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HAL Id: inria-00384366

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Preprint submitted on 16 May 2009

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REGULARITY ANALYSIS FOR SYSTEMS OF REACTION-DIFFUSION EQUATIONS

Thierry Goudon, Alexis Vasseur

To cite this version:

Thierry Goudon, Alexis Vasseur. REGULARITY ANALYSIS FOR SYSTEMS OF REACTION- DIFFUSION EQUATIONS. 2009. �inria-00384366�

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REGULARITY ANALYSIS FOR SYSTEMS OF REACTION-DIFFUSION EQUATIONS

Thierry Goudon1, Alexis Vasseur2†

1 Project-Team SIMPAF–INRIA Lille Nord Europe

& Labo. Paul Painlev´e CNRS–USTLille, Park Plazza, 40 avenue Halley F-59650 Villeneuve d’Ascq cedex, France

E-mail: [email protected]

2 Department of Mathematics University of Texas at Austin

Austin, Texas 78712, USA E-mail: [email protected]

Abstract. This paper is devoted to the study of the regularity of solutions to some systems of reaction–diffusion equations. In particular, we show the global boundedness and regularity of the solu- tions in one and two dimensions. In addition, we discuss the Hausdorff dimension of the set of singularities in higher dimensions. Our approach is inspired by De Giorgi’s method for elliptic regularity with rough coefficients. The proof uses the specific structure of the system to be considered and is not a mere adapta- tion of scalar techniques; in particular the natural entropy of the system plays a crucial role in the analysis.

esum´e. Ce travail est consacr´e `a l’´etude de la r´egularit´e des solutions de certains syst`emes d’´equations de r´eaction–diffusion. En particulier, nous montrons que les solutions peuvent ˆetre born´ees et r´eguli`eres en dimensions un et deux alors qu’en dimensions sup´erieures nous discutons la dimension de Hausdorff de l’ensemble des points singuliers. L’approche propos´ee ici s’inspire de la m´ethode de De Giorgi pour ´etudier la r´egularit´e de probl`emes elliptiques avec des coefficients discontinus. La preuve exploite la stucture sp´ecifique des syst`emes consid´er´es et n’est pas une simple adaptation de techniques scalaires. L’entropie associ´ee naturellement au syst`eme joue un rˆole crucial dans cette analyse.

Key words. Reaction-diffusion systems. Regularity of solutions.

AMS Subject classification. 35Q99, 35B25, 82C70

This work has been done while Th. G. was visiting ICES and the University of Texas at Austin. Thanks are addressed for their warm hospitality and support. We also thank J.-F. Coulombel who read preliminary versions and has suggested many improvements.

A. Vasseur was partially supported by the NSF grant DMS-0607053.

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1 Introduction

This paper is devoted to the analysis of the following system of reaction-diffusion equations

tai− ∇ ·(Diai) =Qi(a), i∈ {1, . . . , p}, Qi(a) = (µiνi)

kf Yp

j=1

aνjjkb Yp

j=1

aµjj , ai |t=0 =a0i.

(1.1)

The equation holds fort0 and the space variable x lies in Ω where - either Ω =RN,

- or Ω RN is a bounded domain with smooth boundary and the system is completed by imposing the Neumann boundary condition

Diai·ν(x)|∂Ω= 0, whereν(x) stands for the outer normal vector at x∂Ω.

Throughout the paper, the symbol denotes the gradient operator with respect to the space variable x only. The matricesDi(x) are required to satisfy

Di L(Ω)N×N

,

Di(x)ξ·ξα|ξ|2, α >0 for any ξ RN, xΩ. (1.2) Let us comment this assumption:

- the analysis below is interesting when there are different diffusion matrices: assuming Di = D, a common value, makes the problem easier;

- there is no regularity assumption on the coefficients;

- the standard uniform coercivity condition is assumed. The case of degenerate coefficients leads to specific difficulties which are beyond the scope of this paper.

