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Bell-Type Inequalities to Detect True n -Body Nonseparability

COLLINS, Daniel Geoffrey, et al.

Abstract

We analyze the structure of correlations among more than two quantum systems. We introduce a classification of correlations based on the concept of nonseparability, which is different a priori from the concept of entanglement. Generalizing a result of Svetlichny [Phys.

Rev. D 35, 3066 (1987)] on threeparticle correlations, we find an inequality for n-particle correlations that holds under the most general separability condition and that is violated by some quantum-mechanical states

COLLINS, Daniel Geoffrey, et al . Bell-Type Inequalities to Detect True n -Body Nonseparability.

Physical Review Letters , 2002, vol. 88, no. 17

DOI : 10.1103/PhysRevLett.88.170405

Available at:

http://archive-ouverte.unige.ch/unige:36788

Disclaimer: layout of this document may differ from the published version.

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Bell-Type Inequalities to Detect True n-Body Nonseparability

Daniel Collins,1,2 Nicolas Gisin,3Sandu Popescu,1,2David Roberts,1and Valerio Scarani3

1H.H. Wills Physics Laboratory, University of Bristol, Tyndall Avenue, Bristol BS8 1TL, United Kingdom

2BRIMS, Hewlett-Packard Laboratories, Stoke Gifford, Bristol BS12 6QZ, United Kingdom

3Group of Applied Physics, University of Geneva, 20 rue de l’Ecole-de-Médecine, CH-1211 Geneva 4, Switzerland (Received 1 February 2002; published 12 April 2002)

We analyze the structure of correlations among more than two quantum systems. We introduce a classification of correlations based on the concept of nonseparability, which is differenta priorifrom the concept of entanglement. Generalizing a result of Svetlichny [Phys. Rev. D35, 3066 (1987)] on three- particle correlations, we find an inequality forn-particle correlations that holds under the most general separability condition and that is violated by some quantum-mechanical states.

DOI: 10.1103/PhysRevLett.88.170405 PACS numbers: 03.65.Ud, 03.67. – a

Quantum mechanics (QM) predicts remarkable correla- tions between the outcomes of measurements on subsys- tems (particles) of a composed system. This prediction is consequence of the linearity of QM, which allows one to build superposition states that cannot be written as prod- ucts of states of each subsystem. Such states are calleden- tangled. Entanglement is at the heart of some of the most puzzling features of QM: the Einstein-Podolski-Rosen argument, the measurement problem, the paradox of Schrödinger cat … . In the past decade, it has been noticed that entanglement is also a resource that allows one to perform tasks that would be classically impossible.

This new, more effective standpoint caused a renewed interest in the study of quantum correlations [1].

The correlations among more than two quantum systems have been the object of several recent studies, also moti- vated by the fact that experiments aimed to check such correlations are becoming feasible. Usually, the structure of correlation has been classified according to entangle- ment. In this Letter, we propose a complementary classi- fication, in terms ofnonseparability. Before entering the technicalities, it is useful to explain why the concepts of entanglement and of nonseparability area prioridifferent concepts. We do this on the simplest case, that of correla- tions between three particles.

The classification through entanglement presupposes that the system of three particles admits a quantum- mechanical description. Thus, any state of the system is described by a density matrix r. To classify a given r in terms of entanglement, one must consider all possible decompositions of the state as a mixture of pure states r 苷P

ipijCi典 具Cij. Then, (i) if there exists a decompo- sition for whichalljCi典are product statesjci1典jci2典jci3典, then r is not entangled at all; that is, it can be prepared by acting on each subsystem separately. For this situation, we use the acronym 1兾1兾1QM. (ii) If all jCi典 can be written as eitherjci12典jc3i典orjci13典jci2典orjci23典jci1典, and at least one of thejcijk典 is not a product state, thenr is entangled, but there is no true three-particle entanglement.

We shall say that r exhibits two-particle entanglement,

and use the acronym 2兾1QM to refer to it. (iii) Finally, if for any decomposition there is at least onejCi典that shows three-particle entanglement, then to prepare r one must act on the three subsystems: rexhibits true three-particle entanglement (acronym 3QM).

It is difficult to establish to which class a given r belongs, because, in principle, one should write down all the possible decompositions ofronto pure states. In fact, to date no general criterion is known. However, we know a sufficient criterion: There exists an operatorM3such that (a) if Tr共rM3兲 .1, then certainly ris entangled; (b) if Tr共rM3兲 .p

2, then certainly r exhibits true three- particle entanglement. The operator M3 is the Bell operator that defines the so-called Mermin inequality [2];

we shall come back to it later.

