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Inflation of elastomeric circular membranes using

network constitutive equations

Erwan Verron, Gilles Marckmann

To cite this version:

Erwan Verron, Gilles Marckmann. Inflation of elastomeric circular membranes using network

consti-tutive equations. International Journal of Non-Linear Mechanics, Elsevier, 2003, 38 (8), pp.1221-1235.

�10.1016/S0020-7462(02)00069-0�. �hal-01006966�

(2)

using network onstitutive equations

Verron E. 

and Mar kmann G.

Laboratoire de Me anique et Materiaux, Division Stru tures



E ole Centrale de Nantes, BP92101, 44321 Nantes edex 3, Fran e

Tel: (33) 2.40.37.25.14 Fax: (33) 2.40.37.25.73

Abstra t

The present paper deals with the use of network-based hyperelasti onstitutive

equationsinthe ontext ofthinmembranesin ation.Thestudyfo usonthe

in a-tion of plane ir ularmembranesand the materialsareassumed to obey Gaussian

and non-Gaussian statisti al hains network models. The governing equations of

thein ation of axisymmetri thin rubber-like membranes arebrie y re alled. The

materialmodelsareimplementedina numeri al toolthat in orporatesan eÆ ient

B-spline interpolation method and a oupled Newton-Raphson/ar -length solving

algorithm.Twonumeri alexamplesarestudied:thehomogeneousin ationof

spher-i alballoonsand the in ation ofinitiallyplane ir ular membranes. In these ond

example, the in ation pro les and the distributions of extension ratios along the

membrane are extensively analyzed during the in ation pro ess. Both examples

highlight theneedof ana urate modeling ofthe strain-hardeningphenomenon in

elastomers.



Towhom orresponden e shouldbe addressed

(3)

In the last few years, lassi al phenomenologi al onstitutive equations for

rubber-likesolids, su h asMooney-Rivlin orOgden models, are progressively

repla ed by more physi al models based on statisti al onsiderations, in

var-ious engineering appli ations [1℄. The determination of the material

parame-tersofthe onstitutivemodelsisoftenperformedusing lassi alhomogeneous

strain experiments (uniaxial extension or pure shear tests for example). For

biaxial deformation, authors use frequently the bubble in ation te hnique,

that onsistsinin atinganinitiallyplane ir ularthin membrane(see [16,22℄

and more re ently [8,20℄). In this type of experiments, deformations are not

homogeneous and the analysis of experimental data needs eÆ ient numeri al

methodtosolvethein ationproblem.Theproblemof ir ularmembranes

in- ationis lassi allysolved for phenomenologi alrubber-likemodels. Here, we

present some solutions orresponding with new statisti al onstitutive

equa-tions.

The governing equations of the large strains in ation of axisymmetri

mem-branes were established by Green and Adkins[11℄. Then, some authorssolve

the orrespondingproblemby dire tlyintegratingthe system of ordinary

dif-ferentialequationsusingshootingmethods.Bothhyperelasti [17,33℄and

vis- oelasti [30,10℄ onstitutive equations are onsidered. Nevertheless, most of

the works are based on numeri al dis retized methods, su h as nite element

analysis [19,5,15,28℄.Most of the papers fo us onthe numeri al methodsand

onsider simple phenomenologi al onstitutive equations. Very re ently,

Has-sager et al. study the response of polymeri uid membranes under in ation

(4)

tomeri membranesusingnetworkbasedrubber-like onstitutiveequations.In

Se tion 2,the governing equations of the axisymmetri in ation problemare

re alledandthe onstitutiveequationsarepresented.Fourmodelsarestudied:

the lassi alneo-HookeanmodelbasedonGaussianstatisti sandthree hains

models that are based onnon-Gaussian statisti s.Se tion3 is devoted tothe

solving pro edure. The numeri als heme and our original B-spline

interpola-tion, detailed in [29℄, are brie y re alled.The numeri al analysis of spheri al

balloons and ir ular plane membranes are presented in Se tion 4. Finally,

on luding remarks are proposed inSe tion 5.

