Density matrix approach
to
the complex
heavyion optical potential
R.
Sartor andFl.
StancuInstitut de Physique B5, Uniuersite de Liege, Sart Tilman, B-4000Liege 1,Belgium (Received 28 April 1982)
We extend the applicability ofthe density matrix expansion to a complex effective in-teraction depending both onthe density and the kinetic energy density. A detailed study of the kinetic energy density dependence ofthe density matrix expansion coefficients is given. The corresponding energy density has a parametrized form which is tested in the calcula-tion ofthe optical potential ofthe '
0+
'0
system at several energies. Exact results are well reproduced bythe complex density matrix expansion.NUCLEAR REACTIONS Density matrix expansion for acomplex ef-fective interaction; application toheavy ionoptical potential.
J
I.
INTRODUCTIONIt
is now common practice' ' to define the heavy ion optical potential at a separation distanceD
as the difference between the expectation valueof
some effective Hamiltonian
H
at distanceD
and the expectation valueof
the same Hamiltonian at infini-tyV»,
(D)=(H(D))
—
(H(ce))
.
Early computations' used an energy functional or an effective interaction which can be related to G matrix calculations in nuclear matter with a spheri-cal Fermi sea. As a consequence those computa-tions could only determine the real part
of
the opti-cal potential. However,if
the heavy ion collision is locally described as the collisionof
two nuclear matter systems, one isled to anon-Hermitian6
matrix ''
' ' which will also enable thecompu-tation
of
ImV,„,
(D)through the useof
Eq.
(1.
1). The direct computationof
V», from a finite range effective interaction is, however, cumbersome and time consuming. As a consequence, approxi-mation schemes have been proposed. Aconvenient procedure, extensively used for the real part'of
V»„
is based on energy functionals. In aprevious work ' weproposed acomplex Skyrme-type interac-tion which generates a complex energy density, to be used in the calculationof
both the real and imag-inary parts. The imaginary partof
the Skyrme-type interaction was obtained by multiplying the real Skyrme-interaction used inRef.
3by a scaling fac-tor. This was assumed todepend on the local densi-typ
and the intrinsic kinetic energy density v' 'andfound numerically from the finite range complex
ef-fective interaction
of Ref.
12.In
Ref.
14, more emphasis was put on avoiding the explicit useof
any wave function in the compu-tationof
the expectation values appearing inEq.
(1.
1). Suitable approximations for p and r'~' have been found toreproduce the exact results at low en-ergies by meansof
a generalized double folding method.In this paper we extend the density matrix expan-sion (DME)
of
Negele and Vautherin to the com-plex domain in order tojustify the energy function-al introduced inRef. 21.
The present paper is organized as follows. In Sec.
II,
we briefly recall theDME
and single out the peculiar features arising from its application to acomplex effective interaction. In Sec.III,
we dis-cuss the asymptotic behaviorof
two colliding nu-clear matter systems when the Fermi sea is nearly spherical, and its consequences on the imaginary partof
the optical potential. InSec.
IV,we provide a parametrized form for theDME
coefficients, and in Sec.Vwe apply it tothe calculationof
the opti-cal potentialof
the '0+
'0
system and compare the present results with the exact calculationsof
Ref.
13.
II.
THE DENSITY MATRIX EXPANSION WITH ACOMPLEX EFFECTIVEINTERACTION
In this section, we recall the relevant
DME
for-mulas derived inRef.
22 and adapt them tothe caseof
a complex effective interaction. The discussion is limited tonuclei having an equal numberof
neu-trons and protons. The effective N-N interaction 10251982
TheAmerican Physical Societycomponent can be written as psL(kFS) is the Slater approximation given by 6 UsT(r) ( 1 e
—
2x)2e—3x~
g
sT X m=0 m& PSL(kFS)= 3J
(kFS) sk~ (2.4) forr
(1
fm,
(2.
1) 7 (1 —2x)2y
ZST m=1 for r)1
fm,(2.
2) 1/3p(R)
(2.5)In Eqs. (2.3) and (2.4), the local Fermi momentum kF is related tothe matter density
p(R)
bywith
x
=0.