Such a system is intended to describe e.g. the evolution of a chemical solution: the unknownai stands for the density of the species labelled by i∈ {1, . . . , p} within the solution. The right hand side of (1.1) follows from the mass action principle applied to the reversible reaction

Xp

i=1

νiAi Xp

i=1

µiAi,

where theµi andνi’s — the so-called stoichiometric coefficients — are integers. The (positive) coefficients kf and kb are the rates corresponding to the forward and backward reactions, respectively. According to the physical interpretation, the unknowns are implicitly non-negative quantities: ai 0. In fact, this property holds thanks to the structure of the system. Indeed, (1.1) can be written

tai− ∇ ·(Diai) +Li(a)ai =Gi(a) (1.3) where the nonlinear functions Gi and Li have the property: if the components ak of a are non-negative then Gi(a) 0 andLi(a) 0. Hence preservation of non-negativity, when starting from a non-negative initial data, can be considered among the a priori estimates of the problem (see appendix for more details).

The main ingredients of our analysis rely on the following properties:

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The mass is conserved. The stoichiometric coefficients satisfy

There exists (m1, . . . , mp)Np,mi 6= 0, such that Xp

i=1

miµi = Xp

i=1

miνi. (1.4)

It implies the mass conservation

d dt

Xp

i=1

Z

mi aidx= 0.

The entropy is dissipated. We setK =kb/kf, then

Xp

i=1

Qi(a) ln(ai/K1/(p(µi−νi))) =kfYp

i=1

aµiiK Yp

i=1

aνii ln

Yp

i=1

aµii

K Yp

i=1

aνii

0. (1.5)

In order to simplify the notations, and without loss of generality, we restrict ourselves to the case mi= 1, kf = 1 =kb.

A crucial role will be played by the quantity µ=

Xp

i=1

µi= Xp

i=1

νi,

where the coefficientsµi andνi are still integers.

In our study of such systems restrictions on the space dimension N and the parameterµappear. One of the most interesting situations we are able to deal with is the following example corresponding to 4 species subject to the reactions

A1+A3 A2+A4. It leads to

Qi(a) = (1)i+1(a2a4a1a3). (1.6) We refer for a thorough introduction to the modeling issues and mathematical properties of such reaction diffusion systems to [11, 13, 14, 19, 20, 21, 23, 28, 31]. Information can also be found in the survey [6]

with connection to coagulation-fragmentation models and in [24] for applications in biology. Let us also mention that (1.1) can be derived through hydrodynamic scaling from kinetic models, see [2].

In this contribution we are interested in the derivation of new L estimates and we investigate the regularity of the solutions of (1.1). Quite surprisingly, the question of global boundedness becomes trivial when the diffusion coefficients vanish. Indeed, considerDi = 0, and a bounded initial value. The property (1.4) implies that for each x fixed, the total mass Pp

i=1miai(t, x) is time independent. Then, the non- negativity of the ai’s implies that each ai is uniformly bounded. Conversely, certain reaction diffusion systems might exhibit blow up phenomena, see e.g. [22, 26], as it is also well known when considering nonlinear heat equations [15, 35]. Therefore global well-posedness and discussion of smoothing effects — that is gain of regularity of the solution compared to the initial data — is an issue.

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Standard techniques can indeed be applied to show the existence of a smooth solution of (1.1) locally in time, with, say, initial data inL1L(Ω). We sketch in the appendix the basic argument that proves the local existence of a smooth non negative solution. The challenging question consists in extending the result on arbitrarily large time intervals. Roughly speaking, this is due to a lack of estimates since the only natural bounds are provided by the mass conservation (1.4) and the entropy dissipation (1.5). In particular, the mass conservation only provides an estimate of the solution in L1 which is not enough for the right hand side Qi(a) to make sense as a distribution! However, by using the tricky techniques introduced in [25, 26], it has been shown recently in [10] that the solutions of (1.1) in the quadratic case (1.6) are a priori bounded inL2((0, T)×Ω) so that the nonlinear reaction term makes sense at least inL1. This non trivial estimate can be obtained by exploiting the entropy dissipation and the non degeneracy of the diffusion coefficients. In [10], using also the arguments introduced in [25], it allows to establish the global existence of weak solutions of (1.1), (1.6). Dealing with higher order nonlinearities or degenerate coefficients the difficulty might lead to introduce a suitable notion of renormalized solutions, see [10] again.