Theclassification through nonseparability(or nonlocal- ity) does not presuppose that the system of three particles admits a quantum-mechanical description. Rather, we have the following cases:

(i) Each particle separately carries a script l, which determines the outcome of each possible measurement.

When the experiment is repeated, the script can be differ- ent — the script l occurring with probability r共l兲. This is the so-calledlocal variables(ly) model, which we will also denote as 1兾1兾1S. More exactly, in the ly model, the joint probabilitiesPa1,a2,a3兲that an arbitrary experi- mentA1performed on particle 1 yields the resulta1, while the measurementA2performed on particle 2 yieldsa2and the measurement A3on particle 3 yieldsa3, is given by

Pa1,a2,a3兲苷Z

dl r共l兲P1a1jl兲P2a2jl兲P3a3jl兲, (1) whereP1a1jl兲is the probability that when particle 1 car- rying the scriptlis subjected to a measurement of A1it yields the resulta1, and similarly forP2andP3. Note that ly is more general than 1兾1兾1QM. For instance, in ly one can build a state such that the measurement of the spin of particle 1 along both directionszˆ andxˆ gives11with certainty, while such a state does not exist in QM.

170405-1 0031-9007兾02兾88(17)兾170405(4)$20.00 © 2002 The American Physical Society 170405-1

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(ii) The intermediate case, first considered by Svetlichny [3], is a hybrid local– nonlocal model: for each triple of particles, we allow an arbitrary (i.e., nonlocal) correlation between two of the three particles, but only local correla-

tions between these two particles and the third one; which pair of particles is nonlocally correlated may be different in each repetition of the experiment. If we define pi,j to be the probability that particlesiandjare nonlocally cor- related, then in this model

P1,2,3a1,a2,a3兲 苷 X3 k1

pi,jZ

dl关ri,j共l兲Pi,jai,ajjl兲PkAkakjl兲兴, (2) where兵i,j,k其is an even permutation of兵1, 2, 3其. We refer

to this situation by the acronym 2兾1S. Note again that 2兾1Sis more general than 2兾1QM, since we do not require that the two correlated particles are correlated according to QM.

(iii) The last situation (3S) is the one without con- straints: We allow all three particles to share an arbitrary correlation.

It is not evidenta prioriwhether three-particle entangle- ment 3QM is stronger, equivalent, or weaker than 2兾1S.

The proof that 3QM is actually stronger than 2兾1S was given some years ago by Svetlichny [3], who found an inequality for three particles that holds for 2兾1S and is violated by QM. In this Letter, we are going to exhibit a generalized Svetlichny inequality for an arbitrary number of particlesn, that is, an inequality that allows one to dis- criminate n-particle entanglement nQM from any hybrid model k兾共n 2kS.

The plan of the paper is as follows. First, we introduce the family of the Mermin-Klyshko (MK) inequalities [2,4], which will be the main tool for this study. With this tool, we rederive Svetlichny’s inequality for three particles and compare it to Mermin’s. We move then to the case of four particles, and show that the MK inequality plays the role of generalized Svetlichny inequality. Finally, we generalize our results for an arbitrary number of particlesn.

We consider, from now on, an experimental situation in whichtwo dichotomic measurementsAj andA0jcan be performed on each particlej苷1, . . . ,n. The outcomes of these measurements are writtenajanda0j, and can take the values61. LettingM1a1, we can define recursively the MK polynomialsas

Mn12Mn21共an 1a0n兲 1 12Mn210 共an 2 an0兲, (3) where Mk0 is obtained from Mk by exchanging all the primed and nonprimeda’s. In particular, we have

M212共a1a21 a10a2 1a1a022a01a02兲, (4) M312a1a2a30 1a1a02a3 1a10a2a3 2a01a02a03兲. (5) The recursive relation (3) gives, for all1#k #n21,

Mn12Mn2kMk 1Mk0兲 1 12Mn2k0Mk 2Mk0兲. (6) We shall interpret these polynomials as sums of expecta- tion values; e.g., we shall interpretM2as

1

2EA1A2兲1 EA01A2兲1 EA1A02兲2EA01A02兲兴, (7)

where EA1A2兲 is the expectation value of the product A1A2when A1andA2 are measured (note thatA1 andA01 cannot be measured at the same time). We call quantities such asEA1A2A3兲correlation coefficients. We shall look at the values of these polynomials under QM and hybrid local/nonlocal variable models, and show that they give generalized Bell inequalities.