7r, where r isthe separation distance be-tween the interaction nucleons, and Am and Zm"are complex coefficients depending upon the local density p, the local intrinsic kinetic energy density T' ' defined in Sec.
III,
and the incident energy (seeRefs. 10
—
14for full details).The basic approximation
of
theDME
proposed inRef.
22was touse the following truncated Bessel function expansion forthe density matrix:P
R+
—,
R
—
—
=PSL(kFS)P(R)+
2skp3Xj,
(kFS)[—,V'P(R)—
T(R)Bywriting asimilar expansion for the product
p
R+
—
2 pR
——
2(H
)~,
=
f
4
~,
(R)dR,
(2.6)where the potential energy density
4
~,
(R)
reads:~Pot(R)
VNM+
2 VD(P~'P—
I~P
l')
which appears in the direct term
of
the expectation value(H),
one can express the potential partof
(H) as":
+
—,kFP(R)],
+
Vs( 5kFP2T+
—,V—
P).
(2.7)(2.3)
I
The expression
of
P
p thas two distinct partsV~M
—
—
f
ds[3v
(s)+3usa(s)+9v
(s)+Uso(s)]
2
+
f
d sPSL (kFS)[3U(s)+3U
(s)—
9U (s)—
U(s)]
32 (2.8)
is the potential energy
of
nuclear matter corre-sponding to the local densityp(R),
and V23 and Vsare the direct (D) and exchange (E) finiteness corrections given by I with 35
g(kFS)=
j3(kFs)
.
2(kFs) (2.11) and VD—
—
1Jd
ss
g(kFS)[3u(s)+3U
(s)+9u
(s)+U
(s)]
(2.9) Vz—
—
dss
PsL(kFS)g(kFs) 16 X [3v(s)+3U
(s) (2.12) Negele and Vautherin then proceed to eliminate the Vpterms by an integration by parts. In the caseof
acomplex effective interaction, this implies the ap-pearanceof
U derivatives with respect to both pand ~. In order to avoid any derivative here we keep the Vpterms.
. We introduce the following notation: '2/3 A
=V~~+
3 37K s/3 5 2 pVE,
9~ To(s } Uso(s)]
(2.10)B
=
—
pVE,
1C=
—
—,VD, (2.13) (2.14)FIG.
2. Brueckner-Hartree-Fock contribution to the binding energy ofthe Fermi sea depicted in Fig. 1. The wiggly line depicts the Brueckner reaction matrix G.22 treats a static case. The replacement
of
~byr'
' appears as a consequenceof
preserving the Galilean invarianceof
the interaction.FIG.
1. A deformed Fermi sea used in the local description of a heavy ion collision as the collision of two nuclear matter systems.III.
THE BINDING ENERGY OFNUCLEAR MATTER FORANEARLY SPHERICALFERMISEA
1 1
D
=
,
p(Vn+
——,VE),
(2.15)where
2, 8,
C,andD
are complex quantities, which depend onp, ~' ',and the incident energy. Then the potential energy density (2.7) becomes4
~,
(R)=A+Br'
'+C(Vp)
+DV' p . (2.16) At this point we stress that the potential energy density (2.16)depends on the intrinsic kinetic ener-gy densityr'
' defined inEq. (3.
15) insteadof
the kinetic energy density ~ as introduced by Negele and Vautherin. The difference comes from the fact that we deal with a moving system whileRef.
I
As itwill turn out in Sec. IV, it isuseful to study the ~' ' dependence
of
the imaginary partof
the binding energy for a nearly spherical Fermi sea. The present analysis takes place in the momentum space and the density and the incident relative momentum EC, given by the separation distance be-tween the centersof
the two spheres constituting the Fermi sea shown in Fig. 1 are fixed quantities. The intrinsic kinetic energy density ~' ' is then uniquely determined by the radiiof
the two spheres.In the Brueckner-Hartree-Fock (BHF) approxi-mation, the potential energy
of
nuclear matter is given by the diagramof
Fig.2.
It
can be easily shown that its imaginary part is proportionalto
the integralImVEHF cc
f
dk)dk2dk3dk4
[(k)k2
~G(co&+cop) ~ k3k4)A I @coi+coz
—
co3—
~4(3.