We also mention the recent work [27] where the quadratic system is analyzed with diffusion acting only in one direction. The dissipation property (1.5) is also the basis for studying the asymptotic trend to equilibrium [8, 9] in the spirit of the entropy/entropy dissipation techniques which are presented e.g. in [34] (we refer also to [1] for further investigation of the large time behavior of nonlinear evolution systems using the entropy dissipation).

Our approach is inspired by De Giorgi’s methods for studying the regularity of solution of diffusion equations without requiring the regularity of the coefficients, see [7]. The crucial step consists in estab- lishing aLestimate on the solution. Regularity of the solution follows in a classical way (see appendix).

This approach has been used in [33] to obtain an alternative proof to the regularity results for the Navier- Stokes equation [4, 17] and it also shares some features with the strategy introduced in [29, 30]. It has also been applied to study convection-diffusion equations [18] and regularity for the quasi-geostrophic equation [5]. Here, it is worth pointing out that the proof utilizes strongly the structure of the whole system and the argument is not a mere refinement of a scalar approach. As we shall see however, restrictions appear between the space dimension N and the degree of nonlinearity of the reaction term measured by means of µ. For this reason, the L estimates can be proved in two dimension for the quadratic operator (1.6) or in one dimension considering cubic terms.

Theorem 1.1 We consider the quadratic operator (1.6) (or assume µ= 2). Let N = 2 and suppose that the diffusion coefficients fulfill (1.2). Let a0i 0 satisfy

X4

i=1

Z

a0i 1 +|x|+|ln(a0i)|

dx=M0 <. (1.7)

Then, (1.1) admits a global solution such that for any 0< T T <, ai belongs toL((T, T)×Ω).

Theorem 1.2 Let N = 1 with µ3 and suppose that the diffusion coefficients fulfill (1.2). Let a0i 0 satisfy (1.7). Then, (1.1) admits a global solution such that for any 0 < T T < , ai belongs to L((T, T)×Ω).

We point out that these statements do not require any regularity property on the diffusion coefficients Di which are only supposed to be bounded. As a byproduct, by using the new bound, a direct bootstrap argument shows the global regularity of the solution (see appendix).

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Corollary 1.1 Let the assumptions of Theorem 1.1 or 1.2 be fulfilled. Suppose moreover that the Di’s belong to Ck(Ω) with bounded derivatives up to order k. Then, for any 0 < T T < , the solution belongs toL(T, T;Ck(Ω)). Accordingly forC coefficients with bounded derivatives, the solution isC on (T, T)×Ω.

Such statements could be helpful for investigating the large time behavior: they can be the starting point to apply the strategy developed in [8, 9] and then this would lead to the proof of the convergence to the equilibrium state for large time, with an exponential rate. We do not discuss further this issue which requires a sharp estimate of the bound with respect to the final time T. Instead, we consider the case of higher dimensions: the same method provides information on the Hausdorff dimension (definitions are recalled in Section 4) of the set of the singular points of the solutions.

Theorem 1.3 Let N 3 and µ = 2. We suppose that the coefficients Di are constant with respect to xΩ. Let a0i 0 satisfy (1.7). We consider a solution of (1.1) on (0, T)×Ω. We call a singular point, any point (t, x) having a neighborhood on which one of the function ai is not C. Then, the Hausdorff dimension of the set of singular points of the solution adoes not exceed (N24)/N.

In the next section, we briefly recall the fundamental estimate that follows from (1.5). This bound is used in Section 3 where we adapt De Giorgi’s approach to the system (1.1). Section 4 is devoted to the estimate of the Hausdorff dimension of the set of singularities in higher space dimensions.

2 Entropy dissipation

In the following Sections, we adopt the viewpoint of discussing a priori estimates formally satisfied by the solutions of (1.1). As usual the derivation of such estimates relies on various manipulations such as integrations by parts, permutations of integrals and so on. Of course, such formulae apply to the smooth solutions of the problem that can be shown to exist on a small enough time interval by using classical reasoning for nonlinear parabolic equations (see the appendix). Moreover, these estimates also apply to solutions of suitable approximations of the problem (1.1). Such approximations should be defined so that the essential features of the system are preserved. Hence, let us reproduce the reasoning in [10]: by truncation and regularization we deal with an initial data

a0,ηi Cc(Ω), a0,ηi 0 which converges inL1(Ω) toa0i asη >0 tends to 0 and such that

sup

η>0

Xp

i=1

Z

a0,ηi 1 +|x|+|ln(a0,ηi )|

dxC0

Xp

i=1

Z

a0i 1 +|x|+|ln(a0i)|

dx=C0 M0 <.