We shall first look at hybrid local/nonlocal variable models. For technical simplicity, throughout this paper we consider onlydeterministicversions of the hybrid variable models, which means that the scriptlin Eqs. (1) and (2) completely determines the outcome of the measurements [i.e., the probabilitiesP1Xxjl兲 and similar are either zero or one]. It is known that any nondeterministic local variable model can be made deterministic by adding addi- tional variables [5]. In addition, we can also use the script lto determine which particles are allowed to communi- cate nonlocally: e.g., for three parties, the probabilities are now given simply by

Pa1,a2,a3兲 苷Z

dl r共l兲Pa1,a2,a3jl兲, (8) where for eachlthe probabilities must factorize as some 2兾1grouping (though not necessarily the same for different l). Now, for any l, the outcomes of all productsA1A2A3 etc. are fixed, and so we can define the fixed quantityMnl. The value of Mn is just the probabilistic average over l of Mnl. Thus, if we can put a bound upon all possible Mnl, then we have a bound uponMn. For example, it can be shown that, for any ly model, Mn #1. This can be easily seen from (3) using a recursive argument, noting that for any script of local variables it holds that either ana0n or an 苷 2an0. In particular, M2 #1 for ly is the Clauser-Horne-Shimony-Holt inequality for two par- ticles [6]. On the opposite side, if we consider the model without constraintsnS, thenMncan reach the so-calledal- gebraic limitMnalg, achieved by setting at11(respectively 21) all the correlation coefficients that appear inMnwith a positive (respectively negative) sign. So, for example, M2algM3alg 苷2.

Turning to QM, since we consider dichotomic measure- ments, we can restrict to the case of two-dimensional sys- tems (qubits) [7]. In this case, the observable that describes the measurement Aj can be written as aj ? s៬ ⬅saj, with aj a unit vector and s៬ the Pauli matrices. The equivalent ofMn is the expectation value of the operator Mn obtained by replacing all a’s by the corresponding sa. It is thus known that QM violates the inequality

170405-2 170405-2

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Tr共rMn兲# 1. More precisely, it is known [4] that (I) the maximal value achievable by QM is Tr共rMn兲 苷2n21兲兾2, reached by the generalized Greenberger-Horne-Zeilinger (GHZ) states 共1兾p

2兲 共j0 . . . 0典 1j1 . . . 1典兲; (II) if r exhibits m-particle entanglement, with1# m# n, then Tr共rMn兲# 2m21兲兾2 [8]. In other words, if we have a state of n qubits r such that Tr共rMn兲 .2m21兲兾2, we know that this state exhibits at least 共m 11兲-particle entanglement. This means that the MK polynomials allow a classification of correlations according to entanglement.

But do they allow also the classification according to nonseparability? The answer to this question: yes for n even, no for n odd. As announced, we demonstrate this statement first forn 苷3, then for n苷4, and finally for all n.

Three particles.— Let us take the Mermin polynomial M3given in (5). We have already discussed the following bounds: M3ly 苷1, M321QM苷 p

2, M33QMM3alg 苷2.

We lack the bound for 2兾1S. This is easily calculated:

Consider a script in which particles 1 and 2 are correlated in the most general way, and particle 3 is uncorrelated with the others. Then we use (3), which readsM312M2a3 1 a03兲 1 12M20a3 2a03兲. For any particular script, as we said above, a3 can only be equal to 6a03. Without loss of generality, we choose a3a03苷 1, whenceM321S 苷 maxM2. Since particles 1 and 2 can have the highest correlation, maxM2M2alghere. In conclusion,M321S 苷 2. Thus, for Mermin’s polynomial,

M321SM33QMM3alg 苷2 . (9) The Mermin polynomial does not discriminate between the deterministic variable models 2兾1S and 3S, and the quantum-mechanical correlation due to three-particle en- tanglement. The deep reason for this behavior lies in the fact thatM3has only four terms: The correlationsa1a2a3, a01a02a3,a10a2a30, anda1a02a03do not appear inM3given in (5). But these correlations are those that appear in M30; thus we are led to check the properties of the polynomial, S312共M3 1M30兲 苷 12共M2a03 1M20a3兲. (10) For both ly and 2兾1S, the calculation goes as follows:

