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MEASUREMENTS OF UV -B SPECTRAL IRRADIANCE BEGINNING OF A REGIONAL NETWORK

J.L.Bocquet, E.Pachart, C.Brogniez, J.Lenoble, Universite des Sciences et Technologies de Lille

59655 Villeneuve d'Ascq, France D.Gillotay, D. Bolsee

Iinstitut d' Aeronomie Spatiale de Belgique B-llS0 Brussels, Belgium

ABSTRACT

The University of Lille has developed an instrument to monitor the solar UV irradiance. After many improvements, consecutive to European intercomparison campaigns, it is installed at the top of the LOA building at Lille. This spectroradiometer is planned to take part in a regional network involving, among others, France and Belgium. As validation test for such a network, comparisons of measurements performed, in different conditions, simultaneously by LOA at Lille and by IASB at Brussels have been performed and presented here.

1. INTRODUCTION

The impact of the UV-B (280-315 nm) potential trend on the biosphere is an important topic which is intensively studied since the end of the eighties. Monitoring networks have been deployed in many countries and continents. In Europe, the variability of the meteorological conditions from North to South and East to West is an important difficulty to achieve a global interpretation of the European UV climatology. Plans are therefore currently considered for regional networking including, for instance, a Dutch- Belgian-French dense network.

We present here several comparisons made with spectroradiometers operating by LOA, Lille and by IASB, Brussels, SO km far from Lille. We compare (i) measurements obtained by both instruments located at IASB and (ii) measurements with one instrument located at Lille and the other one located at Brussels. In the first case there is an excellent consistency between the measurements. In the second case a good agreement is found only for stable meteorological conditions.

2. DESCRIPTION OF THE INSTRUMENTS

2.1 The French instrument

The instrument used at the University of Lille to monitor the solar UV irradiance, is a Jobin Yvon

IRS '96: Current Problems in Atmospheric Radiation

Smith and Stamnes (Eds.) ISBN 0·937194-39-5

890

spectroradiometer which has undergone several modifications. It participated in two European intercomparison campaigns in Garmisch-Partenkirchen, Germany, in July 1993 (Gardiner and Kirsch, 1995) and in Ispra, Italy, in May 1995, and has been further improved after this campaign; it is presently operating regularly at the top of the physics building of Lille University at Villeneuve d' Ascq (50.65° N - 3.1° E ) since February 1996. The characteristics and performances of the instrument are presented in table l.

The main improvement it has undergone is the temperature stabilization (within 0.1 degree).

2.2 The Belgian instrument

One of the Belgian instruments is also a temperature stabilized modified Jobin Yvon H IOD spectroradiometer whose characteristics are reported in table 1. The instrument installed at IASB (50.So N - 4.4°

E) is performing measurements since April 1993 (Gillotay, 1996). The other one is an Optronics 754 presently under validation.

Spectrometer

type

Focal length (nm) Gratings

concave holographic lines/mm

Bandwidth FWHM(nm) step (nm) usual finest

Usual

r~nge

(nm) from

to

Direction of scan Scan duration (s) Diffuser Detector

type Weatherproof Automatic

LOA J&Y DHlO 100 two 1200 0.8 0.5 0.05 280 450

UP

500 Teflon PM Hamamatsu R4220P ves yes

IASB J& Y modified DH10 100 two 1200 0.49 0.5 0.05 210 680

UP

400 Teflon PM Hamamatsu R292 yes yes

Copyright OA. DEEPAK Publishing All rights reserved

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UV RADIATION MEASUREMENTS AND MODELLING

Temperature

Stabilized optics 301 K yes

Dark ClUTent yes yes

removed

Stray light yes yes

removed

Radiation standard Oriel NIST

Main Lamp (W) 1000 1000

Secondary lamp no 4

Table 1. Specification of both instruments

3. COMPARISONS

OF SIMULTANEOUS MEASUREMENTS The two spectroradiometers have been separately calibrated, the French one with an Oriel standard lamp, the Belgian one with four NIST standard lamps (FEL lOOOW). Moreover, after the July 17 comparison the USTL instrument calibration was also verified by means of the Belgian standard lamps.

Comparisons of the irradiance measurements have been conducted in two different manners:

(i) the instruments were both located at the same place, at Brussels,

(ii) the instruments were located in places separated by 80 kIn, one installed at Villeneuve d' Ascq, the other at IASB.

In both cases the scan step was the same for the two instruments (0.5 nm) and the measurements occurred at approximately the same time (within a few seconds in the UV-B range).

3.1 Instruments at the same location

We present first the comparison of the measurements performed at lASB on July 17, 1996.

