie distance of trie disk which is part of trie interface at an abscissa

(see Fig. 2).

We mentioned earlier that we

only

wished to take into account trie

"overlap"

mode. This is done

by assigmng

a threshold t~ to trie admissible citruatitre

(%-1 2%

+

%+1)

of trie interface

at each point. This threshold is meant to take into account trie diflerence of orientation in two consecutive menisci, as well as trie distance between trie disks. Trie directedness we impose

on trie front allows one

single pair

of menisci to be considered at each

site,

whereas in trie

original

CR

model,

ail

pairs

of bonds

onginating

from a site had to be taken into account to describe ail trie

possible overlaps properly.

Trie thresholds are chosen at random from a uniform

distribution between o and tmax. For a

given configuration

of trie

front,

%, and of trie

pinning

strength

t~, we bave to decide where trie front will move. When trie pressure increases, trie

angle

between trie two menisci

touching

a

given

site decreases in a non-linear fashion.

However,

(7)

o-i) o) o+1)

Fig. 2. Illustration of the discrete model studied in this paper. The front shown

as a bold line

consists in a series of discrete heights y~. Pinning centers are located at fixed abscissa along the

thin vertical bues but at random heights and with randomly varying strength. The force exerted by

the front on the pinning center is approximated by the dilference of slopes between the two segments (1

1)-j)

and

j)-(1+1).

assuming

that 1) the distance between

pinning

centers varies

only

in a small

interval,

and that ii

)

trie deformation of each meniscus is limited to a small range, we con linearize finis relation.

Moreover,

we will consider that trie rate of

change

of trie

angle

at any site with trie pressure

is a constant, A.

Or, altematively,

we assume that trie

fiuctuating

part of this

quantity

is absorbed in trie randomness of trie thresholds. A site1 will be able to support trie pressure p

only

if trie

following

condition is met

(vi+1 2vi

+ vi-i +

AP

< t~

(1)

Since A can be seen as

defining

trie scale for pressure, we will in trie

following

set A

= 1.

Therefore,

trie pressure necessary to move trie interface will read

p =

minlti

+

(2vi

vi-i

vi+i)1 (2)

We do not include trie

description

of trie fiow

(we neglect

trie viscous

forces),

and as in trie invasion

percolation

model and in trie CR

model,

we atm at

modelling only

trie

quasistatic

limit.

Therefore,

we assume

that,

at each time step, trie pressure is

adjusted

to trie threshold value of equation

(2).

This

corresponds experimentally

to a control of trie fiow rate rather than trie pressure. Trie evolution of trie interface is considered as

irreversible,

and thus trie interface

is not allowed to recede from an invaded area.