We choose a3a30 苷1, and we are left with S3···

1

2max共M2 1M20兲. ButM2 1M20a1a20 1a01a2, which can take the value of 2 in both ly and 2兾1S. There- fore S3lyS231S 苷1, and this implies immediately S321QM苷 1 since 2兾1QM is more general than ly and is a particular case of 2兾1S. The algebraic maximum is obviouslyS3alg 苷2. We have to findS33QM. As above, we define an operatorS3 by replacing thea’s in the polyno- mialS3with Pauli matrices. On the one hand, we have

Tr共rS3兲 苷 12关Tr共rM2sa30兲1Tr共rM20sa3兲兴# p

2 , (11)

since by the Cirel’son theorem [9] each term of the sum is bounded byp

2. On the other hand, we know [10] that the eigenvector associated to the maximal eigenvalue for such an operator is the GHZ state共1兾p

2兲 共j000典1 j111典兲. For some settings [11], we have具GHZjS3jGHZ典 苷p

2: The bound can be reached; that is,S33QM 苷p

2. Thus, the GHZ state generates genuine three-party nonseparability (non- locality). We note that, in fact, S3 is one of Svetlichny’s two inequalities [the second inequality is equivalent, and is associated to 12M3 2M30兲].

The results for Mermin’s and Svetlichny’s inequalities for three particles are summarized in Table I. We see that combining Mermin’s and Svetlichny’s inequalities one can discriminate between the five models for correlations that we consider in this paper. This concludes our study of the case of three particles.

Four particles.— As above, we begin by considering the MK polynomial M4. Like M2, and unlike M3, the polynomial M4 is a linear combination of the correla- tion coefficients of all measurements. From the gen- eral properties of the MK inequalities [4], the following bounds are known: M4ly 苷1, M4112QMM422QM苷 p

2, M431QM苷 2, M44QM苷2p

2. The algebraic limit is M4alg 苷4(sixteen terms in the sum, and a factor 14in front of all).

Now we have to provide the bounds for1兾1兾2S,2兾2S, and 3兾1S. This last one can be calculated in the same way as above: using (3), we haveM412M3a4 1a04兲1

1

2M30a4 2a04兲; we seta4a04 苷1, and, since we allow the most general correlation between the first three parti- cles, we have maxM3M3alg 苷2. ThereforeM431S 苷 2.

One must be more careful in the calculation of1兾1兾2S and 2兾2S. This goes as follows: Using (6), we have M412M1,2M3,41M3,40 兲1 12M1,20M3,4 2M3,40 兲, where to avoid confusion we wroteMi,jinstead ofM2, withiand jthe labels of the particles. Now,M3,4 1M3,40a3a041 a03a4, and M3,4 2 M3,40a3a4 2a03a04. So, if we allow the most general correlation between particles 3 and 4, these two quantities are independent and can both reach their algebraic limit, which is 2. Consequently, for both 1兾1兾2S and 2兾2S we obtain M···4 苷max共M1,2 1 M1,20 兲, which is again 2 in both cases. So, finally,

M4112SM422SM431S 苷2 ,M44QM苷 2 p

2 . (12)

TABLE I. Maximal values of M3 and S3 under different as- sumptions for the nature of the correlations (see text). The last line is the product of the two values.

3S

ly 2兾1QM 2兾1S 3QM (algebraic)

M3 1 p

2 2 2 2

S3 1 1 1 p

2 2

product 1 p

2 2 2p

2 4

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For four particles, the MK polynomial M4 detects both four-particle entanglement (this was known) and four- particle nonseparability, and is therefore the natural generalization of Svetlichny’s inequality.

Arbitrary number of particles. — For a given number of particlesn, we discuss only the maximal value allowed by QM, that is the case nQM, against any possible partition intwosubsets ofkandn 2kparticles, respectively, with 1# k# n21, that is the case k兾共n2kS. Partitions in a bigger number of smaller subsets are clearly special cases of these bilateral partitions. We are going to prove the following.

Proposition: Define the generalized Svetlichny polyno- mial Sn as

Sn

Mn, n even

1

2共Mn 1Mn0兲, n odd. (13) Then all the correlationsk兾共n 2k兲Sgive the same bound Skn, and the bound that can be reached by QM is higher by a factor

p 2:

SnnQM 苷p

2Snk. (14)

The tools for the demonstration are the generalization to all the MK polynomials of the properties of M2 and M3that we used above: namely, (I) the algebraic limit of Mk is Mkalg 苷2k2MkQMk

p

2 for k even, andMkalg 苷 2k21兲兾2MkkQM for k odd. (IIa) For k even, Mk and Mk0 are different combinations of all the correlation coef- ficients; Mk 1Mk0 and Mk 2Mk0 contain each one-half of the correlation coefficients, and the algebraic limit for both is Mkalg. (IIb) For k odd, Mk and Mk0 contain each one-half of the correlation coefficients. These properties are not usually given much stress, but can indeed be found in [4], or easily verified by direct inspection.

