MASTER of PHYSICS Examination
Lecture : Ultrafast phenomena and optoacoustics (P. Ruello)
Part 1 : WITHOUT DOCUMENT
Heisenberg relation :
1-‐ Localization time :
We consider the two electronic structures depictured below. The grey area corresponds to occupied levels. Give an order of the localization time of an electron in the vicinity of a cation for both electronic structure for the band of 10eV and 0.5ev width.
2-‐ Interaction time between electrons
What is the typical energy of the Coulomb interaction between two electrons ? What is then the typical interaction time
3-‐ Interaction time between an electron and a phonon
What is the typical energy of an optical phonon of 3THz ? Deduce the typical time of interaction between an electron and that optical phonon.
!"#$%
&#'()*+%,-%
,../0)#1%
(*2*#(%
34%%
#'#56+%
"78#$%
34%%
#'#56+%
What is the typical energy of an acoustic phonon of 50GHz ? Deduce the typical time of interaction between an electron and that acoustic phonon.
Which process among electron-‐acoustic phonon and electron–optical phonon is the fastest process ?
4 Femtosecond Pump-‐probe setup
The objective of the question is to describe the principle of the optical pump-‐probe method.
Explain the different elements shown below (fill the boxes for examples).
Part 2 WITH DOCUMENT
Electronic pressure and optoacoustics
1-‐ We consider a free electron gas at 3D (N electrons in a volume V) according to the Sommerfeld model. The metal will be considered as isotropic. The lattice is cubic with a lattice parameter a=0.2nm. Each atom provides 2 conduction electrons. The molar mass is 80g/mol. The longitudinal acoustic sound velocity is 5000m/s.
-‐ give the energy of the free electron
-‐ what is the concentration of conduction electrons in this metal ? -‐ give the wave function form of a free electron
-‐ considering the Born Von Karman boundary limits, give the density of state g(k)
!L
!!
!
!!
!
!!
!
!!
!
!!
!
!!
!
!!
!
!!
!
-‐ Detail the calculation leading to g(E) : g(E)= V
2!2 (2m*
!2 )3/2 E -‐ calculate EF.
3-‐ Considering the definition of the pressure P=-‐(dE/dV)N, calculate it for a quantum free electron gas (T=0K). Give an estimate of this pressure.
(question 4 to 7 are independent to previous questions)
A femtosecond laser excites a metal giving rise to a rapid increase of the electron gas pressure (following model of question 3 that we assume to be valid). The pump light penetrates beneath surface over a distance L=10nm according to the profile P=P0exp(-‐
z/L).
4-‐ What is the typical acoustic frequency which is generated by the femtosecond laser ?
5-‐ The maximum electronic pressure on the surface is P0=1GPa. Considering Newton Law, what is the force F imposed to the atoms ? Give the numerical value of F for z=0.
6-‐ Considering this metal has a longitudinal sound velocity of 5000 m/s. Deduce the elastic constant C characterizing the elastic interatomic force. Deduce the lattice parameter change Δx induced by the electronic pressure for atoms on the surface (z=0).
Deduce Δx/a.
7-‐ If we consider the photoelastic effect with Δn=P×(Δx/a), where P is the photoelastic coefficient with P= 1 here, what will be the order of the change of optical reflectivity induced by this photo-‐induced acoustic wave ? Can we detect directly this optical reflectivity change by a photodiode ?
!"#!$
%$ &$
'()*+$