1)where the momenta k~ and k2 are inside the de-formed Fermi sea
F
of Fig.
1,while k3 and k4 are outside it, and G is the Brueckner reaction matrix. The single particle energies co;are defined as1
where we have shifted from k
=
~ k ~ tocoasthein-tegration variable. This causes no problem since co(k} is a monotonously increasing function
of k.
Hence, wecan writeA'k,
'
co;
=
+
U(kc),
201 (32) Im
V,
„„fdco~d-co2dco3dcl)4I (co]&c02&c03&c04) where U is a continuous auxiliary potential.For
any k integration, one has
X
5(co~+cop—
co3—
co4) (3.4)f
dk
=
f
k dk dk=
f
k (Co} dCodk,(3.
3) withI(
„,
,)=g
k;f
gdk;
)(k,
k ~G(,
+
)~ k k)„('.
(3 5)I.
et us consider the Fermi seaof
Fig. 1and denote by coF~ the energy associated with the momentum kF& andby
~~~+
g
thatof
E,
+k&2. The quantityg
issmall compared toruz~ since the Fermi sea isnearly spherical. Since co3and co4are greater than coF&,the 5function inEq. (3.
4)vanishes except when k& or/and k2 liein-(3.6) side
it.
Since all the above expressions are symmetrical in k1 and k2, the case in which k1 is insideZ
and k2 isoutside itwould yield the same result. The contribution to (3.4)isF1 ~F1+~ 00 00
(ImVBHF)1
—
dco1 dcog dco3 dco4I(co„co2,co3, 4)5(co1~co2—
co3—
40 F1 ~F1
COF1
—
g&CO1&COF1, NF1(C02(COF1+'g,
F1
&3(F1+9
(3.7)
The function I(co1,co2,co3,co4) can thus be
appmxi-where we have specified the integration limits.
It
is, however, clear that the 6 function imposes further restrictions over the rangeof
integrationof
co1, co3,and ~4. One can easily see that in fact, the integra-tion limits are restricted to
mated by l(coF»coF»coF»coF,)and be taken outside the integral sign in
Eq.
(3.6). The remaining in-tegrations arethen straightforward and yield(ImVBHF)1
I
(COF» COF»COF»COF1)9
3
I
(COF1~COF1~COF1~~F
1)X [co(K,
+
kF2)—
co(kF1)]'. (3.&)Case
2.
Both k1 and k2 lie insideZ.
The contri-bution to (3.4) isnow~F1+& F1+'9 00 00
(ImVBHF)~- ~F1 dco1 dco2 dco3 dco4J(co1,co~, co3co4)5(co1+co2 co3 co4)
~F1 F1 NF1 (3.9)
and the further restrictions imposed by the 6 func-tion give
I
(3.12)can be written in leading order
ImVBH&-(51+5&)3 . (3.14)
N3&Q)F1+2'g ~
Q)4&COF1+2Y/
.
(3.10)Therefore the function I(co1,co2,co3,co4)can again be
approximated by I(coF1,coF1,coF1,coF1) and taken outside the integral sign. Explicit integration then yields
VBHF)2 i(COF1 COF1 COF1 COF1)C)3
I
(COF1&NF»COF1~NF1)=r—
pkG(2)
(3.15) where p is the density, ~is the kinetic energy densi-ty given by
We have now to relate 61 and 62to the variation
of
the intrinsic kinetic energy density ~' ' when one goes from the spherical Fermi seaof
radius kF to the deformed seaI' of
Fig.1.
The intrinsic kinetic energy density ~' 'is defined as10
X
[co(K„+
kF~) co(kF,)]',
—
i.
e., the same as in case1.
Therefore, one hasImVBHF [co(Ki
+
kF2) co(kF1)]—
(3.11)(3.12)
r=
1gk—
V-
kcryand kG isthe mean momentum per nucleon
(3.16)
(3.17)
kF1 kF 61 ~
K„+kF2
—
—
kFj62,
(3.13)
where 61and 62are small with respect to kF and the change in the Fermi sea is such as the density remains equal to p (constant volume). Then
Eq.