2 Problem formulation

2.1 Governing equations

We onsider an axially symmetri hyperelasti membrane of uniform

thi k-ness h 0

in its undeformed on guration. The geometry of this membrane

an be des ribed by the ylindri al oordinates of its mid-surfa e. In ea h

- onstant plane, both undeformed and deformed on gurations are redu ed

to one-dimensional urves, as shown in Figure 1. Consider a parti le of

un-deformed oordinates (r 0

;z 0

)of the undeformed membrane. Thispointis

dis-pla edtoanewposition(r;z)inthe deformed on guration. Thethi knessof

the deformedmembraneis denoted h.Every geometri aldata r 0

,z 0

,r, z and

h are fun tions of the ar -length oordinate in the undeformed on guration

s, that varies between 0 and l 0

,the lengthof the initialmembrane.As shown

(5)

 m = v u u t r 2 ;s +z 2 ;s r 2 0;s +z 2 0;s ;  = r r 0 ;  n = h h 0 (1) inwhi h ;s

stands forthe di erentiationwith respe t tos. As the materialis

assumed in ompressible, thethi kness of the deformedbodyissimplyrelated

tothe thi kness inthe naturalstate by:

h= 1  m  h 0 (2)

Underaquasi-stati pressure load, thePrin ipleofVirtual Work anbe

writ-ten in the following form:

Z V0 ÆWdV 0 Z S ÆuP ndS =0 8Æu (3) whereV 0

and Sare respe tivelythevolumeoftheundeformed membraneand

thesurfa e ofthe deformedmembrane.W isthe strainenergy,P nisthe

out-ward oriented blowing pressure and Æu is an admissiblevirtual displa ement

ve tor.Noting that the omponents of nare (z ;s = q r 2 ;s +z 2 ;s ; r ;s = q r 2 ;s +z 2 ;s ),

the previous equation (3)simpli es:

Z l 0 0 2r 0 h 0 (t m Æ m +t Æ ) ds Z l 0 0 2P r (Æuz ;s Ævr ;s )ds =0 (4) where t m and t

are the prin ipal rst Piola-Kir hho stressesrespe tively in

the meridian and ir umferential dire tions, and (Æu;Æv) stand for the

om-ponentsof the virtual displa ement ve tor.

2.2 Network onstitutive equations for elastomers

As mentioned above, the use of statisti al network models for rubber-like

(6)

they agree well with experiments invarious modes of deformation[32℄.

Inthestatisti alapproa h,polymersare onsideredasnetworksoflong exible

hains randomly oriented and joined together by hemi al ross-links. More

details onthis subje t an befound in[26,9℄.

2.2.1 Gaussianstatisti s model

Treloar rstproposedastatisti altreatmentofrubberelasti ity.He onsidered

thatthe on gurationof polymer hains an be des ribed by Gaussian

statis-ti s.Thisleadstothewell-knownneo-Hookean onstitutiveequation[25℄.The

orresponding strainenergy fun tionis:

W = 1 2 nkT(I 1 3) (5)

where n denotes the averagenumberof polymer hains per unit of volume, k

isthe Boltzmann onstant,T isthe absolutetemperatureand nallyI 1

isthe

rst invariant of the stret h tensor, said its tra e. This model only depends

ona unique parameter C R de ned as: C R =nkT (6)

2.2.2 Non-Gaussian statisti s models

Inordertoover omethelimitationsofthepreviousmodelthatisrestri tedto

smallstrains,authorsusenon-Gaussianstatisti stheorytodes ribemole ular

(7)

Gaussianstatisti stheorytomodelthelimitedextensionof hains[18℄. Their

approa his based onthe randomwalk statisti s of anideal phantom hain.

Consider a mole ular hain omposed by N monomer segments of length l.

Its average unstret hed length is p

Nl and its maximum stret hed length is

Nl. Moreover, the strain energyfun tion ofthe hainw an bewritteninthe

following form: w=NkT "  p N +ln sinh # (7)

where  is the extension of the hain and with = L 1  = p N  . L 1 is

the inverse of the Langevin fun tion de ned by L(x) = oth(x) 1=x. The

rst Piola-Kir hho stress inthis single hain isobtained by derivation ofthe

strain energy with respe t tothe extension:

t = w  =kT p NL 1  p N ! (8)

2.2.2.2 p- hains models In order to develop onstitutive equations, a

network of hains whi h strain energy fun tions are given by (7) should be

onsidered. Re ently, Wu and van der Giessen integrate the previous stress

(8) on a unit sphere de ned by its hains density [32℄. Their full network

model agrees well with experiments but ne essitates numeri al integration

pro edures on the sphere. This numeri al integration does not lead to an

eÆ ient implementationin numeri alsoftwares.

Otherauthorsusedthenon-Gaussianstatisti stheorytodevelopsimpler

mod-els whi h do not need numeri al integration. The most employed are the

3- hains and the 8- hains models. Moreover, we mention the approa hed full

(8)

by onsideringprivilegeddire tionsintheunitsphere. Denotingnthe density

ofpolymer hainsasintrodu edfortheneo-Hookeanmodel,itisassumedthat

n=p hainsperunitofvolumeareorientedinea hofthepprivilegeddire tions

inthe undeformed on guration. Then, the previous numeri alintegrationof

the strain energy on the unit sphere is advantageously repla ed by a sum of

p single hain strain energy fun tions weighted by the fa tor n=p. Parti ular

ases of p- hains models are presented inFigure 2.

