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High-visibilty two-photon interference at a telecom

wavelength using picosecond regime separated sources

Pierre Aboussouan, Olivier Alibart, Daniel Barry Ostrowsky, Pascal Baldi,

Sébastien Tanzilli

To cite this version:

Pierre Aboussouan, Olivier Alibart, Daniel Barry Ostrowsky, Pascal Baldi, Sébastien Tanzilli.

High-visibilty two-photon interference at a telecom wavelength using picosecond regime separated

sources. Physical Review A, American Physical Society, 2010, 81 (2), pp.021801(R).

�10.1103/Phys-RevA.81.021801�. �hal-00511975�

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arXiv:0912.5312v1 [quant-ph] 29 Dec 2009

Pierre Aboussouan,OlivierAlibart, Daniel B.Ostrowsky,Pas alBaldi, and SébastienTanzilli

Laboratoire de Physique de la Matière Condensée, CNRS UMR 6622, Université de Ni e  Sophia Antipolis, Par Valrose, 06108 Ni e Cedex 2, Fran e.

(Dated: De ember31,2009)

Wereportonatwo-photoninterferen eexperiment inaquantumrelay onguration usingtwo pi ose ondregimePPLNwaveguidebasedsour esemittingpairedphotonsat1550nm. Theresults show that the pi ose ond regime asso iated with a guided-wave s heme should have important reper ussionsforquantumrelayimplementationsinreal onditions,essentialforimprovingboththe workingdistan eandthee ien yofquantum ryptographyandnetworkingsystems. In ontrast toalreadyreportedregimes, namelyfemtose ond andCW,it allowsa hievinga99%netvisibility two-photon interferen e while maintaining a high ee tive photon pair rate using only standard tele om omponentsanddete tors.

PACSnumbers:03.67.-a,03.67.Bg,03.67.Dd,42.50.Dv,42.50.Ex,42.65.Lm,42.65.Wi Keywords: QuantumCommuni ation,Two-photoninterferen e,Guided-waveOpti s

Forthe realization ofquantum networks,interferen e betweenphotonsprodu edbyindependentsour esis ne -essary. Photon oales en e(or two-photoninterferen e) lies at the heart of quantum operations and is seen as arststeptowardsa hievingbothteleportation[1℄ and entanglementswapping[2,3, 4,5,6,7℄. Thisee t has been extensively studied theoreti ally [8, 9℄ and exper-imentally, initially based on two photons oming from asingledown onversionsour eand thereforesharinga ommonpast[10,11,12℄. However,experiments involv-ing truly independent photons represent an important hallengefora hievinglongerquantumlinksbymeansof quantum relays[13℄. Inthis frame, it hasbeen demon-strated theoreti ally that atwo-photon interferen e net visibility ofat least 95%isrequiredfor pra ti al imple-mentationsusing urrentlyavailablephotonpairsour es and multimodequantum memories [14℄. Rea hing su h ahighvisibilitythereforeappearstobeahardtasksin e a perfe t syn hronization between independent sour es isne essarytopreventanykindofdistinguishability be-tween the interfering photons. Several papers fo using onthesyn hronizationissuehavedemonstratedthat en-tanglementswappingwithfullyindependentsour esisin prin iplefeasibleinthefemtose ond[3,4℄andCW[5,7℄ regimes. Unfortunately, beyond the fundamental inter-est,thereportedinterferen evisibilitiesremaineitherfar from95%orshowverylowoverallphotonpairrate. For instan e, the best visibility reported so far in the fem-tose ondregimehasbeenobtainedby ompensatingthe syn hronization-indu ed temporal distinguishability by dramati ally in reasing the photons oheren e time up toafewpi ose ondsattheexpenseoftheoverall bright-ness [4℄. Sin e laser avities an easily be syn hronized to subpi ose onda ura y[15, 16℄, thestudy of the pi- ose ondregime [6,17℄,itsasso iatedlterbandwidths,

Ele troni address: sebastien.tanzilliuni e.fr

andthetypeofphotonpairgenerators,be omesofprime interesttoensuresimultaneouslyahighdegreeof indis-tinguishabilityandahighoverallbrightness.