Let us define kF as the radius
of
the spherical Fer-mi-sea corresponding to the fixed densityp.
One can writeN
—
=p=constant
.
V (3.18)
The intrinsic kinetic energy density ~' ' defined
In Eqs.
(3.
16) and(3.
17), the k summations extend over the deformed Fermi seaF,
o. and ~are the spin and isospin degreesof
freedom, V is the volumeof
the boxin which the system is contained, while Nis the total number
of
nucleons. As usual Vand N tend toinfinity withabove represents the same quantity as that given by formula (6)
of Ref.
21.
Denoting by
M
the variationof
any quantityx
when one goes from the spherical Fermi sea tothe deformed one depicted inFig.
1, one has(3.19)
kF kF
—
1 5
+
2p+
&r(3.
24) Hence, whenhp=O,
wehave in the lowest orderbecause ko
—
—
0
for a spherical Fermi sea (static case). By explicit calculation we obtain up to second order in 5; 2 2) kF kF—
1 52 3m'(3.
25) 2 2 1 kFbp=
—
kp5)+
kp3+
5) 2%2Bycomparing Eqs. (3.14)and (3.25) and taking into account
Eq. (3.
21),we getkF kF
2n
L
&m~mrF
-~&
(2)(3.
26)kF kF
+
—
15)52+
(3.20) which is the main resultof
this section and will beused as abasic argument in the next section.
5)
—
—
0(52 ).
(3.21)Hence, up tothird order in 52,a consistent approxi-mation to Ap is provided by
kF
bp=
—
kF5)+
—
1 522'
pEquation (3.20) shows that 5~ and 52 cannot be
of
the same order
of
magnitude. The reason is that the density must remain constant and the constraint Ap=O would imply5;=0,
i.
e., no deformation at all. Therefore, the constraintAp=0
imposesIV. THEPARAMETRIZED FORM OF DME COEFFICIENTS
We have computed the A,
B,
C, andD
coeffi-cientsof Eq.
(2.16) forE„=O,
0.
5, and 1fm '/nucleon and for a series
of
spherical and de-formed Fermi seas. In viewof
possible futureap-K„=0.5fm kF kF
—
1 5)5p r kF+
2rr' (3.22) C) X QJl K„=1.0fmThe variation
of
the intrinsic kinetic energy density r' ' is then related to the variation b,p
of Eq.
(3.22) by 20 15 10h~=kF
bp+
—
1 62 3m-2 0.5+0(5
)+.
(3.23)where the term 0(52)also contains the variation
of
k62given by
FIG. 3. The ratio (=ImA/ReA for various densities and two K, values as a function of x defined by Eq. (4.1). po
—
—
0.17 nucleon/fm is the normal nuclear rnatter density.following,
4
will designate anyof
the A,8,
C, and Dcoefficients.nomial we take the following expression for Im@':
ImÃ=x(Ii+I2x+I3x
) (4.2)A. ~' 'parametrization
It
turns out that the dependence onE„and
r' 'of
the real part
of
any4
coefficient is negligible and therefore we only have to discuss ther'
' parame-trizationof ImÃ. It
isuseful to define thep depen-dent ratio(2) (2) (2) (2)
ax VmIII %max Vm
(4.1)
where z'
„and
~',
',
are the minimum and max-imum intrinsic kinetic energies associated with a de-formed Fermi seaof
a given densityp.
The value~' „corresponds to aspherical Fermi sea and gives
x
=0.
The other extreme ~ma'x impliesx
=l
andcorresponds to a deformed Fermi sea composed
of
two spheresof
equal radii having their centers separated by adistancej:„.
At present we wish to make use
of
the result ob-tained in the previous section.For
a small defor-mationof
the Fermi sea,i.
e., smallx,
expression(3.
25) indicates that the imaginary partof
all 4'and find values
of
the coefficientsI„(n
=1
—
3) which reproduce the exact results within3/o.
We note that eachI„depends
onE„and
p.
The p dependence is parametrized below. In Figs. 3—
6, we plot the ratioIm@'
Re@
as a function
of
x
for a seriesof
valuesof
p andE,
.
Parametrization (4.2) is used for Im@'. These fig-ures are very much reminiscent
of Fig.