Figure la shows the spectral irradiance measured by both instruments at 1215 UT from 280 to 450 nm, for a the solar zenith angle (SZA) of 30.24°.

The general consistency looks good.

E 1600

..e 1400

... ~ ... f··· .: ...

+ ... -: ...

~

... : ...

~

..

~ .!

1200 1000 800 600 400 200

... ~ ~ .. _ .. ~~ 1 .... I ... f ..

m . .

+ ... i '. :

:::::::::r::::::I::::::r:::::::r··::·· t:::··· F···

r· .

···r···r·· .... : .. r···r···-r···

:::::::::r:::: ···t:·:::::·r::::::·j::::::::r:::···r:::::::r::::::r::

o

~~~~~~~~~~~~~~

280 300 320 340 360 380 400 420 440 wavelength (run)

Fig. la. Spectral irradiance measurement comparison.

Brussels: July, 17th 1996. 12h15 UT SZA: 30.24°

891

The small differences appear more clearly on the ratio of the IASB to USTL measured irradiance shown in Figure Ib (light line). It exhibits oscillations due to different bandwidth of the instruments (see Table I) and to the wavelength calibration. The thick line represents the ratio after smoothing. The measurements agree within 5 % for wavelengths larger than 295 nm.

For shorter wavelengths the discrepancies maybe related to large uncertainties due to the very low signal level.

1.4

1.2

. .

. .

0.8

...

- · · ·

...

.

...

. . - . . .

..

-

...

.

~

. . ... . . .

-.

- . .

:

... . .

:

- . .

: .. .

0.6

1

~ !

1 1 : : :

. ... r···r···T·· · ···T···r···l··· ··t···T ..

0.4

280 300 320 340 360 380 400 420 440 waveleogtb (om)

Fig. lb. July, 17th 1996 12hl5 UT SZA: 30.24°

ratio (lASB/LOA)

Figure 2 presents the ratio obtained later on the same day at 1630 UT, with SZA = 61.6°. The consistency between the measurements is again quite good, the ratio remaining close to unity, within 5 %.

1.6 ,...~~~~ ... ~~~ ... ~~~...,...,

::::1· 1 .IJ....r·· ;;:

o. 6

... ~ ... :

...

~ ... ,. ... ! ... .,. ... : ... ~ ... .

l j j ~ 1 1 1 l

0.4

L...:I~...:... ... .:...:. ... ...:...~-'-'-...:.~....:...J

280 300 320 340 360 380 400 420 440 waveleogtb (om)

Fig. 2. July, 17th 1996 16h30 UT SZA: 61.6°

ratio (IASB/LOA)

These error limits are in close agreement with

those observed during the previous European

Intercomparison Campaigns (Gardiner et aI., 1993,

Gardiner and Kirsch, 1995).

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892 IRS '96: CURRENT PROBLEMS IN ATMOSPHERIC RADIATION

The irradiances integrated over the UV-B spectral range are drawn in Figure 3a versus time, two wavelength intervals are considered: 280-315 nm and 280-320 nm. The erythemal dose, which is defined as the integral over 280-400 nm spectral range of the measured spectral irradiance weighted by the erythemal action spectrum integral (McKinlay and Diffey, 1987) is also shown in Figure 3a. In the three cases the IASB and USlL measurements are in very good agreement.

Figure 3b shows the IASB/USlL ratios obtained for the three cases. The ratios are very close to unity up to 70°.

SZA for the UV-B irradiances. Above 70°, we have a disagreement which increases more and more, probably due, on the one hand to the unperfected synchronization and, on the other hand, to the difference in the cosine responses of both instruments. For the doses the ratio is close to unity up to 80° SZA.

)' zoo

~ a

~ 150

ti ~ ..

100

.g

~

1 ..

50

.c ~

..

0

~

4 6 8 1 'TI~ (ur)14 16 18 20

Fig. 3a. Erythemal dose measurement comparison.

Brussels: July, 17th 1996

1.2 IT"~~""'~-'-'-~~~~""-~~"""-~"'"

0.8

--.8:..-

1';U~~UUU

.mmu;m1m.muuJuu::uumtmm ... u~ .... ummu·.·. ':~ __ .. ':~: __

0.6

0.4

--....-lAlSD/LOA l~ao to 315 Dm) _ _ lASB!LOA (280 to 310 om)

•. ____ .IASBILOA (e..,tbemal dOle)

0.2

u"~~~~~~~~~~~~~~~~~~~

30 40 50 60 70 80

Solar zenithal angle (degree)

Fig. 3b. UV -B irradiance and erythemal dose

measurement ratio (IASBILOA) 3.2 Instruments at different locations

90

The first two following comparisons were achieved on March 27th, 1996 at 1045 UT, and on April