Here, we demonstrate that to a hieve this, the pi- ose ondregimeshould provideane ienttrade-o en-ablingnear-perfe ttwo-photoninterferen eandhigh ef-fe tive photon pair rates, when asso iated with stan-dard omponentsavailablefromthetele ommuni ations industry. More pre isely, we realized an experiment basedon a single pi ose ond pump laser and two peri-odi allypoledlithiumniobate(PPLN)waveguides emit-tingpairedphotonsaround1550nmtoapproximate in-dependent sour es. We report the highest two-photon interferen enetvisibility,i.e. of99%,everdemonstrated ina ongurationextendable toquantum relays. Su ha proof-of-prin ipleemphasizes why guided-wave te hnol-ogy, in the pi ose ond regime, should lead to realisti quantum relays hemes,namely byoeringan redu ed- onstraint solution for the syn hronization issue when two ompletelyindependentlasers areemployed. Inthe following, we briey introdu e the entanglement swap-ping based quantum relay s heme and dis uss why the pi ose ondregimeisavaluabletrade-o. Wethenfo us onourexperimental demonstration. Finally, wedetaila omparativestudy ofperforman e withsimilarreported experiments.

A basi s heme of a quantum relay based on entan-glementswapping is givenin FIG.1 (see aption for de-tails). Forlongdistan equantum ommuni ationlinks, the preferred qubit arriers are photonsat 1550nm al-lowing the users, namely Ali e and Bob, to take ad-vantage of standard opti al bers for distribution pur-poses. Theoreti ally, the two inner photons an ome from any type of sour e, provided theyare identi al at thebeam-splitter(BS)(pre-sele tion)oratthedete tors (post-sele tion). Fromtheexperimentalside,wehaveto ompare their oheren e time,

τ

oh

, to the time un er-tainty,

t

un ert

(3)

FIG. 1: S hemati sof a quantum relay involving twopairs of entangled photons emitted by two syn hronized sour es (EPR).Thetwoinnerphotonsare senttoa50/50BSwhere aBellstatemeasurement(BSM),basedontwo-photon inter-feren e,isperformed. Usingadedi ateddete tion, entangle-ment anbe swapped fromthese photonsto theouterones makingAli eandBob onne tedbyentanglement,asifthey hadea hre eivedonephotonfromanentangledpairdire tly. The BSM serves as a triggerfor Ali e and Bob's dete tors. Itthereforeenablesredu ingtheSNRoftheoverallquantum linkandfurtherin reasingthemaximuma hievabledistan e.

te tor'stiming jitters),whi h anbewrittenas:

τ

oh

≥ t

un ert

(1) Suitable bandpass lters are therefore employed to a hieveoptimalinterferen evisibilities. Upto now,this issuehasbeenaddressedusingdierentapproa hesbased onpulsedorCWlasers(seealsoTableIfor omparison). Ontheonehand,therstexperimentsreportedtwo in-dependent rystalspumpedbyfemtose ondlasers,sin e this regime allows working with broadband lters, i.e. ontheorderofafew nm[2℄. However,thelargephoton bandwidths makes them more prone to hromati and polarizationdispersionsinopti albersandleadsto re-ported visibilities below 85% [18℄. Moreover when two independent lasers are used, the two related laser avi-tieshavetobeproperlysyn hronizedsoastobe identi- alwithinthepumppulseduration(

100fs)[3,4℄. This anbea hievedusingphase-lo kedloopsoratomi lo ks and dedi ated ele troni s[19, 20℄. Anyremaining jitter between the two lasers has to be ompensated by nar-rowing the lters whi h implies a substantialredu tion ofthepairprodu tionrateforequivalentpowers[4℄.