3of
Ref.
21 where thex
dependenceof
the entire imaginary partof
the Skyrme-type interaction had been found nu-merically. The present parametrization is more de-tailed than thatof Ref.
21 and gives an explicit dependence onr'
'of
the imaginary partof
the en-ergy density.B.
pparametrizationWe now discuss the p parametrization
of Re@
and
of
theI„(n
=1
—
3)
coefficients appearing inEq.
(4.2). As can be seen from Eqs. (2.8), (2.12),K„=0.5fm '
20-K„=1.0fm" Pl C) X Qdl 20 K„=1,0 fm" 15 10 10 0.5 0.5K„=0.5fm'
K„=1.0fm "
potential as defined by
Eq.
(1.
1), where we have used the expression (2.16}with the parametrizations found forA,B,
C,andD.
The densities p and v' 'have been calculated with
a two center shell model described in
Ref.
3 and equivalent to Fliessbach's model.In this model the ground state
of
'0+' 0
is described by a Slater determinant built from the single particle states20 15 eik[z+(D/2)] Wa(1) Y'a(1)e —ik[z—(D/2)] 'VP(2) 9'P(2)e (51) 10 0
FIG.
6. Same asFig. 3,but for g=ImD/ReD.(2.13),and (2.15), a p factor can be extracted from the p dependence
of
A, while a p factor can be ex-tracted from thatof
B
andD.
Byparametrizing the remaining p dependence by acubic polynomial, we can writeOwing tothe fact that the single particle states
g
ii~and ltipi2~ are not orthogonal, wehave
—1
X
pv), ( ) ( }C(.
)WP(j) p(j),a(i) (5.3) —1 + Bp(j),a(i) (D)k)V0a(i)Vtkp(q)(5
4)'
p(j),a(i) andwhere Pa~,~ and PP~2~ are eigenstates
of
harmonicos-cillator wells centered at
—
(D/2)
andD/2,
respec-tively. The relation between the single particle momentum component k along the z axis andE,
defined previously is (5.2)Re@
=
p'(R
)+R2p+R
3p'+R4p')
I„=p
(I„(+I„2p+I„3p+I„4p
) (4.3} 1—
1 Bp()a(;) (D, k) P p(j),a(i) X(ga(,;)VQp(;) Vga(i)fpij—)) ~ (5.5)(5
=1
—
3),
(4.
4) where the exponenta
is equal to 2, 1,0, and 1 forthe coefficients A,
B,
C, and D,respectively. Densi-ty parametrizations analogous to (4.3) and(44)
were also used in Refs. 9and 22.
The numerical values
of
Rj
and Iaj (n=1
—
3;j
=1
—
4) of
all4
coefficients are gathered together in TableI.
For
E,
=0,
allI»
vanish because in the static case the G matrix has no imaginary part.V. APPLICATION TOTHE OPTICAL POTENTIAL
In order to check the reliability
of
the density matrix expansion applied toa
complex effective in-teraction, we have calculated the '0+' 0
opticalwhere
Bp(j),a(i) ('Pp(j)&Qadi)
)
(5.6)The results (full curves) are presented in Figs. 7 and 8 for the real and imaginary parts
of
V,„
respectively.%e
compare them with the"exact"
computationof
Ref.
13 (dashed curves}. The agree-ment for ImV,„,
is very good at all separation dis-tances.For
the discussionof
the real part it is useful to roughly divide the rangeof
the separation distanceR
into two intervals.I.
et us call R0 the distance at whichReV»,
has an inflection point.(a) R
)Rp.
This interval is dominated by the nuclear surface propertiesof
the interaction because in the region where the nuclei interpenetrate theK,
=0.
5K„=1
~0 K,=0.
5 K,=1
~0 K,=0.
5 K,=1.
0 K,=0.
5 K,=1
RJIi)
I2J I3JIi)
I2J I3J RJIi)
I2J Ig)I))
I2J I3J Ri I)~ Ip) I3J I)~ I2J Ig) RJ I)~ Ig) Ig) I)~ Ip) I3Jj=1
—
519.42—
1.7061—
0.0639 1.0509—
30.761 55.802—
47.766 178.24 0.89300—
0.30740—
0.12053 9.1548—
14.065 11.292 72.343 0.27056—
0.06102—
0.07316 3.9753—
7.3330 6.2272—
116.90—
0.49381 0.13787 0.10329—
6.2640 10.849—
9.
