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Construction of molecular cathodes and photocathodes for hydrogen evolution

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Academic year: 2021

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Figure I.2. Half catalytic wave overpotential determination exemplified with [Ni(P 2 Ph N 2
Figure I.3. Catalytic Tafel plots for molecular HECs under various conditions, 10 among others [Fe(TPP)Cl] (black), [Ni(P 2
Figure I.5. Proposed catalytic mechanism for H 2 evolution and uptake at a [FeFe] hydrogenase active site 17 (left) and putative intermediate during proton reduction by [FeFe] hydrogenase showing importance of the proximate basic group (right)
Figure I.12. Synthesis scheme of the (DOH) 2 N 3 pn ligand and of the [Co(DO)(DOH)N 3 pnL 2 ] complex (L = Cl – , Br – )
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