On the other hand, the development of narrow-bandwidthberBragggrating(FBG)ltersallowsusing twoindependentCWlasersstabilizedagainstanatomi transition [5, 6℄. Sin e this regime does not provide anyreferen e lo k,thetimingfun tion istransferredto the oin iden edete tionafter theBS.Toensureahigh quality interferen e, the photons oheren e time hasto be longer than the jitter of the dete tors. Experimen-tally, thisis madepossibleusing asuitable ombination oflow-jitterdete tors (basedonsuper ondu tingor up- onversionte hnologies),ontheorderof70ps,asso iated withultra-narrowFBGlters,ontheorderof10pm[5℄. In su h asituation, onegets rid of thesyn hronization

u tuationsofthelters entralwavelengths,low exper-imental rates due to the narrow lters oupled to the randomnessof entanglingphotonsby oin iden e dete -tion, and high statisti al u tuations due to low ount rates. All theseissuespreventrea hinghigh visibilities.

Betweenthesetwoextremes,thepi ose ondregime ap-pears to be an e ient ompromise. First, the timing ondition(1) iseasilymetbyusingFBGltersshowing mu h larger bandwidths than in CW, i.e. on the or-derof100pm[17℄. Se ond,thisallowstakingadvantage of o-the-shelf InGaAs avalan he photodiodes (APD). Last, when ompared to the femtose ond regime, nar-rower bandwidthsloosen the onstraints on both path-lengthstabilizationfortheinterferingphotonsandlaser syn hronization to subpi ose ond a ura y [15, 16℄ to obtainhigh-visibilityHong-Ou-Mandel interferen e. All thesekeypointsmotivateinvestigatingthisregime.

Assumingsyn hronization is fairly feasible, we there-forefo usedoureortsat in reasingtheoverallspe tral brightness by employing a pi ose ond pump laser asso- iated with state-of-the-art waveguide sour es emitting at tele om wavelengths. As shown in FIG.2, the pump laser (Coherent MIRA 900-D) provides 1.2ps-duration, time-bandwidthlimited(

∆λ

p

=

0.25nm) pulses, at the wavelength of

λ

p

=

768nm and at a repetition rate of 76MHz. Thepulses aresentto aBS whoseoutputsare dire tedtowardstwo10mm-longPPLNwaveguides fab-ri atedin ourlaboratoryusing thesoft-protonex hange te hnique[21℄. Thesedevi esaresinglemodeattele om wavelengths enabling only one nonlinear pro ess to o - uravoidinganyadditionnalba kgroundnoisewithinthe bandwidthofinterestwhi hisakeyadvantage ompared to four-wave mixing sour es [6, 17℄ limited by Raman ba kgroundphotons. Bothsamplesopto-geometri al pa-rameterswere designed to produ e identi al degenerate pairedphotonsat1536nmwithin abandwidthof50nm whenpumpedat768nminthepi ose ondregime. Sin e thelterbandwidthsaremu h narrowerthanthe down onversion bandwidth (

∆λ

spdc

∆λ

f ilter

≥ 10

2

), experimentally, the two sour es are simply independently stabilized at thetemperatureof343Ktowithin 0.1K.

Fromea h sour e,wesele tpairs of photonsmeeting theFouriertransform riterionusingnarrowband demul-tiplexers made of two opti al ir ulators and a pair of FBGlters. Thesearesettoree tenergy-mat hedpairs of wavelength at 1537.4nm and 1534.6nm, i.e. around degenera y, asso iated with bandwidths of 800pm and 250pm, respe tively. A slightlywider (800pm) lter is used onthe longwavelength(1537nm) photons mainly to minimizeoverall losses. This lteringsolution based on standardtele om omponentsprovides a lever way to separate deterministi allythe photonsat theoutput of the waveguides and makes them ea h available in a singlemodeber[5℄. The250pmltersbandwidth has been hoosenfortworeasons: (a)itisnarrowenoughto a ommodatethe1.2ps-durationofthelaserpulsesand anypossiblejitterupto4psduetolasersyn hronization

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FIG.2: Coales en eexperimentbasedontwoPPLN waveg-uidespumpedbyasinglepi ose ondlaser. Averyweakpart of thisbeamis sentto asili on APD (not represented) em-ployedas alaser lo k randomdivider. Itsele tri al output isusedtotriggerfourInGaAs-APDs.