Thesimplestp- hainsmodelisde nedby onsideringthethreeprin ipalstrain

axes as privileged dire tions. It was derived by James and Guth [13℄ and is

widely known asthe 3- hains model. Figure2(a) presents this model.

Prin i-palstresses(t 3- hains i

) i=1;3

are expressed as fun tionsof prin ipalstret h ratios

( i ) i=1;3 by: t 3- hains i = q  i + 1 3 C R p NL 1  i p N ! (9)

where q is the hydrostati pressure introdu ed by the in ompressibility

as-sumption.

A more re ent model based on non-Gaussian statisti s is the 8- hains model

developed by Arruda and Boy e [2℄. Privileged dire tions are de ned by the

half diagonalsof a ube ontained inthe unit sphere. Figure 2(b) shows this

hains distribution of the model. Its major property is its symmetry with

respe t to the three prin ipalaxes. Therefore, the eight hains are stret hed

with the sameextension ratio, h

, that orresponds tothe stret hing of ea h

halfdiagonals of the ube:

 h = q ( 2 1 + 2 2 + 2 3 )=3 (10)

(9)

t 8- hains i = q  i + 1 3 C R p N  i  h L 1  h p N ! (11)

Finally, we an mention the approa hed full network model proposed by Wu

and vander Giessen [31℄. Authors use a linear ombination of the stresses of

the 3- hainsand 8- hainsmodelstoapproximatethe fullnetwork stressesby:

t fullnetwork i =(1 )t 3- hains i +t 8- hains i (12)

where  isa parameter that isrelated tothe maximalprin ipal stret h ratio:

 = 0:85 p N max( 1 ; 2 ; 3 ) (13)

in whi h the fa tor 0.85 is hosen to give the best orrelation with the full

integration onthe unit sphere.

3 Solution pro edure

In this part, the resolution pro edure used to integrate the problem (4)

as-so iated with one of the stress-strain relationships de ned above is brie y

presented. For more details,the reader an refer to[29℄.

3.1 Dis retized equationsand solution pro edure

Whatever the interpolation method adopted, the membrane is dis retized by

onsideringn+1nodes, (N i ) i=0;n . Ea hnode N i

isde ned by itsundeformed

ar -length oordinate s i

. Its displa ements in radial and axial dire tion are

respe tivelyu i

andv i

(10)

U 2i 1 =u i and U 2i =v i 8i=0;:::;n (14)

Using interpolation formulas (detailed in the next paragraph), the Prin iple

of Virtual Work (4)be omes:

ÆU T [F int (U) F ext (U;p)℄=0 8ÆU T (15) where F int (U) and F ext

(U;p) are the internal and external for es ve tors

re-spe tively, ÆU is the virtual nodal displa ement ve tor and  T

denotes the

transposition. F int

is the dis retized ounterpart of the rst left-hand side

term in Eq. (4) and F ext

orresponds to the se ond term in this equation. It

is obvious that the system (15) is highly non-linear both geometri ally and

by the onstitutiveequation. Thus, aniterativemethodmust be employed to

solve this system and the tangent operator must be derived. This operator

is denoted K and represents the derivative of the out-of-balan e for e ve tor

(F int F ext ) with respe t toU: K= F int U F ext U (16)

The detailed ready-to-program formulas of F int

, F ext

and K are given in[23℄

forthe lassi altwonodes membrane niteelementandin[29℄forouroriginal

B-spline interpolation.

As shown by Beatty for stati in ation [4℄ and Verron et al. for dynami

in ation [27℄, the pressure-displa ement urves orresponding to rubber-like

membranesin ationexhibitlimitpoints.Consequentlya ontinuationmethod

has tobeadopted to ompute the equilibriumpath [24℄. Here, the ar -length

method is implemented. It onsists in ompleting the system of equilibrium

(11)

the present ase, the displa ement ontrol method is onsidered [3℄ and the

additionalequationis:

kUk 2

da 2

=0 (17)

where U is the displa ement in rement ve tor between two equilibrium

pointsand da is the pres ribed ar -length. This equationis addedtothe

pre-vioussystem (15) asa bordered equation and the assembled system is solved

by the lassi alNewton-Raphson algorithm[21℄.