Next, let us consider a cut-off functionζ Cc(R) such that 0ζ(s)1, supp(ζ)B(0,2) andζ(s) = 1 for|s| ≤1. Then, in (1.1) we replaceQi(a) by

Qηi(a) =Qi(a)ζ(η|a|), with |a| = q

a21+...+a2p. Accordingly, for any η > 0 fixed, andai L1(Ω), Qηi(a) belongs to L(Ω).

We can show that the corresponding regularized problem admits a unique (non-negative) smooth solution,

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globally defined, see [16, 28]. Therefore, in what follows we discuss a priori estimates on solutions of (1.1):

for the sake of simplicity we detail the arguments working directly on (1.1), but we keep in mind that the arguments apply to the regularized problem as well. In turn, we obtain bounds on the sequenceaηi, which are uniform with respect to η >0. Finally, existence of a global solution satisfying the estimates follows by performing the passage to the limitη0; a detail that we skip here, referring for instance to [10].

We start by discussing the a priori estimates that can be naturally deduced from (1.4) and (1.5). The results here apply in full generality, without assumptions onp, N, µ.

Proposition 2.1 Assume (1.2), (1.4) and (1.5). Let a0i 0 satisfy Xp

i=1

Z

a0i 1 +|x|+|ln(a0i)|

dx=M0 <. (2.1)

We set

D(t, x) =Yp

i=1

aµii Yp

i=1

aνii ln

Yp

i=1

aµii Yp

i=1

aνii

(t, x)0.

Then, for any 0< T <, there exists 0< C(T)< such that sup

0≤t≤T

nXp

i=1

Z

ai 1 +|x|+|ln(ai)|

(t, x) dx +

Xp

i=1

Z t

0

Z

ai2(s, x) dxds+ Z t

0

Z

D(s, x) dxdso

C(T).

If is a bounded domain, this estimate holds for T = +. Proof. As a consequence of (1.4) and (1.5), we get

d dt

Xp

i=1

Z

ai 1 + ln(ai) dx+

Xp

i=1

Z

Diai·ai

ai dx+ Z

Ddx= 0.

Then, the coercivity condition (1.2) means that we can establish the following lower bound Xp

i=1

Z

Diai·ai

ai dxα Xp

i=1

Z

|∇ai|2

ai dx= 4α Xp

i=1

Z

ai2dx.

In the case when Ω is a bounded domain then the conclusion of the theorem follows as Xp

i=1

Z

ai|ln(ai)|dx = Xp

i=1

Z

ailn(ai) dx2 Xp

i=1

Z

ailn(ai)110≤ai≤1dx

Xp

i=1

Z

ailn(ai) dx+p2 e||,

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where here and below, 11M denotes the characteristic function of the set M. In the case when Ω =RN, then the argument proceeds as follows. By using (1.4) and denoting by M the supremum norm of the diffusion coefficients, we get

d dt

Xp

i=1

Z

ai|x|dx = Xp

i=1

Z

Diai· x

|x|dx

M Xp

i=1

Z

|∇ai|dx=M Xp

i=1

Z

|∇ai|

ai

aidx

α 2

Xp

i=1

Z

|∇ai|2

ai dx+M2

Xp

i=1

Z

aidx, by using the standard inequality |rs| ≤r2/2 +s2/2. Hence, we arrive at

Xp

i=1

Z

ai 1 +|x|+ ln(ai)

dx+ α 2

Xp

i=1

Z t

0

Z

|∇ai|2

ai dxds+ Z t

0

Z

Ddxds

M0+ M2

Xp

i=1

Z t

0

Z

aidxds

1 +tM2/(2α) M0.