Λ

: polingperiodofthe PPLN waveguides; I:isolator; R: retro-ree tor; C: ir ula-tor;&: AND-gate. TheInGaAs-APDsfeature10%quantum e ien yandadark ountprobabilityofabout

10

−5

ns

−1

.

stabilizetheir entralwavelengthusingtwoindependent proportional-integral-derivativetemperature ontrollers. To observe the two-photon interferen e, four-fold o-in iden es are dete ted thanks to four InGaAs-APDs (idQuantique201)triggered byaPeltier ooledSi-APD (idQuantique100) pla ed onthe path of an attenuated fra tion of thepump beam. Sin e these InGaAs-APDs are designed to handle a maximum triggering rate of 1MHz,thiste hniqueallowsworkingatanaverage lo k of600kHzrandomlypi kedfromthe76MHzlaser repe-titionrate. Inour ase,fasterInGaAs-APDwouldhighly improvetheoverall oin iden erateasshowninRef.[6℄. The evolutionof the ee tive four-fold oin iden e rate is givenin FIG.3in whi h aremarkabledip isobtained whenthedelaybetweenthetwoinner photonsiszero.

Using only 1mW of mean pump power per sour e, we obtained

4 × 10

3

two-fold oin iden es perhour and persour e whi h orrespondsto about 0.05photon per pulse. In terms of normalizedbrightnessit means that our sour es rea h

1.6 × 10

3

pairs

·

s

−1

·

pm

−1

·

mW

−1

after the ltering stage. This brightness orresponds to the state-of-the-art for PPLN waveguides and is basi ally ve orders of magnitude larger than that of bulk rys-tals [21, 22℄. When the two photons are made indis-tinguishable in time (

δt

) thanks to the adjustment of the retro-ree tor (R) pla ed in front of onesample, a

93%±3%

redu tionintherawfour-fold oin iden e ount

isobtained. By orre tlyre ordingthea idental oin i-den es,weareabletodemonstratethatthenetvisibility rea hes

99%±3%

. Thefullwidthathalfmaximumofthe dipisapproximately

∆τ ≈ 11

ps,whi hisingood agree-mentwiththe oheren etimeof14psexpe tedfromthe lterbandwidths. This interferen evisibilityis also ex-tremely losetothemaximumvalueof

99.9%

al ulated from the theory taking into a ount our ltering band-widths,asproperlyoutlinedinRefs.[8,9,18℄. Notethat theveryhighstabilityoeredbyourguided-waves heme

0

5

10

15

20

25

30

35

-50

-40

-30

-20

-10

0

10

20

30

40

0

1000

2000

3000

4000

5000

6000

Four-fold coincidences (per 2 hours)

Two-fold coincidences (per 2 hours)

Relative delay (ps)

Accidental 4-fold coincidences

4-fold coincidences

Gaussian fit V=99%

2-fold coincidences

FIG.3: Four-fold oin iden e rateasa fun tionof the rela-tivedelay,

δt

,between the interferingphotons (

0.04

pho-ton/pulse). We learly observeadipfor

δt = 0

that rea hes thenoise level. TheGaussiantof theinterferen e pattern showsanetvisibilityof

99% ± 3%

. Wealsoplottedoneofthe two-fold oin iden esrelated to oneof the sour esafter the BStoverifythisgureis onstant.

morethan30pointsevenlyspreadoverthedip.