3.2 B-splines interpolation method

In this study, the membrane is interpolated by two ubi splines de ned on

the set of nodes (N i

) i=0;n

, one for ea h oordinater 0 and z 0 : r 0 (s)= n+1 X i= 1 i B i (s=l 0 ) (18) z 0 (s)= n+1 X i= 1 i B i (s=l 0 ) (19) where ( i ) i= 1;n+1 and ( i ) i= 1;n+1

are the parameters of the two splinesand

fun tions B i

(12)

0 B i ()= 8 > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > < > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > > : 0  i 2 (  i 2 ) 3 ( i+1  i 2 )( i  i 2 )( i 1  i 2 )  i 2 < i 1 ( i 2) 2 (i ) ( i+1  i 2 )( i  i 2 )( i  i 1 ) + (i+1 )( i 1 )( i 2 ) ( i+1  i 1 )( i  i 1 )( i+1  i 2 ) + ( i 1) 2 (i+2 ) ( i+1  i 2 )( i  i 1 )( i+2  i 1 )  i 1 < i ( i+1 ) 2 (  i 2 ) (i+1 i 2

)(i+1 i 1)(i+1 i) + ( i+2 )( i+1 )(  i 1 ) (i+2 i 1)(i+1 i 1)(i+1 i)

+ ( i+2 ) 2 (  i ) ( i+2  i 1 )( i+2  i )( i+1  i )  i  < i+1 ( i+2 ) 3 ( i+2  i 1 )( i+2  i )( i+2  i+1 )  i+1 < i+2 0  i+2  (20) where  i

is the redu ed ar -length oordinate of the node N i

and where the

following onventions are adopted:

 i =s 0 =l 0 for i0 (21)  i =s n =l 0 for in (22)

With these two onventions some denominators are equal to 0 and we adopt

the equality: 0=0=0.

In Eqs (18, 19), the n+3 parameters of ea h splines are de ned ina unique

mannerusingtheundeformed oordinatesofthen+1nodesandbytakinginto

a ountend onditions todetermine the twoextra parameters. Dependingon

(13)

1. if the extreme point does not lies in the symmetry axis, both r 0

and z 0

interpolation admit natural end onditions, i.e. the se ond derivative of

both fun tions are equalto zero atthis point,

2. ifthe extreme point liesinthe symmetry axis,the z 0

-spline admitsnatural

end onditionsbutther 0

-splineadmitsHermiteend onditions,i.e.the rst

derivative of the fun tion is pres ribed at the point and, in our ase, is set

tozero.

These boundary onditions provide two additional linear relations between

parameters for both splines, and interpolationformulas (18,19) redu e to:

r 0 (s)= n X i=0 i B r i (s=l 0 ) (23) z 0 (s)= n X i=0 i B z i (s=l 0 ) (24) where(B r i ) i=0;n and(B z i ) i=0;n

arethenewinterpolationbasis,de nedaslinear

ombinationsof the lassi al B-spline fun tionsB i

.

Similarly to isoparametri al nite elements, the displa ement eld (u,v) is

interpolatedby two splines developed on the same basis fun tions:

u(s)= n X i=0 i B r i (s=l 0 ) (25) v(s)= n X i=0 Æ i B z i (s=l 0 ) (26) inwhi h ( i ) i=0;n and (Æ i ) i=0;n

are the parameters of these twosplines.

Some al ulations are now ne essary to establish the dis retized problem

(14)

In this se tion, some numeri alexamples are presented.

Theaimofthispaperisthe omparisonofdi erentnetworkmodels.Thus,the

di erent onstitutive equations have to be tted for the same material using

the same type of experimental data. Here, experimental data orresponding

to the uniaxial extension of a naturalrubber as reported by James et al. are

onsidered[14℄.Moreover, weadoptthematerialparameterspreviously

deter-minedby Wuand vander Giessen[32℄. It istonote that network parameters

N and C R

must be determined for ea h model. But, as the small strain

be-haviouris governed primarilyby C R

, Wu and vander Giessen rst determine

it, and onsider an identi al value of C R

for allmodels, said C R

= 0:4 MPa.

Thenafterwards,the averagenumberof monomersper hain is ttedforea h

onstitutiveequation:N =80forthe3- hains model,N =25forthe 8- hains

model, and nallyN =50for the approa hed fullnetwork model.

4.1 Spheri al balloons

Before examiningthe ase of ir ularmembranes, we onsider the simple

ho-mogeneous in ation of spheri al balloons. This problem was widely studied

for lassi alhyperelasti models, both instati s[4℄and dynami s[27℄. Asthe

deformationremains biaxialinevery materialpoints of the sphere, the

prob-lemredu es toa simple analyti al governing equation that relies the blowing

pressure and the deformed radius. Here, our numeri al approa h is used to

solve the problem and the numeri alresults were su essfully ompared with

(15)

equal to1.0 and the uniform thi kness is 0.01. The semi-spheri al ap is

dis- retized using21nodes. It isassumed thatthe balloonremainsspheri al

dur-ing the in ation, so that no bifur ating phenomenon o urs. Consequently,

the extension ratios are:

 m = ;  = ;  = 1  2 (27)

where istheadimensionaldeformedradius r=r 0

.The urvespressure versus

 are presented in Figure 3 for the four onstitutive equations studied here.