It remains to control the negative part of the ailn(ai)’s. To this end, we use the following classical argument:

Z

ai|ln(ai)|dx = Z

ailn(ai) dx2 Z

ailn(ai) 110≤ai≤e−|x|/2+ 11e−|x|/2≤ai≤1

dx

Z

ailn(ai) dx+4 e

Z

e−|x|/4dx+ Z

|x|aidx sincesln(s) 2e

sfor any 0s1. We conclude by combining together all the pieces.

3 L bounds

In the spirit of the Stampacchia cut-off method,L bounds of solutions of certain PDEs can be deduced from the behavior of suitable nonlinear functionals. Here, such a functional is constructed in a way that uses the dissipation property (1.5). Let us consider the non-negative, C1 and convex function

Φ(z) =

(1 +z) ln(1 +z)z ifz0,

0 ifz0.

Then, fork0, we are interested in the evolution of Xp

i=1

Z

Φ(aik) dx.

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Lemma 3.1 There exists a universal constant C, such that for every a= (a1, . . . , ap) solution of (1.1), for anyk0, and for any 0st <, we have

Xp

i=1

Z

Φ(aik)(t, x) dx+ 4α Xp

i=1

Z t

s

Z

p

1 + [aik]+2(τ, x) dx

Xp

i=1

Z

Φ(aik)(s, x) dx +C

Xp

i=1

Z t

s

Z

1 +kµ+ (1 +k)[aik]µ−1+

ln(1 + [aik]+)(τ, x) dx where [z]+ = max(0, z) denotes the non-negative part of z.

Remark 3.1 Notice that the universal constant does not depend on the actual solution a nor on k. It is also worth noticing that, in order to make sense of this inequality we need only aµ−1i ln(1 +ai) to be integrable, although it is required to have aµi to be integrable to make sense of the equation (1.1). This point will be very important in the next section. Crucial to the analysis is the similarity of the functionΦ and the natural entropy of the system (1.1).

Proof. Multiplying (1.1) by Φ(aik) and summing yields d

dt Xp

i=1

Z

Φ(aik) dx+ Xp

i=1

Z

Diai· ∇ai Φ′′(aik) dx= Xp

i=1

Z

Qi(a)Φ(aik) dx. (3.1) Then, we observe that (1.2) leads to

Xp

i=1

Z

Diai· ∇ai Φ′′(aik) dx= Xp

i=1

Z

Diai· ∇ai 11ai≥k 1 + [aik]+dx

= Xp

i=1

Z

Di(1 + [aik]+)· ∇(1 + [aik]+) dx 1 + [aik]+

α Xp

i=1

Z

(1 + [aik]+)2 1 + [aik]+

dx

Xp

i=1

Z

p

1 + [aik]+2dx.

Next, we rewrite the right hand side of (3.1) as Xp

i=1

Z

Qi(a) ln(1 + [aik]+) dx

= Xp

i=1

Z

Qi(a)Qi(1 + [ak]+)

ln(1 + [aik]+) dx +

Xp

i=1

Z

Qi(1 + [ak]+) ln(1 + [aik]+) dx,

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where (1.5) implies that the last term is non-positive. We are thus left with the task of estimating Qi(a)Qi(1 + [ak]+)

ln(1 + [aik]+).

To this end, let us consider the polynomial functionP :Rp Rdefined byP(u) =Qp

i=1uνii. Clearly, given u, vRp, we have

|P(u)P(v)|= Z 1

0 P(u+s(vu))·(uv) dsCkuvk Z 1

0 k∇P(u+s(vu))kds where k · k represents for any norm on Rp. As a matter of fact, since the µi’s and νi’s are non-zero integers, we have jP(u) =νjQp

i=1uν

i,j

i whereνi,j =νi ifi6=j and νj,j =νj1. In particular, note that Pp

i=1νi,j =µ1. Therefore, working with the1 norm, we get k∇P(u)k ≤

Xp

j=1

νj Yp

i=1

|ui|νi,j

which yields, by using the convexity of the functionsz7→zνi,j ,

|P(u)P(v)| ≤ Xp

ℓ=1

|uv| × Xp

j=1

νjYp

i=1

|ui|νi,j + Yp

i=1

|vi|νi,j .