0502J=2
1936.5—
22.876 38.424—
36.367 282.88—
671.27 623.59—
1058.2—
1.6991—
4.2111 6.5022—
91.
622 163.45—
141.52—
385.83 1.6955—
3.5555 3.5791—
38.71091.
173—
82.406 650.39—
1.2707 4.6082—
5.2046 61.615—
132.03 117.79J=3
—
5391.2 175.19—
227.17 191.34—
950.54 2707.1—
2649.9 3359.3—
13.110 34.202—
36.914 319.86—
634.96 578.26 1085.1—
16.537 22.764—
19.642 136.09—
374.66 352.60—
1925.0 19.815—
31.314 28.871—
216.05 533.39—
497.16j=4
6265.3—
289.25 349.65—
2S2.25 1086.1—
3541.0 3600.5—
3969.4 32.117—
57.614 56.152—
376.59 808.30—
763.18—
1184.6 28.762—
35.986 29.476—
161.54 496.01—
480.85 2176.9—
36.791 50.390 ~—
43.514 255.68—
698.08 671.64density is not higher than the saturation density
of
the nuclear matter. This can be easily seen within the proximity concept. ' In this interval theDME
results are slightly higher than the exact re-sults. The difference shows that the surface proper-tiesof
the exact interaction have somewhat been al-tered by theDME.
This is not surprising because theDME
introduces a truncationof
the higher or-der or-derivativesof
the density matrix.To
find the effectof
this truncation it would be interesting to calculate the surface energyof
semi-infinite slabsof
nuclear matter both with the exact interaction and the energy density resulting fromDME.
(b) R
&Ro.
At such separation distances the overlapping region has reached the nuclear matter density regime and the behaviorof
Re V,',
is essen-tially given by the bulk propertiesof
the nuclear matter. Owing to the independenceof
Reà onE„
and r' ' the discussion given below is valid for anyE,.
For
nuclear matter theDME
approximation givesE/A
= —
16.
85MeV andd
E
=451.
9MeV fm dp2'
(1)-20
-60
-10
-80
4 D (fm)D
(fmI
FIG.
8. Same asFig. 3,but for ImVp$.FIG.
7. A comparison between the density matrix ex-pansion computation ofReV,~& as a function ofD (full lines) and the exact computation of Ref. 13 (dashed lines). The curves marked I, 2, and 3 correspond toE,
=O, 0.5, and 1 fm ', i.e., E~,b—
—
0, 83, and 332,respectively.
overbinding mentioned above. Towards
R
~0,
both potentials are linear, and the difference between their slope is consistent with the values found forQ2 (jp~
For
the imaginary part, the ~' ' dependence plays the dominant role and thus ImV,„,
is insensitive to the saturation density effects described above.In conclusion, we believe to have found areliable parametrization
of
a complex density functional to be used in the calculationof
the heavy-ion optical potential. Our results are given at two different en-ergies and can be applied to any pairof
nuclei once the density and the kinetic energy densityof
the colliding system are known.One
of
us(R.S.
) acknowledges financial support from the Institut Interuniversitaire des Sciences Nucleaires.other hand the exact binding energy is
—
15.59MeV and its second derivative takes the value 575.8 MeVfm at a lower saturation densityp=0.
1752 fm.
Therefore theDME
overbinds the nuclear matter, as already noticed inRef.
28,and alters the curvature at the saturation point. The changes it produces on the nuclear matter constants can ex-plain the difference between the two results. Name-ly,ReV,
~, calculated with theDME
reaches adeeper minimum at shorter separation distances than the exact
ReV,
&,.
This is because thesatura-tion Fermi momentum kF
—
—
1.
49fm ' given by theDME
is larger than the exact one KF 1.37fm-
—
Hence, in the first case, the saturation density isreached when the nuclei interpenetrate further, bringing in the extra attraction associated with the
K.
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