Values of extension ratios and blowing pressures that orrespond to the two

limitpoints, ( I ;P I ) and ( II ;P II

), are presented in Table 1.As shown

else-where,the neo-Hookeanballoonexhibitsonlyone limitpointthat dividesthe

urve into a stable path and an unstable path. For the three other balloons,

the urvesadmittwolimitpointsandthreepaths,twostable(in reasingparts

ofthe urves) andone unstable(de reasingparts ofthe urves).A similar

be-haviour was highlighted previously for the Mooney-Rivlin model [27℄. Let us

examine more pre isely the rst part of the urves that orrespond to small

strains, i.e. for   2:0. First limit points o ur approximately for the same

values of the extension ratio, said  =1:39. This value an be obtained

ana-lyti allyinthe ase ofthe neo-Hookean modeland isequalto 6 p

7.This result

veri esour previous statementthat the smallstrainsbehaviouronly depends

onthematerialparameterC R

,thatisidenti alforthe fourmodels.Forlarger

strains,in ation urves di er. In the ase of the neo-Hookean material, there

isnostrain-hardening(be auseofthe Gaussianassumption)andthe pressure

slowly de reases to zero as the membrane ontinues to in ate. For the three

other models, polymer hains rea h their limit of extensibility for di erent

(16)

The limitvalues of the adimensionalradius, i.e.values forwhi h the limiting

stret h of hains is rea hed, an be simply predi ted for both 3- hains and

8- hains models. In the ase of the 3- hains model, the limit of extensibility

is rea hed when one of the extension ratios  i

tends to p

N in Eq. (9). Here,

re allingthe equibiaxial deformations (27), we have:

 1 = m = ;  2 = = ;  3 = n =1= 2 (28)

Thus the limiting extensibility is obtained for  = p

80  8:94. Note that

in our numeri al simulations, we are not able to over ome   8:0 due to

onvergen e problems. In the ase ofthe 8- hainsmodel,the stret hing ofthe

hains  h

is de ned by Eq. (10). Using(28), it redu es to:

 h = q (2 2 +1= 4 )=3 (29)

and the limit hain extensionis obtained by:

 h

= p

N (30)

with N = 25. The solution of this equation is   6:12. This value an be

seenasthe asymptoti verti alline orrespondingtothepressure urveofthe

8- hains modelin Fig.3.Finally,the response of theapproa hed full network

model is onsidered. Asthe modelisalinear ombinationof the 3- hainsand

the 8- hains models, the model rea hes its limiting extensibility when one of

them rea hes its own limit.Thus, onsidering now that N =50, the limiting

extensibility is obtained for  = p

50  7:07 for the 3- hains model. For the

8- hains model, Eqs (29) and (30) are solved with N = 50 and the limiting

extensibilityisapproximatelyequalto8:66.Thestresses(12)tendstoin nity

(17)

4.2 Cir ular plane membranes

Consider now an initiallyplane ir ularmembrane of radius 1.0and uniform

thi kness0.01.The exterioredge ofthemembraneis lamped.Themembrane

ismeshedusing21nodes.Inthisproblem,thedeformationisnothomogeneous

in the membrane. At the pole (the node inwhi h r =0:), the deformationis

equibiaxial:  m ;  = m ;  n = 1  2 m (31)

and atthe lamped rim,the membrane is under pure shear onditions:

 m ;  =1 ;  n = 1  m (32)

Moreover, it is obvious that the pole lies in the symmetry axis. With our

numeri al approa h, there is no diÆ ulty to satisfy the tangen y ondition,

said r 0

= 0, be ause this boundary ondition is dire tly taken into a ount

in the B r

i

interpolationfun tions (see Se tion 3.2). Using lassi al nite

ele-ments,this ondition an not be stri tly imposed, be ause there is no degree

of freedom that orresponds to r 0

(see [12℄ for example).

First, we study the urves that show the in ating pressure versus the axial

oordinate of the pole (denoted z pole

through the rest of the paper) for the

di erent onstitutive equations. These results are shown in Figure 4. The

orrespondingvaluesoflimitpoints(z poleI ;P I )and(z poleII ;P II )arepresented

inTable 2.Generalaspe ts of the urves are similartothose observed forthe

spheri al balloons with both in reasing and de reasing paths. In the present

(18)

Gaussian onstitutive equations is highly remarkable and the limiting hain

extension is rapidly rea hed as it an be shown by the nal verti al parts of

urves presented in Fig. 4.