Once a condition for

overlap

is

satisfied,

say at

site1,

trie interface is

moved, by increasing

%

by

an increment d~, and a new threshold

t[

is

picked.

~~~ÎÎ~~~

(3)

t~-t

~

The

displacement

d~ is chosen at random from a uniform distribution over trie interval [dm,n,

dmax].

To check trie elfect of

having

a range of

possible jumps,

we will consider in trie

following

two cases: either dm,n = o, or dm;n = dmax m trie latter case, trie interface

always

lie on a

lattice, y~/dmax being

integer valued. Trie ratio =

tmax/dmax

is trie

only

(8)

free parameter of trie model. It determines how fast trie

"memory"

of a

given

conformation vanishes. We will show below that this parameter

only

affects some aspects of trie model when

àmin " àmax.

Trie

important

features are 1) that

pinning

is taken into account, with a

qitenched

character

(trie

threshold t at a

given

site does not

change

with

time), 2)

trie

propagation

is qitasistatic

(trie

interface is moved at one and

only

one site

during

each

elementary step).

Trie model we

bave defined here shares some similarities with other

approaches

such as those

developed by

Kessler et ai. [7] and Parisi [8] in

particular. However,

trie second condition

diflers,

in trie

sense that a constant

driving

force was

imposed

in both references rather than a controlled

flow. This diiference appears to be

significant

since at

large

flow rate, trie interface

propagation

is

expected

to be described

by

trie

Kardar-Pansi-Zhang equation,

1e. it should

belong

to a

diflerent

universality

Mass.

Both of trie above mentioned features bave been included in a model introduced

by Sneppen ("model

A" of Ref.

[9]).

Trie

only

very minor dilference between this mortel and the

one we bave defined above concems an additional rule

imposed by Sneppen

that trie

slope

of trie interface should

only

assume two

possible

values -1 and 1. This constraint is enforced as

an additional rule. This is in contrast with trie hmit we bave mentioned earlier - for trie lattice version of our model dm;n

=

dmax.

In trie latter case, trie constraint y~ y~-1

naturally

results from trie

updating

rule.

This model is also

extremely

close to a mortel which bas been introduced earlier

by

Zaitsev

[loi,

in order to model trie

propagation

of dislocation lines in a

crystalwith impurities

which act as

pinmng sites,

in a low temperature

regime.

Trie mortel was then named trie "Robin Hood"

model, RH,

and thus we will trie saine

terminology.

In fact trie RH model is very close in its definition to another model which bas received a lot of attention

recently.

It is a cellular automaton model introduced

by

Bak et ai. [16] to illustrate trie concept of

"self-organized criticality". Many

a variant of this model bave been

considered,

and dilferent

applications

bave been discussed

ranging

from

sandpile

avalanches to trie

large

scale structure of trie universe. Trie basic features however of this model are trie

following:

on each site1 of a

regular

network

(for comparison

with trie RH

model,

a one dimensional line is to be

considered)

a variable z~ can assume a few discrete values which increase very

slowly

in time

land

in an

irregular

fashion to introduce a

noise).

Above a threshold z~ > z~, often considered to be

independent

of trie site and constant with time, trie site1 relaxes to a lower value z~ - z~ A and

simultaneously,

trie

neighbormg

sites

j

of1 experience an increase

z~ - z~ + B where B

=

A/n

if n is trie number of

neighbors(1).

If we now interpret z as trie local curvature m RH model then trie local front evolution

equation (3)

appears to be identical as in trie SOC model.

Hence,

trie dilference with usual SOC is trie

heterogeneous (and quenched)

nature of trie threshold.

Similarly,

it is

possible

to draw a

correspondence

with friction models such as trie famous

"Burridge-Knopolf"

model introduced in trie 6o's and which bas

recently

been trie

subject

of an intense

activity

[15]. In this

model,

a linear chain of massive

blocks,

connected

by

elastic spnngs, is

subjected

to a

driving

force

along

trie chain direction.

Moreover,

friction of trie blocks with their support

plane

is described

by

a

velocity weakening

law of

friction,

and

a maximum

(homogeneous)

static force

they

cari sustain. Trie

specific

form of trie

velocity dependent

friction law is not believed to be fundamental as

long

as it is

velocity-weakemng.

Trie most fundamental dilference between this mortel and the RH model is that inertial eifects

are descnbed. Trie motion in finis case bas been shown to be

chaotic,

with a very

large

(~ Violation of trie latter relation has also been investigated in "non-conservative" models. Critical exponents are observed to be dependent on the parameter (A

In -B)

but qualitatively, the phenomenon

is unchanged.

JOURNAL DE PHYSIQUE T 4 " 4 APR'L 1994 0

(9)

distribution of

slip

events, which involve a number of blocks

ranging

from one to trie entire chain. Trie distribution of trie size of

slipping