16, 1996, 1430 UT, by clear sky conditions. The SZAs were slightly different for the two instruments: 49.68° at Villeneuve d'Ascq, 49.52° at Brussels in the first case, and 52.13°, 52.89° respectively in the second case.

Figures 4a,b show the ratio of the IASB to USlL measurements on the two dates. We still have a good agreement between the measurements, within 10

% for wavelengths larger than 320 nm and within 20 % for the shorter wavelength range, 305-320 nm.

1.6

I .I . .

1.4 1.2 1 0.8 0.6 0.4 0.2

o

···j···-j-···t···x.·j···

=:jLtLtttt

.

: : : : : : :

~ ... m~ .. m .. +um···l·mm·tuu ... ! .. um··tuum+uuuul·m

280 300 320 340 360 380 400 420 440 wavelength (nm)

Fig. 4a. Spectral irradiance measurement comparison between Villeneuve d'Ascq and Brussels. March, 27th

1996 1Oh45 UT. Villeneuve d'Ascq: SZA 49.68° . Brussels: SZA 49.52° ratio (lASBILOA)

1.4 1.2

0.8 0.6 0.4 0.2

··T···(···j····.Ll···Pt·:::::::>r::::·!:t:: . . . . . .

. . . . . . .

,

o ilrlilf;

280 300 320 340 360 380 400 420 440

wavelength (nm)

Fig. 4b. Spectral irradiance measurement comparison between Brussels and Villeneuve d'Ascq. April, 16th 1996 14h30 UT. Villeneuve d'Ascq SZA: 52.13°.

Brussels SZA: 52.89°. ratio (IASBILOA).

The agreement is poorer for the last comparison conducted during a variable cloudy day.

The example of ratio, drawn in Figure 5, exhibits large

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UV RADIATION MEASUREMENTS AND MODELLING

variations, with values reaching 1.4 at the end of the scan period, corresponding to more cloudy sky at Villeneuve d'Ascq. The apparent discrepancies are therefore quite justified.

1.8 ,...--.--,-~...,...~...,,...,....,...,...,-...,...~.,...,,...,....,...,...,-~

1 6 ' , . . . . .

. ···T···r···T···!"···T···T···r··· ..

1 .4

···j···l···r···l···t···j···r··· r .

;:;~r::;:~il

0.4 L...o---.:..~...:...~..:...,...:.~...:...~..:...:.~~

280 300 320 340 360 380 400 420 440

wavelength (nm)

Fig. 5. Spectral irradiance measurement comparison between Brussels and Villeneuve d'Ascq. June, 11 th 1996 15h30 UT. Villeneuve d'Ascq SZA: 50.74°.

Brussels SZA: 51.88°. ratio (IASB/LOA)

4. CONCLUSION

We have compared in this paper the spectral irradiance measurements obtained with two instruments located first at the same place, and then separated by 80 km.

The excellent agreement found in the first case and in the second case by clear and stable meteorological conditions demonstrates the ability of both instruments to measure the UV spectral irradiance.

The differences observed by unstable weather conditions confirm the UV spatial variability and demonstrate the difficulties to give a global representation of the UV -B climatology even for a small geographic area.

The Belgian and French spectroradiometers are currently involved in a Dutch-Belgian-French network covering a relative small area of N.W. Europe with stations distant of no more than 200 km. A looser network covering the French territory with three stations (Lille, Brian\(on and maybe Toulouse), distant by about 500-800 km is planned.

ACKNOWLEDGMENTS

This study was partially supported by European Union (contract #EVSV -CT93-0353).

893

REFERENCES

Gardiner B.G., Webb A.R., Bais A. E, Blumthaler M., Dirmhirn I., Forster P., Gillotay D., Henriksen K., Huber M., Kirsch P.J., Simon P.C., Svenoe T., Weihs P. and Zerefos C.S., 1993, European intercomparsion of ultraviolet spectroradiometers, Environ. Technol., 14, 25-43.

Gardiner, B. G. and P. J. Kirsch, 1995: Setting Standards for European Ultra-violet spectro- radiometers. , Air pollution research report 53, Gillotay D., 1996, UV monitoring in Belgium: Past,

present and future. in Measurements and Trends of Terrestrial UVB Radiation in Europe, (Ed. B. L.

Diffey), pp. 41-53.

McKinlay, A. F. and B. L. Diffey , 1987 : A reference action spectrum for ultra-violet induced erythema in human skin. In human exposure to ultra-violet radiation: risks and

regQ.Wtion~.

PassIer and B. F. M. Bonsnajakovic eds.) Elsevier,

Amsterdam, 83-87.

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