Letusnowexaminethein ationpro lesshown inFigure5.Forthe four

mod-els,wepresentpro lesthat orrespondtoz pole

=1.0,2.0,3.0and4.0.Moreover,

the last pro les obtained before numeri al divergen e are also drawn for the

non-Gaussian onstitutive equations.It an beseen that forz pole

equalto1.0

and 2.0 the pro les orresponding to the four models are similar.

Neverthe-less, for higher values of the axial oordinateof the pole, said z pole

3:0, the

pro les orrespondingtothe three non-Gaussianmodelsare similar,but they

highly di er from the shape of the deformed neo-Hookean membranes. The

neo-Hookean bubble is more "spheri al" than the other ones. This example

showsthatthestrain-hardeningofthematerialhasaverysigni antin uen e

of the shapeof in ated membranes.

Thisremark is on rmedbythe thi kness distributionspresented inFigure6.

The thi kness is plottedasfun tionof theundeformed radiusr 0

. Asobserved

by Hassager et al., the neo-Hookean membrane exhibits a strong thinningat

the pole[12℄.Here, we showthatthe same observations anbe madefor

non-Gaussian statisti almodels. As predi ted by the examination of the pro les,

the threenon-Gaussian thi kness distributionsare almostsimilar atthe pole,

and areof thesame orderofmagnitude alongthe membranefor agiven value

of z pole

. The last pro le of ea h non-Gaussian membrane exhibits the same

thi kness distribution that an be seen as the ultimate state before the

o - urren eof hainsrupture. Moreover, thedi eren ebetween theneo-Hookean

(19)

pole

lamped rimare identi al and values at the pole tend tozero (see Fig. 6(a)).

Inthe aseofthethreeothermodels,the thi kness atthe lampedrimevolves

signi antlywithrespe ttoz pole

andthe thinningatthepoleremainssmaller

than inthe neo-Hookean ase.

In order to highlight the in uen e of the strain-hardening modeled by the

inverse Langevin fun tion in onstitutive equations (9), (11) and (12), the

distribution of the in-plane extension ratios  m

and 

along the membranes

arepresentedinFigure7.First,weverifythatthe ir umferentialstret hratio



variesbetween  m

atthe poleand1.0atthe lampedrim.Fig. 7(a)reveals

that,fortheneo-Hookeanbubble,bothdistributionsare similar,aspreviously

demonstrated by Yang and Feng [33℄. Moreover, for z pole

= 5:0, extensions

ratios are equalto 25.0 at the pole. This result has nophysi al meaningand

provestheimportan eofagoodmodelingofstrain-hardeningofelastomersat

large strains. In the ase of the non-Gaussian models, distributions of 

for

thethreemodelsare omparableforthesamedeformationlevel.Distributions

of m

arealsosimilaruntilthematerialrea hesitsstrain-hardeningbehaviour.

Inthis ase,the8- hainsmodelsdistribution(Fig.7( )forz pole

=4:02)di ers

fromthe3- hains andthe approa hedfullnetworkdistributions(Fig.7(b) for

z pole

=5:60 and Fig. 7(d) for z pole

=3:87). In the former ase,  m

is greater

at the lamped extremity than at the pole; in the later,  m

is approximately

uniform for both 3- hains and approa hed full network membranes.This last

observation an be explained by examining the maximum hain extensibility

along the membrane for the three non-Gaussian bubbles. Re all that for the

(20)

 hmax =max( m ; ; n ) (33)

and in our ase, it is always equal to  m

. For the 8- hains model, it is given

by:  hmax = q ( 2 m + 2 + 2 n )=3 (34)

and nally,for the approa hed full network model, it is the greater values of

the 3- hains and 8- hains data:

 hmax =max( m ; ; n ; q ( 2 m + 2 + 2 n )=3) (35)

and here,itis alwaysequalto m

.In thethree ases,as  hmax

tends to p

N,

the material hardens and the asymptoti verti al line in the pressure versus

z pole

diagram is approa hed (Fig. 4). The distributions of  hmax

along the

membranesareplottedversustheundeformedradiusinFigure8,forthe three

non-Gaussiannetworkmodels.Theyarehighlysimilarforthethreemodels:at

the beginningof the in ationthe distributionis uniform,then the membrane

extends more signi antly in the neighbourhood of the pole than near the

lampedrim,and nallyforhighervaluesofz pole

the hainextensibility tends

tobe omeuniformandapproa hesthe limitvalue p

N,whilefewevolutionof

strains takes pla e at the pole. This an be seen as the in ationof a ir ular

membrane with a rigid in lusion at the pole, onsidering that the radius of

this in lusionin reases duringthe in ation.