blocks in one event shows a

power-law

behavior for small sizes which can be

compared

with trie burst size distribution discussed below and an additional contribution from events very close to trie system size. Trie latter seems to be

specific

of trie inertia of trie blocks.

In trie

following,

we will

analyse

trie results of extensive numerical simulations.

System

size varies in trie range L = 64 to L = 1024. A "time" parameter is introduced so that an interval of 1

corresponds

to L individual moves in a system of size L

(on

average one move per unit

length during

one time

step).

This unit of time is sucl~ tl~at on average a volume

(dmax

+

dm;n)L/2

is

injected.

Tl~e time range varies

according

to what property is examined. In order to

study

trie

early development

of trie

roughness,

trie time

laps

is chosen to be at most

equal

to trie

lengtl~.

For

analysing

tl~e front structure at a fate stage time, tl~e front is first grown for a time wl~icl~ ensured tl~at most

early

stage features bave died

off,

and then tl~e furtl~er evolution is

followed over a

long period

of time. Tl~en ail tl~e data collected are

averaged

over

independent

realizations

(up

to loo realizations for L

= 1024 and t = 1024 (1.e. a total of 10~ individual

moves).

Most of tl~e simulations are

performed

witl~

tmax/dmax

= 5, and dm;n

= o.

Trie results are

presented

in trie

following

way: first we will discuss tl~e

geometrical

aspects

of trie invasion front, then we will report trie

analysis

of trie pressure

signal. Finally,

we will

investigate

trie influence of various parameters used in trie definition of trie model

(ratio

of

maximum threshold over maximum

displacement tmax/dmax, amplitude

of tl~e

displacement

interval dmax

dm,n)

and discuss in

particular

a transition towards a faceted

growth regime.

Conceming

tl~e

geometrical

aspects of trie front

development, figure

3

gives

a

qualitative picture

of trie front geometry at diiferent times for

= tmax

/dmax

= 5, dmax = 1 and dm;n

= o.

Figure

4 shows

qualitatively thjt

trie parameter does non seem to

play

any

significant

role when dm;n = o.

However,

when trie interface is constrained to lie on a

lattice,

1-e- dm;n

=

dmax,

trie situation is diiferent. For > 1, we find

again

a similar pattem, as for

figure

3, but when

approaches

1, trie

underlying

discretisation of y becomes much more visible. A little above 1, trie interface consists of

straight

facets with

slopes

-1, o or 1, and thus it can be cast in trie

general

framework of Solid-On-Solid models.

Figure

5 shows an example of such a situation for

= I.oS. For < 1, trie interface is

always straight

if one starts with a

straight

line. If trie initial

configuration

is a sawtooth

profile

y

assuming

trie values o and

1/2

for odd and

even

index1respectively,

then trie value of wl~icl~

corresponds

to a facetted

regime

is 0. It is

interesting

to note tl~at in tl~e

original

CR model for a small

disorder,

tl~e lattice structure of tl~e support of trie disks also becomes apparent and tl~e interface is facetted in a similar way

as m trie

example pictured

in

figure

5.

Starting

from a fiat

front,

tl~e

roughness

first increases witl~ tl~e

injected

volume and tl~en it saturates and becomes

independent

of lime as

usually

seen in sucl~ models. Tl~e widtl~ of tl~e front w is written [31] in a

scaling

form w

= L"

ifi(t/L°/~)

witl~ a

scaling

fucntion ifi wl~ich

assumes trie

followmg asymptotic

behavior:

ifi(x)

c~ x° for x < 1 and

ifi(x)

c~

x~

for x » 1.

Therefore trie two important

scalings

of trie front are trie

steady

state

regime

w c~

L",

and trie

early

lime behavior w c~

t~.

In sections 4 and 5 we will first discuss trie features of trie

fully developed

front as it is trie easier to

analyze expenmentally.

Then we will tum to trie

early

stage

regime

in section 6.

4. Structure of tl~e front in tl~e

steady-state regime.

We consider trie

profile (y~)

for very

large

lime so as to ensure that we are m a

steady

state

regime.

In order to

mvestigate

trie

self-affinity

of trie

front,

we used two diiferent methods:

(10)

~= 5.oo ~= ios

Fig.

3

Fig.

4

Fig. 3. Illustration of the front geometry at dilferent limes for

= 5, dmax

" 1 and dn~;n = 0.

Periodic boundary conditions are implemented in the horizontal direction. The initial geometry is the bottom fine. The system size is here 128, and the last interface shown on the figure was drawn at lime 128.

Fig. 4. Same as figure 3 for a dilferent set of parameters: = 1.05, dmax = 1 and dn~;n " 0. No striking dilference with figure 3 is visible.

1) window measurement of the

roughness, 2)

power spectrum of trie front. Trie results are discussed in trie

following

subsections.

4.1 ROUGHNESS ANALYSIS. Let us first report trie results of trie first method. We measure trie

roughness

of trie front over windows of varying

lengths.

Let à be trie window size. For each

starting point, 1, we define trie two estimates of trie

roughness

w2(1, à)~

=

~2 ~j y)16 £ A/à

~<~<i+à

<~<i+à

(4)

wm(1, à)

= max

(A)

mm

(A)