Clearly, we have Qp

i=1|ui|νi,j C Pp

i=1(1 +|ui|µ−1) and finally we obtain

|P(u)P(v)| ≤C Xp

ℓ=1

|uv| × Xp

i,j=1

νj(1 +|ui|µ−1+|vi|µ−1).

We apply this inequality with ui = ai and vi = 1 + [aik]+ and we make use of the following simple

remarks

0(1 + [aik]+)µ−1 C (1 + [aik]µ−1+ ),

0ai[aik]++k so that 0aµ−1i C([aik]µ−1+ +kµ−1), ai(1 + [aik]+)1 +ai[aik]+1 +k.

Applying the same reasoning withµi replacingνi, we arrive at Qi(a)Qi(1 + [ak]+)C (1 +k)

Xp

j=1

1 +kµ−1+ [ajk]µ−1+ ,

where the constant C depends on µ and p <. Then, we end the proof by using the simple inequality:

for anyu, v 0, uµ−1ln(1 +v) +vµ−1ln(1 +u)2 uµ−1ln(1 +u) +vµ−1ln(1 +v)

. (As usual we have adopted the convention to keep the same notationC for a constant that does not depend on the solution, even when the value of the constant might change from one line to the other.)

Remark 3.2 We point out that the arguments above do not extend straightforwardly to situations where the unknown a is an infinite sequence, like e.g. for coagulation-fragmentation models (the constant C involves a sum over the reactants).

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Let 0< T < T < and 0< K < be fixed. Set

0< tn=T(11/2n)< T < T, 0< kn=K(11/2n)< K.

Let us denote Un= sup

tn≤t≤T

Xp

i=1

Z

Φ(aikn)(t, x) dx+ 4α Xp

i=1

Z T

tn

Z

p

1 + [aikn]+2(τ, x) dxdτ.

The aim is to show that, for a suitable choice ofK >0,Untends to 0 as n→ ∞ which will yield theL bound.

We start by making use of Lemma 3.1 with 0tn−1 stn tT and we average with respect to s(tn−1, tn). Sincetntn−1 =T /2n, we obtain

T 2n

Xp

i=1

Z

Φ(aikn)(t, x) dx+ 4α Xp

i=1

Z tn

tn−1

Z t

s

Z

p

1 + [aikn]+2(τ, x) dxds

Xp

i=1

Z tn

tn−1

Z

Φ(aikn)(s, x) dxds+C Xp

i=1

Z tn

tn−1

Z t

s

Z

Γ(kn, aikn)(τ, x) dxds

with the short hand notation Γ(k, u) = (1 +kµ+ (1 +k)[u]µ−1+ )) ln(1 + [u]+). Since in the integration domainstn−1 and tT, the last integral can be dominated by

Xp

i=1

Z tn

tn−1

Z T

tn−1

Z

Γ(kn, aikn)(τ, x) dxds T 2n

Xp

i=1

Z T

tn−1

Z

Γ(kn, aikn)(τ, x) dxdτ.

Similarlystn leads to the following bound from below

Xp

i=1

Z tn

tn−1

Z t

s

Z

p

1 + [aikn]+2(τ, x) dxds

Xp

i=1

Z tn

tn−1

Z t

tn

Z

p

1 + [aikn]+2(τ, x) dxds

T 2n

Xp

i=1

Z t

tn

Z

p

1 + [aikn]+2(τ, x) dxdτ.

Hence, for anytntT, we have Xp

i=1

Z

Φ(aikn)(t, x) dx+ 4α Xp

i=1

Z t

tn

Z

p

1 + [aikn]+2(τ, x) dx

2n T

Xp

i=1

Z tn

tn−1

Z

Φ(aikn)(s, x) dxds+C Xp

i=1

Z T

tn−1

Z

Γ(kn, aikn)(τ, x) dxdτ.

Taking the supremum overtntT, we obtain Un 2n

T Xp

i=1

Z tn

tn−1

Z

Φ(aikn)(s, x) dxds +C

Xp

i=1

Z T

tn−1

Z

1 +knµ+ (1 +kn)[aikn]µ−1+

ln(1 + [aikn]+)(τ, x) dxdτ.

(3.2)

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Under reasonable assumptions which cover a wide class of systems, we show that such complex networks generate continuous dynamical systems whose asymptotic behavior can be described