Let us first prove the proposition forneven. In this case, the QM bound is known to beSnQMn 苷2n21兲兾2. As in the case of four particles, to calculateSkn we must distinguish two cases.

(i) For k and n 2k even: in (6), both Mk 1Mk0 and Mk 2Mk0 can be maximized independently because of property (IIa) above; therefore, we replace them by Mkalg. We are left withSkn12Mkalgmax共Mn2k 1Mn2k0 兲, and this maximum is again Mn2kalg . So, finally, Snk12MkalgMalgn2k 苷 2n22兲兾2.

(ii) Fork andn 2k odd: in (6),Mn2kand Mn2k0 can be optimized independently because of (IIb) above. We have thenSnkMn2kalg maxMkMn2kalg Mkalg 苷2n22兲兾2.

Thus, we have proven the proposition forneven.

To prove the proposition forn odd, we must calculate bothSnkandSnnQM. We begin withSnk. Inserting (6) in the definition ofSn for nodd, we find

Sn12Mn2kMk0 1 12Mn2k0 Mk. (15) Without loss of generality, we can suppose k odd and n2 keven. Therefore, if we assume correlationsk兾共n 2

kS,Mk andMk0 can both reach the algebraic limit due to property (IIb). SoSnk12Mkalgmax共Mn2k 1 Mn2k0 兲; and due to property (IIa) this maximum isMn2kalg . ThusSkn 苷 2n23兲兾2. Let us calculateSnQMn . From the polynomialSn given by (15), we define the operatorSn in the usual way.

Therefore for the particular casek 苷 1we have Tr共rSn兲苷 12关Tr共rMn21sa0n兲 1Tr共rMn210 san兲兴,

(16) which is bounded by 2n22兲兾2 because each of the terms in the sum is bounded by that quantity. This bound is reached by generalized GHZ states, for suitable settings [11]. ThereforeSnQMn 苷2n22兲兾2fornodd, and we have proven the proposition also fornodd.

In conclusion, n-particle entanglement and n-particle nonseparability are a priori different concepts. We have shown that it is possible to discriminate quantum entan- glement, not only against local variable models, but also against all possible hybrid models k兾共n 2kS, allowing arbitrarily strong correlations inside each subset but no cor- relation between different subsets. Experiments aimed at demonstratingn-particle entanglement should be analyzed using the generalized Svetlichny inequalities described in this Letter [12].

This work was partially supported by the European Union project EQUIP (IST-1999-11053) and by an ESF Short Scientific Visit Grant.

[1] See, for instance, G. Alberet al., Quantum Information:

An Introduction to Basic Theoretical Concepts and Ex- periments, Springer Tracts in Modern Physics Vol. 173 (Springer-Verlag, Berlin, 2001).

[2] N. D. Mermin, Phys. Rev. Lett.65,1838 (1990).

[3] G. Svetlichny, Phys. Rev. D35,3066 (1987).

[4] A. V. Belinskii and D. N. Klyshko, Phys. Usp. 36, 653 (1993); N. Gisin and H. Bechmann-Pasquinucci, Phys.

Lett. A246,1 (1998); R. F. Werner and M. M. Wolf, Phys.

Rev. A 61, 062102 (2000).

[5] See, for instance, I. Percival, Phys. Lett. A244,495 (1998).

[6] J. F. Clauser, M. A. Horne, A. Shimony, and R. A. Holt, Phys. Rev. Lett.23,880 (1969).

[7] R. F. Werner and M. M. Wolf, Phys. Rev. A 64, 032112 (2001).

[8] Note that this implies that the bound for ly is equal to the bound for 1

1

1QM (product states in QM). From now on, we shall not distinguish these two cases anymore.

[9] B. S. Cirel’son, Lett. Math. Phys.4,83 (1980).

[10] V. Scarani and N. Gisin, J. Phys. A34,6043 (2001).

[11] To maximize 1

2

Mn 1Mn0

GHZ for n odd, the saj are taken of the form cosajsx 1sinajsy. One possible choice for the settings is ak

a0k1 p

2 for all k, a10

· · ·

an210

0,an0

p4. For such settings, each corre- lation coefficient becomes equal to1兾p

2in modulus, with the good sign. See [12].

[12] P. Mitchel, S. Popescu, and D. Roberts (to be published).

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