5 Con luding remarks

In this paper, we have presented some results on erning the in ation of

(21)

onsti-that was proved to be very eÆ ient for large strains in ation of

axisymmet-ri membranes. The non-Gaussian models are implemented and ompared

with the lassi alneo-Hookean onstitutive equation.The in uen e of

strain-hardening on the membrane response is highlighted. It is shown that both

in ation pro les and thi kness distribution are highly in uen ed by the

na-ture of the materialmodel.

These results are of interest in the ontext of the identi ation of material

parameters in biaxial onditions. In order to perform biaxial experiments on

elastomers or heat-softened plasti s, the bubble in ation te hnique is widely

used. In most of the ases, only experimental data obtained at the pole are

onsidered to determine parameters of onstitutive equations, be ause the

deformationisequibiaxialatthispoint.The presentworkshows thatthe

evo-lutionof the membranepro leduring in ationandsome data on erningthe

thi knessdistributionmaybeofgreatinterestinthe hoi eofthe onstitutive

equationthatmustbeadopted,andinthedeterminationofthe orresponding

material parameters. Thus, the numeri al analysis of the entire membrane is

highlysuitable inthe identi ationpro edure.

Referen es

[1℄ J. M. Allport and A. J. Day, Statisti al me hani s material model for the

onstitutivemodellingofelastomeri ompounds.Pro .InstnMe h.EngrsPart

C 210, 575 (1996).

[2℄ E. Arruda and M. C. Boy e, A three-dimensional onstitutive model for the

(22)

[3℄ J. L. Batoz and G. Dhatt, In remental displa ement algorithms for nonlinear

problems.Int. J. Num. Meth. Engng 14, 1262 (1979).

[4℄ M. F. Beatty, Topi s in niteelasti ity: hyperelasti ityof rubber, elastomers,

and biologi altissues -with examples.Appl. Me h. Rev.40, 1699 (1987).

[5℄ J. M. Charrier, S. Shrivastava and R. Wu, Free and onstrained in ation of

elasti membranes in relation to thermoforming - Axisymmetri problems. J.

Strain Analysis 22,115 (1987).

[6℄ M. A. Cris eld, Non-linear nite element analysis of solids and stru tures.

Volume 1: Essentials.John Wileyand SonsLtd, Chi hester, England(1994).

[7℄ C. DeBoor, A pra ti al guide tosplines.Springer, New-York (1978).

[8℄ A. Derdouri, F. Er hiqui, A. Bendada, E. Verron and B. Peseux, Vis oelasti

behaviour of polymer membranes under in ation. Pro eedings of the 13th

International Congress on Rheology, Cambridge UK, August 20-25, 3.394

(2000).

[9℄ M. Doi,Introdu tion to Polymer Physi s. ClarendonPress, Oxford(1996).

[10℄W. W. Feng, Vis oelasti behavior of elastomeri membranes, J. Appl. Me h.

ASME 59, S29 (1992).

[11℄A.E.GreenandJ.E.Adkins,Largeelasti deformations.TheClarendonPress,

Oxford(1960).

[12℄O. Hassager, S. B. Kristensen, J. R. Larsen and J. Neergaard, In ation and

instability of a polymeri membrane. J. Non-Newtonian Fluid Me h. 88, 185

(1999).

[13℄H.M.JamesandE.Guth,Theory oftheelasti propertiesofrubber,J.Chem.

(23)

I. Chara terizationof gumvul anizates. J. Appl. Polym. S i.19, 2033 (1975).

[15℄L. Jiang and J. B. Haddow, A nite element formulation for nite stati

axisymmetri deformationofhyperelasti membranes.Comput. Stru t.57,401

(1995).

[16℄D. D. Joye, G. W. Poehlein and C. D. Denson, A bubble in ation te hnique

forthemeasurementofvis oelasti propertiesinequalbiaxial ow.Trans.So .

Rheol. 17, 421 (1972).

[17℄W. W.KlingbeilandR.T. Shield,Somenumeri alinvestigationsonempiri al

strain energy fun tions in the large axi-symmetri extensions of rubber

membranes.Z. Angew. Math. Phys.15, 608 (1964).

[18℄W. Kuhn and F. Grun, Beziehungen zwi hen elastis hen konstanten und

dehnungsdoppelbre hung ho helastis her sto e. Kolloideits hrift 101, 248

(1942).

[19℄J.T.Oden andT. Sato,Finitestrainsand displa ementsofelasti membranes

by the niteelement method.Int. J.Solids Stru t. 3,471 (1967).