TableI presentsthe ompared resultsreported inthe literatureforsimilar ongurationswhi h an be dier-entiated by four key points: (i) the type of nonlinear generators,(ii)theemittedphotonwavelengths,(iii)the pumpingregimeanditsasso iatedtimeun ertainty,(iv) and, nally, the applied ltering bandwidths and their asso iated oheren e times. Froma omparisonbetween thereported results, we on lude that the ombination ofthepi ose ondregimeandthesinglemodeproperties of the employed tele ommuni ation omponents is the mostperformant s heme. It allows mat hing e iently theinequality(1)andobtainingnear-perfe ttwo-photon interferen e. For pra ti allongdistan e quantum om-muni ation,itisalsointerestingto omparetheee tive numberofpairsavailableperse ond atAli eand Bob's lo ations. Thisgureofmeritis al ulatedby normaliz-ingthefour-fold oin iden erateswith respe tto Ali e andBob'sdete tore ien ies. A omparisonwith sim-ilar ongurationsattele omwavelengthsindi atesthat the pi ose ond regime allows maintaining a high ee -tivepair produ tion rate equivalentto that of the fem-tose ondregimebutshowsamu hhighervisibility. One shouldalsonotethetwoordersofmagnituderate dier-en eforequivalentsour ete hnologiesandbrightness be-tweentheCWand pi ose ondregimes. Inaddition,the bestvisibilityreportedinRef.[4℄withphotonsinthe vis-ible omesfromthefa tthatthelteringbandwidthsare ontheorderofthosene essaryforthepi ose ondregime. Consequently, the overall brightness is very low onsid-eringthe use of e ientSi-APDs. Finally, bright ber sour es are ontaminated by intrinsi spontaneous

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Ra-TABLEI:Comparedtwo-photoninterferen evisibilities,sour ebrightness,andoverallexperimental oin iden erates,between reportedworksin ontinuouswave(CW),pi ose ond (ps),andfemtose ond(fs)regimes. Regardingtimeun ertainties, note thatthe rstnumberisalwaysasso iatedwiththepulseduration while the

±

sign orrespondstothe syn hronisationjitter iftwopulsedlasers areinvolved. In ontrast,the timeun ertaintyfor the CW ase is asso iatedwith thedete tor's timing jitters. The oheren etimeis al ulatedforGaussianltersusingthestandardrelation

τ

c

= 0.44

λ

2

c∆λ

. Referen e Sour e Wavelength Brightness Regime

a

Filterbandwidth Rate Raw Net

nm

pair/s/pm/mW

(timeun ertainty) ( oheren etime)

pair/s

visibility visibility Geneva[5 ℄ PPLN/w 1550

0.9 × 10

3

CW(70ps) 0.01nm(350ps)

3 × 10

−3

NA 77% Ni e PPLN/w 1550

1.6 × 10

3

ps(1.2ps) 0.25nm(14ps)

3 × 10

−1

93% 99% Atsugi[6 ℄ Fiber 1550 NA

ps(19ps) 0.2nm(18ps)

2

b 64% NA Bristol[17 ℄ Fiber 600 NA

ps(1.5ps) 0.3nm(1.8ps)

4 × 10

−1

88% NA Geneva[18 ℄ BulkLBO 1310 NA

fs(200fs) 5nm(500fs)

7 × 10

−1

77% 84% Beijing[3 ℄ BulkBBO 800

1.2 × 10

−2

fs (60

±

2fs) 2.8nm(335fs)

3 × 10

−2

82% NA Vienna[4℄ BulkBBO 800 NA

fs(50

±

260fs) 0.4nm(2.3ps)

1 × 10

−2

96% NA a

Inthis olumn,theguresasso iatedwiththepumpregimes orrespondtothenumberoflasersemployed. b

Theexperimentoperatesat500MHzrepetitionratethereforein reasingtheavailablephotonpairrate.

Thetwolasersarenottrulyindependentsin etheysharethesameTi:Sapphire rystalKerrmediumfora uratesyn hronization.

andtoredu edvisibilities[6,17℄.

The results demonstrated in this experiment are of broadinterestsin etheobtainednetvisibilityisthebest valuereportedtodatefor omparable ongurations. A - ording to referen e [14℄, this allows, for therst time, onsideringthepossibilityofusingquantumrelaysin a -tual quantum ryptography networks. In this ontext, wheretwosyn hronizedpi ose ondlasersmustbeused, we notonlyexpe t resultsof thesameorder,thanksto

the high experimental stability and versatility demon-strated, but also be ause of the redu ed- onstraint on thesyn hronizationissue[15,16℄.

The authorsthankM. P.de Mi heliand S. Tas u for the realization of the PPLN waveguides, G. Sauder for te hni alsupport,andA.Beveratos,H.Zbinden,andK. Thyagarajanforfruitfuldis ussions. Thisworkhasbeen supportedbytheCNRS,theUniversityofNi eSophia Antipolis,andtheFren h MinistryofResear h.