i<j<1+6 1<j<1+6

We then average w2 and wm for fixed à over ail available

starting positions

1,

W(à)

= lW(1,

à))1 (5)

For a self-affine

profile,

trie

roughness depends

on trie window size à as a

power-law,

wc~ô", (6)

(11)

~

= i 05

Fig. 5. Same as figure 3 for a dilferent set of parameters: = 1.05 and dmax

= dmin # 1. The front

now lies on a lattice which is clearly apparent on the figure. When À approaches 1, the model tends to a Solid-On-Solid model, with facets of slope -1, 0 or 1 without having to impose this condition

artificially.

where a is the

roitghness

e~ponent [35]. Trie data used to compute this

roughness

are relative to a system size of L =512, first grown for a lime t = 2048

(during

which no data is

collected).

Then further 4096 lime units are used to measure trie

roughness

every 64 lime steps. A total of 100 such

samples

were

generated

and

averaged

upon. We limited trie maximum value of à to 100 in order to avoid an artificial saturation which would result from an

undersampling

for

large

window sizes

(too

few

independent windows).

Figure

6 shows trie evolution of both estimates of trie

roughness

as a function of trie window

size in a

log-log

scale. Trie second moment of trie

height

distribution w2 shows a nice power-law behavior with an exponent a = o.85. A very

slight upward

curvature is

detectable, although l~ardly

visible on trie

plot.

Tl~e wm estimate of tl~e

rougl~ness

also shows a

power-law

behavior

but with a

langer

downward curvature. Trie best

regression

line

gives

an estimate of a m o.88 for à > 20

(whereas

a best fit over trie entire range gives a m

o.92).

From trie curvature of

both

estimates,

it seems

likely

that trie

slopes

of these two sets of data bound trie value of a.

Tl~us,

tl~e use of tl~is metl~od leads to tl~e final estimate

a m o.86 + 0.03

(7)

We note tl~at albeit tl~e

quality

of tl~e lits is quite

satisfactory,

there exists a marked size- eflect. For a smaller system size, very

good

lits witl~

power-laws

are obtained over tl~e entire range but with a smaller exponent in

particular

wl~en w2 is used. For L

= 128, trie

roughness

exponent is measured to be o m 0.75.

This result is consistent with trie estimates of a as

given by Robbins,

1-e- 0.75 in reference [29] or 0.81 as a later estimate m reference [30], which was obtained

using

a similar method

(12)

2.5

w~(ôi

2.0 W~(ôi

m 1.5

lOÎ j Éi 1-Ù

o.5

ù-ù

ù-ù 0.5 0 1.5 2.0

log~~(à)

Fig. 6. Roughness

w(à)

us. window size à for the long time regime of trie invasion. Trie two data sets refer to the two estimates defined in equation (6); (o) for w2

là)

and

(+)

for

woo(à).

The system size is 512, and the other parameters are = 5, dmax # 1 and dmin " 0.

with trie w2 estimate. In reference [7], a value of o.75 is mentioned

although

it is obvious from trie data shown in

figure

1 that a

power-law

fit is non quite

satisfactory. Experimentally,

there exists some scanner in trie determmation of a, trie values

reported

in trie literature are o.73 [20], o.91

[22],

o.81 [21] and o.63 [26]. At low

capillary numbers,

He et ai. [23] obtained a broad

scatter in trie determmation of trie exponent in trie range o.8 to o.9.

in most studies of trie

scaling

of

front,

trie

pair

correlation function or variants of it such

as trie two quantities w2 or wm introduced in this subsection is trie

only

feature which is studied in order to assess trie self-affine geometry of trie front. This is however a

dangerous procedure

because of trie

following

remark: it is

always possible

to consider self-affine

profiles

with a

roughness

exponent

larger

than or smaller than o. This can be done e-g-

through integration (resp. derivation)

which increases

(resp. decreases)

trie

roughness

exponent

by

one.

Nevertheless,

it may be shown

mathematically

that trie method used above cannot reveal an exponent

larger

than 1 nor smaller than o. In practice, trie limitation is even more severe.

As soon as trie

roughness

exponent of a

profile

is

larger

than o.8, trie measured value

using

a

w2 or wm method lies

always

in trie range o.8 to

o.9,

for ail values of trie

original

exponent [36]. Trie

forger

trie system size, trie

forger

trie measured value

(~). Thus,

finis method cannot

be used to

quantify accurately

trie

roughness

exponent, but rather to establish a lower bound.

We bave thus used another measure of trie geometry of trie front: trie power spectrum.

4. 2 FOURIER ANALYSIS oF THE FRONT. Trie front structure con aise be studied

through

trie power spectrum of trie

profile P(k).

Trie square modulus of trie Fourier transform of trie

(~) A simple illustration of this is given by applying the analysis method to the deterministic

parabolic profile y

=

~~. A back-of-the-envelope calculation gives

wm(à)

= ôL. Thus, the scaling

of wm with à at fixed L grues an exportent 1, whereas for à

= L, the scahng of wm with L gives the exponent 2, 1.e. the physically relevant value. A similar elfect can also be shown for the other roughness estimate w2.

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