[20℄N. Reuge, F. M. S hmidt, Y.Le Maoult,M. Ra hi k and F. Abbe, Elastomer

biaxial hara terization using bubble in ation te hnique. I: Experimental

investigations. Polym. EngngS i.41, 522 (2001).

[21℄E.RiksandC.C.Rankin,Anin rementalapproa htothesolutionofsnapping

and bu klingproblems. Int. J.Solids Stru t.15, 529 (1979).

[22℄L. R. S hmidt and Carley J. F., Biaxial stret hing of heat-softened plasti

sheets: experimentsand results. Polym.Engng S i.15, 51 (1975).

[23℄J.ShiandG.F.Moita,Thepost- riti alanalysisofaxisymmetri hyper-elasti

membranesbythe niteelementmethod.Comput.MethodsAppl.Me h.Engng

(24)

determination.Comput. Assist.Me h.Engng S i.4,189 (1997).

[25℄L.R.G. Treloar,Theelasti ityofanetworkof long hainmole ules (IandII).

Trans. Faraday So .39, 36,241 (1943).

[26℄L. R. G. Treloar, Physi s of rubber elasti ity, 3rd Edition. University Press,

Oxford(1975).

[27℄E. Verron, R. E. Khayat, A. Derdouri and B. Peseux, Dynami in ation of

hyperelasti spheri al membranes.J. Rheol. 43, 1083 (1999).

[28℄E.Verron,G.Mar kmannandB.Peseux,Dynami in ationofnon-linearelasti

and vis oelasti rubberlike membranes.Int. J. Numer. Meth. Engng.50, 1233

(2001).

[29℄E.Verronand G.Mar kmann,Anaxisymmetri alB-splinesmodelforthe

non-linearfreein ationofrubberlikemembranes.Comput.Meth.Appl.Me h.Engng

190,6271 (2001).

[30℄A. Wineman, On axisymmetri deformations of nonlinear vis oelasti

membranes.J. Non-NewtonianFluid Me h.4,249 (1978).

[31℄P. D. Wu and E. van der Giessen, On improved 3-D non-gaussian network

modelsforrubberelasti ity.Me h. Res. Comm.19, 427 (1992).

[32℄P. D. Wu and E. van der Giessen, On improved network models for rubber

elasti ityandtheirappli ationsto orientationhardeninginglassy polymers.J.

Me h. Phys . Solids 41, 427 (1993).

[33℄W. H. Yang and W. W. Feng, On axisymmetri al deformations of nonlinear

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Fig.1.Problem des ription.

Fig.2.Des riptionofthemostemployedp- hainsmodels:(a)3- hains,(b)8- hains.

Fig.3.Pressureversusadimensional deformedradiusforspheri al balloons.

Fig. 4.Pressureversusaxial oordinateof thepolefortheplane membranes.

Fig. 5. In ation pro les of the ir ular plane membranes: (a) neo-Hookean,

(b) 3- hains, ( ) 8- hains, (d) approa hed full network. Numbers on the urves

stand forthe orresponding in ating pressure.

Fig. 6. Thi kness distribution in the ir ular plane membranes: (a) neo-Hookean,

(b)3- hains,( )8- hains,(d)approa hedfullnetwork.Numbersonthe urvesstand

forthe orrespondingvalue ofz pole

.

Fig. 7. Extension ratios in the ir ular plane membranes (|)  m

, () 

:

(a)neo-Hookean, (b) 3- hains, ( )8- hains,(d) approa hed fullnetwork.Numbers

on the urvesstandfor the orresponding valueof z pole

.

Fig.8.Maximum hainsextensibilityinthe ir ularplanemembranes(|)

distribu-tioninthemembrane,(--)limitvalue p

N:(a)3- hains,(b)8- hains,( )approa hed

fullnetwork.Numberson the urvesstand forthe orrespondingvalueof z pole

(26)

Model  I P I  II P II Neo-hookean 1.40 4.96e-03  

3- hains 1.40 5.04e-03 5.71 1.97e-03

8- hains 1.39 5.13e-03 3.92 2.88e-03

Approa hedfullnetwork 1.39 5.08e-03 5.10 2.26e-03

Table 1

Limitpointsforspheri alballoons.Cir lesrepresenttheanalyti al solutions.

Model z poleI P I z poleII P II Neo-hookean 1.16 7.52e-03  

3- hains 1.23 7.73e-03 3.16 6.09e-03

8- hains 1.17 8.01e-03 2.17 7.64e-03

Approa hed fullnetwork 1.26 7.84e-03 2.83 6.66e-03

Table 2

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