[1℄ O. Landry, J. A. W. van Houwelingen, A. Beveratos, H.Zbinden, and N. Gisin, J.Opt.So . Am.B24, 398 (2007),andreferen estherein.

[2℄ H.deRiedmatten,I.Mar iki , J.A. W.van Houwelin-gen, W.Tittel, H. Zbinden, andN. Gisin, Phy.Rev.A 71,050302(R)(2005).

[3℄ T. Yang, Q. Zhang, T.-Y. Chen, S. Lu, J. Yin, J.-W. Pan, Z.-Y. Wei, J.-R. Tian, and J. Zhang, Phys. Rev. Lett.96,110501(2006).

[4℄ R. Kaltenbaek, R. Prevedel, M. Aspelmeyer, and A.Zeilinger,Phys.Rev.A79,040302(R)(2009). [5℄ M.Halder,A.Beveratos,N.Gisin,V.S arani,C.Simon,

andH.Zbinden,NaturePhys.3,692(2007).

[6℄ H.TakesueandB.Miquel,Opt.Exp.17,10748 (2009). [7℄ J.Yang,X.-H.Bao,H.Zhang,S.Chen,C.-Z.Peng,Z.-B. Chen,andJ.-W.Pan, Phys.Rev.A80,042321(2009). [8℄ J.Rarity,inFundamentalProblemsinQuantumTheory,

editedbyD.M.GreenbergerandA.Zeilinger(Annalsof theNewYorkA ademyofS ien es,1995),p.624. [9℄ T.Legero,T.Wilk,A.Kuhn,andG.Rempe,Appl.Phys.

B77,797(2003).

[10℄ C.K.Hong,Z. Y.Ou, andL. Mandel,Phys.Rev.Lett 59,2044(1987).

[11℄ J.G.Rarityand P.R. Tapster, J. Opt.So .Am.B 6, 1221(1989).

[12℄ M.Halder,S.Tanzilli,H.deRiedmatten,A.Beveratos,

H. Zbinden, and N. Gisin, Phys. Rev. A 71, 042335 (2005),andreferen estherein.

[13℄ D.Collins,N.Gisin,andH.deRiedmatten,J.Mod.Opt. 52,735(2005).

[14℄ C.Simon,H.deRiedmatten,M.Afzelius,N.Sangouard, H. Zbinden, and N. Gisin, Phys.Rev.Lett 98, 190503 (2007).

[15℄ D.D.Hudson,S.M. Foreman, S.T.Cundi,andJ.Ye, Opt.Lett.31,1951(2006).

[16℄ J. Kim, J. A. Cox, J. Chen, and F. X. Kärtner, Nat. Phot.2,733 (2008).

[17℄ J.Ful onis,O.Alibart,W.J.Wadsworth,andJ.G. Rar-ity,N.J.Phys.9,276(2007).

[18℄ H. de Riedmatten, I. Mar iki , W. Tittel, H. Zbinden, andN.Gisin,Phys.Rev.A67,022301(2003).

[19℄ R.K.Shelton,L.-S.Ma,H.C.Kapteyn,M.M.Murnane, J.L.Hall,andJ.Ye,S ien e293,1286(2001).

[20℄ S. Cundi, B. Kolner, P. Corkum, S. Diddams, and H.Telle,Sele tedTopi sinQuantumEle troni s,IEEE Journalof 9,969(2003).

[21℄ S. Tanzilli, W. Tittel, H. D. Riedmatten, H. Zbinden, P. Baldi, M. D. Mi heli, D. Ostrowsky, and N. Gisin, Eur.Phys.J.D18,155(2002).

[22℄ M. Halder, A. Beveratos, R. T. Thew, C. Jorel, H.Zbinden,andN.Gisin,N.J.Phys.10,023027(2008).

Figure

FIG. 1: Shematis of a quantum relay involving two pairs
FIG. 2: Coalesene experiment based on two PPLN waveg-
TABLE I: Compared two-photon interferene visibilities, soure brightness, and overall experimental oinidene rates, between

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